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Tm <74686520> Tj 1 0 0 1 519.84 146.40 Tm <7374726573736573> Tj 0.72 Tc 1 0 0 1 317.28 134.16 Tm <6F6620> Tj 1 0 0 1 331.20 134.16 Tm <74686520> Tj 1 0 0 1 349.44 133.92 Tm <6465636F6D706F736974696F6E20> Tj 1 0 0 1 419.52 134.16 Tm <70726F636573732E20> Tj 1 0 0 1 460.56 133.68 Tm <54686520> Tj 1 0 0 1 482.88 133.68 Tm <646576656C6F706D656E7420> Tj 1 0 0 1 544.32 133.44 Tm <6F66> Tj ET endstream endobj 4 0 obj 22761 endobj 5 0 obj << /Type /Font /Subtype /Type1 /BaseFont /Helvetica /Encoding /WinAnsiEncoding >> endobj 6 0 obj << /Length 7 0 R >> stream Brazlhan Journalof ChemicalEngineering Vol. 20, No. 03, pp.213 - 282, July - September 2003 jrtISSN 0104-6632Printed in Brazil Ir-Ru/AlzO: CATALYSTS USED IN SATELLITE PROPULSION T.G.Soares Netor, J.Gobbo-Ferreirar, A.J.G.Cobo2 and G.M.Cruz3:Lai-.orlrtino Assocraclo cc'Combusto e Propulso, Instituto Nacional de Pesquisas EspaciarsFone t01lr-560-9-68. r0llt-560-925 l. Far: (012) 561-1992,Cr P 0. 116-0-000. Crchoeira Paulista - SP. Brazil:Fr;udr,ie de Encenhrri: Oumtcr. L'nir ersitadc Estaclual de CampinasCr P r,, j l:o\:-u-!. C.rttrirr: - SP. Br:rziF,re uJrJc Je Engenh,iril Quntic,t Jc- Lrrrc'riiC.P. 16. 11600-000. Ltrrcn: - SP. Brrzrl(Received:rrgrst 31,200 1 :,\ccepred. ,1pril -t. )r trl-t ,Abstract: IrlAl2Oj, Ir-Ru/AlzO: and Ru/Al2Or, catalysts with total metal contents of 30% uere preparedusing the methods of incipient wetness and incipient coimpregnation wetness and were tested in a 2Nmicrothruster. Their performances were then compared with that of the Shell 405 commercial catalyst (30%IrlAlzO:). Tests were performed in continuous and pulsed regimes, where there are steep temperature andpressure gradients, from ambient values up to 650 "C and 14 bar. Performance stability, thrust produced,temperature and stagnation pressure in the chamber and losses of mass were analyzed and compared to thecorresponding parameters in Shell 405 tests. It was observed that the performance of all the above-mentionedcatalysts was comparable to that of the commercial one, except for in loss of mass, where the values washigher, which was attributed to the lower mechanical resistance of the support.Keywords: iridium catalyst, ruthenium catalyst, iridium-ruthenium bimetallic catalyst, hydrazine decomposition,spacecraft propulsion, textural properties, TEM, chloride infl uence. INTRODUCTIONThe use of hydrazine monopropellant in thepropulsion systems of satellites has opened up newhorizons in human knowledge, directly affecting theexploration of natural resources in interplanetaryspace and on earth, weather forecasting, radio andTV communications earth aerial and maritimenavigation [Schmidt, 1984]. The Jet PropulsionLaboratory, JPL, was responsible for pioneeringresearch in this field [Altman and Thomas, 1949].To be considered a good catalyst the productmust be able to start the decomposition of coldhydrazine (at temperatures as low as 215K) with atime delay of less than 15 ms. In addition, itsperformance must remain acceptable during theentire expected life of the satellite. There are three main phenomena responsible fordegradation of a catalyst: mechanical breakup causedby shear external forces and breakup of the grainscaused by a fast increase in internal pressure, both ofwhich contribute to the loss of mass of the catalyst,and the decrease in total specific area produced bythe elevated temperatures that can be attained in thebed, which result in an obstruction of pores andmetal occlusion due to transformations of thestlucture of the support [Schmidt, 1984].Several compounds were tested in hydrazinedecomposition catalysis. They were consideredinadequate for space applications because of theirinaptitude to start the reaction at lowtemperatures (cold start) with acceptable time delaysand their poor mechanical resistance to the stressesof the decomposition process. The development of endstream endobj 7 0 obj 3344 endobj 8 0 obj << /Length 27 >> stream % CANON_PFINF_TYPE0_TEXTON endstream endobj 9 0 obj << /Length 44 >> stream q 595.20 0 0 841.68 0.00 0.00 cm /Obj2 Do Q endstream endobj 10 0 obj << /Type /Page /MediaBox [ 0 0 595.20 841.68 ] /Parent 11 0 R /Resources << /Font << /F3 5 0 R >> /XObject << /Obj2 2 0 R >> /Subtype 6 0 R /ProcSet [ /PDF /Text /ImageB /ImageC /ImageI ] >> /Contents [ 8 0 R 9 0 R 3 0 R ] >> endobj 13 0 obj << /Type /XObject /Subtype /Image /Width 2480 /Height 3507 /BitsPerComponent 1 /ColorSpace /DeviceGray /Filter /CCITTFaxDecode /DecodeParms << /K -1 /Columns 2480 >> /Length 101488 >> stream &ݹ"? `x2H pdRU H 0 6$IH ĀP$$FGhFR"Z# 5ai5Dx+` Ȉj-Y. 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623.52 Tm <494E504520> Tj 1 0 0 1 401.52 624.96 Tm <746F20> Tj 1 0 0 1 416.40 617.52 Tm <2D3131752220> Tj 1 0 0 1 442.08 626.88 Tm <6D6963726F20> Tj 1 0 0 1 471.60 628.08 Tm <616E6420> Tj 1 0 0 1 490.56 629.04 Tm <6D6163726F706F72657320> Tj 1 0 0 1 545.28 631.44 Tm <6C6E> Tj 0.48 Tc 1 0 0 1 53.04 597.12 Tm <686F7572732C20> Tj 1 0 0 1 83.52 598.56 Tm <7768656E20> Tj 1 0 0 1 110.40 599.52 Tm <72686520> Tj 1 0 0 1 127.20 600.24 Tm <636172616C79737220> Tj 1 0 0 1 164.40 601.68 Tm <62656420> Tj 1 0 0 1 183.60 602.64 Tm <7265616368657320> Tj 1 0 0 1 220.08 604.32 Tm <2C2254726666693B20> Tj 1 0 0 1 280.32 599.52 Tm <693A20> Tj 1 0 0 1 317.76 618.72 Tm <5E3131225E722A227220> Tj 1 0 0 1 359.52 610.56 Tm <70726F647563742720> Tj 1 0 0 1 400.08 612.24 Tm <6120> Tj 1 0 0 1 408.72 612.72 Tm <70726F6365737320> Tj 1 0 0 1 446.40 614.16 Tm <6F6620> Tj 1 0 0 1 459.12 614.88 Tm <636F6E74726F6C6C656420> Tj 1 0 0 1 508.08 617.28 Tm <67656E65726174696F6E> Tj 0.24 Tc /F3 16.0 Tf 1 0 0 1 53.76 584.16 Tm <6869676820> Tj 1 0 0 1 76.32 585.12 Tm <617320> Tj 1 0 0 1 89.52 585.84 Tm <3133373320> Tj 1 0 0 1 113.52 586.80 Tm <4B2C20> Tj 1 0 0 1 127.20 587.28 Tm <6F6E20> Tj 1 0 0 1 141.36 588.24 Tm <2AED746E20> Tj 1 0 0 1 164.40 588.96 Tm <6120> Tj 1 0 0 1 171.84 589.20 Tm <72696D6520> Tj 1 0 0 1 194.64 590.40 Tm <64657261767320> Tj 1 0 0 1 225.84 591.60 Tm <6F6620> Tj 1 0 0 1 237.60 592.32 Tm <7265737320> Tj 1 0 0 1 257.04 593.04 Tm <7468616E20> Tj 1 0 0 1 280.32 594.00 Tm <313020> Tj 1 0 0 1 318.72 580.56 Tm <3BEF224C224A3BEF2C4A2E7423313122CFEF2EEF20> Tj 1 0 0 1 440.64 588.48 Tm <7269EFEF3A694AEF2C22EFEF74EF23692224> Tj 0.96 Tc /F3 10.0 Tf 1 0 0 1 54.24 571.20 Tm <6D7322> Tj 0.24 Tc /F3 12.0 Tf 1 0 0 1 69.12 559.20 Tm <5368657520> Tj 1 0 0 1 95.28 560.40 Tm <34303520> Tj 1 0 0 1 115.44 561.12 Tm <68617320> Tj 1 0 0 1 134.40 561.84 Tm <616E20> Tj 1 0 0 1 148.32 562.56 Tm <656C65766174656420> Tj 1 0 0 1 189.12 564.48 Tm <6D6574616C20> Tj 1 0 0 1 217.44 565.68 Tm <636F6E72656E7220> Tj 1 0 0 1 253.92 567.12 Tm <6F6620> Tj 1 0 0 1 266.88 567.60 Tm <61626F757420> Tj 1 0 0 1 319.44 564.24 Tm <3170317279693A312C3A3A3A6922316C7420> Tj 1 0 0 1 430.32 575.28 Tm <74686520> Tj 1 0 0 1 445.92 575.76 Tm <666F6C6C6F77696E6720> Tj 1 0 0 1 489.60 577.68 Tm <6368617261637465> Tj 0.72 Tc /F3 11.0 Tf 1 0 0 1 55.44 545.76 Tm <3330376F2C20> Tj 1 0 0 1 84.96 547.44 Tm <776869636820> Tj 1 0 0 1 118.80 548.88 Tm <70726576656E747320> Tj 1 0 0 1 163.44 550.56 Tm <68796472617A696E6520> Tj 1 0 0 1 213.84 552.72 Tm <7272222A22702222222C3B3B2A7120> Tj 1 0 0 1 321.60 557.52 Tm <6C29546F74616C737065636966696320> Tj 1 0 0 1 398.16 560.64 Tm <617465613A7AEF327272CC6C673B20> Tj 1 0 0 1 495.84 559.44 Tm Tj 0.48 Tc 1 0 0 1 55.92 533.28 Tm <6465657020> Tj 1 0 0 1 82.08 534.48 Tm <696E20> Tj 1 0 0 1 96.00 534.96 Tm <747420> Tj 1 0 0 1 104.88 527.28 Tm <2220> Tj 1 0 0 1 115.20 528.00 Tm <2275747574792A692720> Tj 1 0 0 1 155.04 537.84 Tm <677275696E2C20> Tj 1 0 0 1 183.12 538.80 Tm <7468657265627920> Tj 1 0 0 1 222.00 540.72 Tm <70726F75694A696ECB2D20> Tj 1 0 0 1 270.72 542.88 Tm <676F6FE320> Tj 1 0 0 1 320.88 544.80 Tm <7A6C20> Tj 1 0 0 1 332.64 547.92 Tm <7022742220> Tj 1 0 0 1 355.92 546.48 Tm <75E16C6F2A2220> Tj 1 0 0 1 391.92 548.40 Tm <2868756D696420> Tj 1 0 0 1 426.48 549.84 Tm <706F696E74293A20> Tj 1 0 0 1 459.36 551.04 Tm <3027373120> Tj 1 0 0 1 481.68 552.00 Tm <636D272F673A> Tj 0.48 Tc 1 0 0 1 56.16 520.56 Tm <6865617420> Tj 1 0 0 1 81.84 521.76 Tm <646973736970752C2C6F6E20> Tj 1 0 0 1 137.76 523.92 Tm <75EC3022696C222A20> Tj 1 0 0 1 206.88 527.04 Tm Tj 1 0 0 1 237.84 528.48 Tm Tj 1 0 0 1 270.72 529.68 Tm Tj 1 0 0 1 321.12 531.84 Tm Tj 1 0 0 1 333.60 532.56 Tm <637475696E20> Tj 1 0 0 1 361.44 533.76 Tm <6469616D657465723A20> Tj 1 0 0 1 406.08 535.92 Tm <30273620> Tj 1 0 0 1 422.88 536.64 Tm <746F20> Tj 1 0 0 1 434.40 537.12 Tm <30273820> Tj 1 0 0 1 451.20 537.84 Tm <6D6D3B> Tj 0.48 Tc /F3 19.0 Tf 1 0 0 1 56.88 507.84 Tm <6D696E696D756D20> Tj 1 0 0 1 112.56 510.24 Tm <7272696469756D20> Tj 1 0 0 1 156.72 512.16 Tm <692E2D20> Tj 1 0 0 1 174.72 512.88 Tm <6F22706FEF6974227120> Tj 1 0 0 1 228.48 505.44 Tm <64EF3A2A3A6920> Tj 1 0 0 1 321.84 518.40 Tm <5E7420> Tj 1 0 0 1 334.08 506.16 Tm Tj 0.72 Tc /F3 13.0 Tf 1 0 0 1 57.12 494.88 Tm <48EF3B27696C3A20> Tj 1 0 0 1 107.76 488.88 Tm <223B3B3B3B3A20> Tj 1 0 0 1 147.60 498.96 Tm <2A27ECEC636820> Tj 1 0 0 1 178.32 500.16 Tm <68E27320> Tj 1 0 0 1 197.28 500.88 Tm <696E74657272696E6B656420> Tj 1 0 0 1 249.12 503.04 Tm <6D6963726F20> Tj 1 0 0 1 278.16 504.24 Tm <616E6420> Tj 1 0 0 1 323.28 490.32 Tm <222C3B3A3A3A22EF3A69272C2722222E693B4A2E3A27742C2C693B3B3B27273B723A6C6F736F3120> Tj 1 0 0 1 507.84 501.12 Tm <726F20> Tj 1 0 0 1 523.92 501.84 Tm <6F627275696E20> Tj 1 0 0 1 554.88 503.04 Tm <75> Tj 0.72 Tc /F3 11.0 Tf 1 0 0 1 58.08 482.16 Tm <2C6EE222726F706F72222C20> Tj 1 0 0 1 112.80 482.88 Tm <5B5363686D6964742720> Tj 1 0 0 1 159.84 486.72 Tm <313938345D2720> Tj 1 0 0 1 272.88 485.28 Tm <2720> Tj 1 0 0 1 323.28 492.72 Tm <6F6620> Tj 1 0 0 1 335.76 493.44 Tm <696E63697069656E7420> Tj 1 0 0 1 378.00 495.60 Tm <727665746E65737320> Tj 1 0 0 1 416.88 495.36 Tm <664372757A> Tj 0.72 Tc 1 0 0 1 72.72 470.16 Tm <6F7468657220> Tj 1 0 0 1 103.68 471.60 Tm <636F756E747269657320> Tj 1 0 0 1 150.72 473.52 Tm <636F6E747269627574656420> Tj 1 0 0 1 207.36 475.68 Tm <746F20> Tj 1 0 0 1 221.76 476.40 Tm <74686520> Tj 1 0 0 1 240.72 477.36 Tm <726573656172636820> Tj 1 0 0 1 284.16 479.04 Tm <6F6E20> Tj 1 0 0 1 323.76 480.24 Tm <2D2E2C226AEF6F6E74746E7420> Tj 1 0 0 1 387.60 483.12 Tm <6F6620> Tj 1 0 0 1 400.08 483.60 Tm <3330C74C2720> Tj 1 0 0 1 426.00 484.80 Tm <746872656520> Tj 1 0 0 1 451.68 486.00 Tm <69726E707265676E6174696F745D20> Tj 1 0 0 1 513.84 488.64 Tm <737465707320> Tj 1 0 0 1 538.80 490.32 Tm <5C5C657265> Tj 0.72 Tc 1 0 0 1 59.04 456.96 Tm <68796472617A696E656465636F6D706F736974EFE0EF222D75EF4A7972747422226E6E6F6C6F677920> Tj 1 0 0 1 265.44 465.84 Tm <72685D725F2C5F3A20> Tj 1 0 0 1 324.24 467.52 Tm <6E222E2E2C3B72272E2D482C722E67212E22665D6420> Tj 1 0 0 1 440.64 472.56 Tm <736F726E74696F6E20> Tj 1 0 0 1 482.64 474.96 Tm <7572726820> Tj 1 0 0 1 508.32 475.68 Tm <6120> Tj 1 0 0 1 518.88 476.16 Tm <6672656520> Tj 1 0 0 1 542.40 477.36 Tm <61636964> Tj 0.72 Tc 1 0 0 1 59.76 444.00 Tm <74686520> Tj 1 0 0 1 76.56 444.96 Tm <636173652C20> Tj 1 0 0 1 101.52 445.92 Tm <666F7220> Tj 1 0 0 1 117.84 446.64 Tm <696E7374616E63652C2D696E20> Tj 1 0 0 1 172.32 449.04 Tm <722E756E2E2E2C20> Tj 1 0 0 1 209.04 450.72 Tm <776839723320> Tj 1 0 0 1 239.28 451.92 Tm <636672CA736E6F277220> Tj 1 0 0 1 324.96 455.04 Tm <2E6F6E2E2E2C69FA2C696F6E2D6F6620> Tj 1 0 0 1 402.24 458.40 Tm <3020> Tj 1 0 0 1 410.64 458.88 Tm <3620> Tj 1 0 0 1 419.76 459.36 Tm <5C20> Tj 1 0 0 1 431.76 460.32 Tm <2A617320> Tj 1 0 0 1 452.16 460.56 Tm <7573656420> Tj 1 0 0 1 476.88 461.76 Tm <617320> Tj 1 0 0 1 489.36 462.24 Tm <74686520> Tj 1 0 0 1 506.40 463.20 Tm <707265637572736F7220> Tj 1 0 0 1 552.24 464.88 Tm <6F66> Tj 0.96 Tc 1 0 0 1 60.24 431.52 Tm <77617320> Tj 1 0 0 1 85.44 432.48 Tm <646576656C6F70656420> Tj 1 0 0 1 139.44 432.96 Tm <726E72222A722E27EFF4313B2C20> Tj 1 0 0 1 217.44 438.48 Tm <76616C656E74696E652E20> Tj 1 0 0 1 276.00 440.64 Tm <316731692E2E20> Tj 1 0 0 1 325.44 442.08 Tm <2C742E20> Tj 1 0 0 1 346.08 434.88 Tm <222E6C6969722E20> Tj 1 0 0 1 379.20 444.48 Tm <726E6574616C20> Tj 1 0 0 1 410.40 446.16 Tm <70686173652E20> Tj 1 0 0 1 445.44 447.36 Tm <5468697320> Tj 1 0 0 1 472.32 448.80 Tm <70726F6475637220> Tj 1 0 0 1 512.88 450.96 Tm Tj 1 0 0 1 535.68 451.68 Tm <656974686572> Tj 0.72 Tc 1 0 0 1 60.96 418.56 Tm <5363686D6964742C20> Tj 1 0 0 1 103.92 420.48 Tm <316767345D20> Tj 1 0 0 1 131.76 421.68 Tm <616E6420> Tj 1 0 0 1 150.72 422.64 Tm <4765726D616E6C2E20> Tj 1 0 0 1 197.28 425.04 Tm <2A686572652E6120> Tj 1 0 0 1 235.20 426.48 Tm <63617261727220> Tj 1 0 0 1 261.60 427.44 Tm <737220> Tj 1 0 0 1 271.68 427.92 Tm <63616972656420> Tj 1 0 0 1 325.92 429.60 Tm <707265706172656420> Tj 1 0 0 1 367.68 431.28 Tm <696E20> Tj 1 0 0 1 378.96 431.76 Tm <74686520> Tj 1 0 0 1 395.28 432.48 Tm <6C61626F7261726F722920> Tj 1 0 0 1 444.00 434.64 Tm <61272E20> Tj 1 0 0 1 454.32 435.12 Tm <725C704520> Tj 1 0 0 1 481.92 436.32 Tm <6F7220> Tj 1 0 0 1 493.44 437.04 Tm <70757263686173656420> Tj 1 0 0 1 540.96 439.20 Tm <66726F6D> Tj 0.72 Tc 1 0 0 1 61.44 405.84 Tm <4B4320> Tj 1 0 0 1 80.16 406.80 Tm <313220> Tj 1 0 0 1 92.64 407.28 Tm <4720> Tj 1 0 0 1 108.48 408.00 Tm <77617320> Tj 1 0 0 1 133.20 409.20 Tm <70726F647563656420> Tj 1 0 0 1 181.44 411.12 Tm <622D7220> Tj 1 0 0 1 200.64 411.84 Tm <726169696366726C6C696C20> Tj 1 0 0 1 257.04 412.56 Tm <69486F6E756E672E20> Tj 1 0 0 1 326.16 416.64 Tm <69722D272220> Tj 1 0 0 1 346.08 430.32 Tm <2D456E732E69CC7222726120> Tj 1 0 0 1 408.24 420.48 Tm <636F72706F726172696F6E2C20> Tj 1 0 0 1 476.64 423.60 Tm <4672616E636520> Tj 1 0 0 1 520.80 425.52 Tm <5072696F7220> Tj 1 0 0 1 554.16 426.96 Tm <696F> Tj 0.72 Tc 1 0 0 1 62.88 393.36 Tm <313937343B20> Tj 1 0 0 1 89.04 394.56 Tm <48617272756E6720> Tj 1 0 0 1 127.44 396.24 Tm <657420> Tj 1 0 0 1 138.24 396.48 Tm <616C2E2E20> Tj 1 0 0 1 153.84 397.44 Tm Tj 1 0 0 1 181.44 398.40 Tm Tj 1 0 0 1 223.92 400.32 Tm <3139673B726C2E20> Tj 1 0 0 1 327.12 403.92 Tm <696D707265676EE374696F6E2720> Tj 1 0 0 1 393.60 407.04 Tm <74686520> Tj 1 0 0 1 412.56 407.76 Tm <737570706F727420> Tj 1 0 0 1 450.48 409.68 Tm <77617320> Tj 1 0 0 1 472.80 410.40 Tm <6F76656E20> Tj 1 0 0 1 498.72 411.60 Tm <647269656420> Tj 1 0 0 1 526.32 413.04 Tm <617420> Tj 1 0 0 1 539.04 413.76 Tm <3339334B> Tj 0.48 Tc 1 0 0 1 76.56 381.36 Tm <54686520> Tj 1 0 0 1 97.68 382.08 Tm <75736520> Tj 1 0 0 1 116.88 383.04 Tm <6F7220> Tj 1 0 0 1 130.08 383.52 Tm <2E6F747472226E69756D2C20> Tj 1 0 0 1 182.64 386.16 Tm <776869636820> Tj 1 0 0 1 214.32 387.12 Tm <697320> Tj 1 0 0 1 225.12 387.84 Tm <66617220> Tj 1 0 0 1 241.44 388.32 Tm <6368656170657220> Tj 1 0 0 1 279.84 390.00 Tm <7468616E20> Tj 1 0 0 1 327.36 391.20 Tm <663A6C20> Tj 1 0 0 1 346.32 392.16 Tm <3B74683B3B74742220> Tj 1 0 0 1 390.72 394.08 Tm Tj 1 0 0 1 420.00 387.60 Tm <2275EC6E20> Tj 1 0 0 1 446.64 396.72 Tm <69746E702722676E6174696F6E20> Tj 1 0 0 1 511.20 399.60 Tm <736F6C69647320> Tj 1 0 0 1 542.40 401.04 Tm <77657265> Tj 0.48 Tc 1 0 0 1 63.12 367.92 Tm <6972696469756D2C20> Tj 1 0 0 1 102.96 369.60 Tm <697320> Tj 1 0 0 1 114.96 370.08 Tm <6120> Tj 1 0 0 1 124.32 370.56 Tm <7665727920> Tj 1 0 0 1 148.08 371.76 Tm <70726F6D6973696E6720> Tj 1 0 0 1 197.76 373.68 Tm <616C7265726E6174697671272A696922EC7620> Tj 1 0 0 1 286.56 377.52 Tm <72222C20> Tj 1 0 0 1 328.08 378.48 Tm <61726922E120> Tj 1 0 0 1 354.72 379.68 Tm <697220> Tj 1 0 0 1 367.20 380.40 Tm <2A2275756D20> Tj 1 0 0 1 405.60 382.08 Tm <666F7220> Tj 1 0 0 1 423.36 382.80 Tm <7420> Tj 1 0 0 1 431.52 383.28 Tm <686F757220> Tj 1 0 0 1 456.00 384.24 Tm Tj 1 0 0 1 475.68 385.20 Tm <7265647563656420> Tj 1 0 0 1 514.32 386.88 Tm <696E20> Tj 1 0 0 1 526.56 387.36 Tm <487A20> Tj 1 0 0 1 541.44 388.08 Tm <666C6F7727> Tj 0.24 Tc /F3 20.0 Tf 1 0 0 1 64.08 342.24 Tm <23EF2E3B6C272272624A2A693A72272A2AEF4A2C2222272C2C20> Tj 1 0 0 1 233.28 349.44 Tm <2D2C586C6C696922EF3B20> Tj 1 0 0 1 328.80 355.20 Tm <22273B6922694A275E312CE3222EEF3B2227722C2C2C20> Tj 1 0 0 1 448.32 358.32 Tm <636F6E7461696E696E6720> Tj 1 0 0 1 498.48 360.48 Tm <3330252C3574617220> Tj 1 0 0 1 548.40 362.88 Tm <776173> Tj 0.48 Tc /F3 11.0 Tf 1 0 0 1 65.04 329.52 Tm <616E6420> Tj 1 0 0 1 85.20 330.48 Tm <61706F67656520> Tj 1 0 0 1 120.96 331.92 Tm <73617465747469746520> Tj 1 0 0 1 160.08 333.84 Tm <6D2D6F69E372722D69732272722A6964742C20> Tj 1 0 0 1 242.40 337.44 Tm <31393834312C20> Tj 1 0 0 1 274.32 338.88 Tm <776865726520> Tj 1 0 0 1 329.76 340.56 Tm <7027223B3B3B3BE320> Tj 1 0 0 1 374.16 342.24 Tm <757920> Tj 1 0 0 1 390.72 342.96 Tm <697472652E61626F766C20> Tj 1 0 0 1 439.68 338.16 Tm <276D6574686F646FCC6F67792720> Tj 1 0 0 1 508.56 348.24 Tm <7573696E2D672D617320> Tj 1 0 0 1 552.48 350.16 Tm <746865> Tj 0.48 Tc 1 0 0 1 65.28 317.04 Tm <746F72616C20> Tj 1 0 0 1 88.32 318.00 Tm <6275726E696E6720> Tj 1 0 0 1 126.24 319.68 Tm <72696D6520> Tj 1 0 0 1 149.52 320.64 Tm <7265616368657320> Tj 1 0 0 1 186.48 322.08 Tm <6120> Tj 1 0 0 1 194.64 322.56 Tm <6D6178696D756D20> Tj 1 0 0 1 241.20 324.48 Tm <6F6620> Tj 1 0 0 1 255.60 324.96 Tm <3520> Tj 1 0 0 1 264.24 325.44 Tm <6D696E757465732720> Tj 1 0 0 1 330.24 325.20 Tm <6E274A3B3B3B2720> Tj 1 0 0 1 374.64 329.52 Tm Tj 1 0 0 1 386.40 330.00 Tm <27E0EC7527696F6E20> Tj 1 0 0 1 424.80 326.16 Tm <2D6F6C20> Tj 1 0 0 1 438.00 326.16 Tm <2D5275636C3A20> Tj 1 0 0 1 471.12 334.08 Tm <7769746820> Tj 1 0 0 1 495.36 335.04 Tm <6120> Tj 1 0 0 1 504.00 335.52 Tm <6672656520> Tj 1 0 0 1 525.36 336.48 Tm <48436C20> Tj 1 0 0 1 548.40 337.44 Tm <61636964> Tj 0.48 Tc 1 0 0 1 66.00 304.32 Tm <496E20> Tj 1 0 0 1 78.00 304.80 Tm <7468697320> Tj 1 0 0 1 97.68 305.76 Tm <6361736520> Tj 1 0 0 1 120.48 306.72 Tm <6120> Tj 1 0 0 1 128.88 306.96 Tm <2C757465747469742220> Tj 1 0 0 1 166.80 308.64 Tm <6C61756E6368696E6720> Tj 1 0 0 1 214.08 310.56 Tm <7573657361626F757420> Tj 1 0 0 1 264.96 312.72 Tm <38303020> Tj 1 0 0 1 284.64 313.92 Tm <6720> Tj 1 0 0 1 293.28 313.92 Tm <6F6620> Tj 1 0 0 1 330.96 314.88 Tm <74222222EF22FC227469226E20> Tj 1 0 0 1 402.96 318.00 Tm <6F6620> Tj 1 0 0 1 423.36 318.96 Tm <3027323F2E4E2720> Tj 1 0 0 1 465.12 321.36 Tm <70757263686173656420> Tj 1 0 0 1 521.04 323.52 Tm <66726F6D20> Tj 1 0 0 1 553.68 324.72 Tm <746865> Tj 0.48 Tc 1 0 0 1 66.48 291.60 Tm <636174616C7973742E20> Tj 1 0 0 1 106.08 293.28 Tm <4163636F7264696E6720> Tj 1 0 0 1 156.00 295.44 Tm <726F20> Tj 1 0 0 1 167.52 295.92 Tm <7268652E456E67656C7420> Tj 1 0 0 1 216.00 289.92 Tm <226720> Tj 1 0 0 1 232.80 295.68 Tm <675E22726E22EC3B3AFA2A20> Tj 1 0 0 1 331.20 302.16 Tm <657474226669745E744A20> Tj 1 0 0 1 379.68 304.32 Tm Tj 1 0 0 1 472.56 308.64 Tm <4E22746F20> Tj 1 0 0 1 497.28 309.60 Tm <657420> Tj 1 0 0 1 508.08 310.08 Tm <61CC272720> Tj 1 0 0 1 525.12 311.04 Tm <313939395D27> Tj 0.48 Tc 1 0 0 1 66.96 278.64 Tm <636F737420> Tj 1 0 0 1 89.76 279.60 Tm <6F6620> Tj 1 0 0 1 103.68 280.32 Tm <74686520> Tj 1 0 0 1 122.16 281.04 Tm <6972696469756D20> Tj 1 0 0 1 159.84 282.72 Tm <6D6574616C20> Tj 1 0 0 1 189.36 284.16 Tm <707265637572736F7220> Tj 1 0 0 1 236.16 286.08 Tm <727320> Tj 1 0 0 1 248.64 286.56 Tm Tj 1 0 0 1 283.68 288.00 Tm <55532420> Tj 1 0 0 1 345.60 289.92 Tm Tj 1 0 0 1 418.08 293.28 Tm <6D6574686F647320> Tj 1 0 0 1 462.00 295.20 Tm <7765726520> Tj 1 0 0 1 490.08 296.40 Tm <656D706C6F79656420> Tj 1 0 0 1 539.76 299.04 Tm <696E20> Tj 1 0 0 1 554.64 299.28 Tm <746865> Tj 0.48 Tc 1 0 0 1 72.72 266.16 Tm <32372E4F4F6C6772616D2C20> Tj 1 0 0 1 130.08 268.80 Tm <776869CC6520> Tj 1 0 0 1 164.40 270.24 Tm <72757468656E69756D20> Tj 1 0 0 1 219.36 272.64 Tm <636F73727320> Tj 1 0 0 1 251.04 273.84 Tm <61626F757420> Tj 1 0 0 1 284.40 275.28 Tm <75732420> Tj 1 0 0 1 332.64 274.08 Tm <6F2A6E2A6931392220> Tj 1 0 0 1 387.36 271.20 Tm <22EF6C74272D6E226C65727A6F7220> Tj 1 0 0 1 456.96 282.24 Tm <636174616C7973747320> Tj 1 0 0 1 499.68 282.24 Tm <66736F6172657320> Tj 1 0 0 1 535.68 285.60 Tm <4E65746F20> Tj 1 0 0 1 560.88 286.80 Tm <6574> Tj 0.48 Tc /F3 13.0 Tf 1 0 0 1 68.40 253.44 Tm <2C2E6769EFEFFC20> Tj 1 0 0 1 117.84 242.64 Tm <74686520> Tj 1 0 0 1 135.36 243.36 Tm <7261737420> Tj 1 0 0 1 154.56 244.08 Tm <2C3B3B727320> Tj 1 0 0 1 215.76 246.72 Tm <746865722C6C68617320> Tj 1 0 0 1 259.92 248.64 Tm <6265656E20> Tj 1 0 0 1 284.64 249.84 Tm <6C6975726520> Tj 1 0 0 1 333.36 251.04 Tm Tj 1 0 0 1 389.52 253.68 Tm <7765746E65737320> Tj 1 0 0 1 428.16 255.36 Tm <6D6574686F643A20> Tj 1 0 0 1 468.48 257.04 Tm <4120> Tj 1 0 0 1 480.24 257.52 Tm <73657269657320> Tj 1 0 0 1 509.04 258.96 Tm <6F7220> Tj 1 0 0 1 523.68 259.44 Tm <3330766F20> Tj 1 0 0 1 547.20 260.40 Tm <6D6574616C> Tj 0.48 Tc /F3 11.0 Tf 1 0 0 1 69.36 227.76 Tm <726573656172636820> Tj 1 0 0 1 109.44 229.44 Tm <6F6E20> Tj 1 0 0 1 123.12 230.16 Tm <6E657720> Tj 1 0 0 1 144.48 230.88 Tm <6D6174657269616C7320> Tj 1 0 0 1 188.40 232.80 Tm <696F20> Tj 1 0 0 1 199.92 233.28 Tm <626520> Tj 1 0 0 1 213.36 233.76 Tm <656D70726F79656420> Tj 1 0 0 1 259.92 235.92 Tm <696E20> Tj 1 0 0 1 271.44 236.16 Tm <736174656C6C69746520> Tj 1 0 0 1 334.32 238.08 Tm <2E4AEF3B3B693B3B3B22FC7269722720> Tj 1 0 0 1 416.40 242.16 Tm <2A697472742E72722F527520> Tj 1 0 0 1 467.52 244.08 Tm <6D61737320> Tj 1 0 0 1 493.92 245.28 Tm <726174696F7320> Tj 1 0 0 1 522.48 246.72 Tm <6F6620> Tj 1 0 0 1 535.68 247.44 Tm <326C722720> Tj 1 0 0 1 557.52 248.40 Tm <6C6C6C> Tj 0.48 Tc 1 0 0 1 69.84 215.76 Tm <70726F70757273696F6E2E20> Tj 1 0 0 1 125.52 217.44 Tm <6F222220> Tj 1 0 0 1 149.76 210.48 Tm <227231742220> Tj 1 0 0 1 183.12 219.84 Tm <6C617465737420> Tj 1 0 0 1 212.40 221.04 Tm <646576E3726F706D656E747320> Tj 1 0 0 1 278.88 223.92 Tm <77617320> Tj 1 0 0 1 301.68 224.64 Tm <7520> Tj 1 0 0 1 335.04 225.36 Tm <756E6F27EF3B3B3B3B20> Tj 1 0 0 1 400.32 225.84 Tm <667222706F2722642C20> Tj 1 0 0 1 447.12 230.16 Tm <616C7761797320> Tj 1 0 0 1 482.64 231.84 Tm <7769746820> Tj 1 0 0 1 506.88 232.80 Tm <6972696469756D20> Tj 1 0 0 1 544.08 234.48 Tm <617320> Tj 1 0 0 1 557.52 235.20 Tm <746865> Tj 0.48 Tc 1 0 0 1 70.32 203.04 Tm <706174656E7420> Tj 1 0 0 1 101.52 203.52 Tm <7265676973726572656420> Tj 1 0 0 1 149.04 205.68 Tm <627920> Tj 1 0 0 1 164.40 206.16 Tm <5368656C6C20> Tj 1 0 0 1 191.52 205.68 Tm <5B41726D7374726F6E672D3B3B692E2C20> Tj 1 0 0 1 276.72 210.96 Tm <31393767625D20> Tj 1 0 0 1 335.28 212.64 Tm <746972727420> Tj 1 0 0 1 357.60 213.60 Tm <2A2274757220> Tj 1 0 0 1 386.40 215.04 Tm <746F20> Tj 1 0 0 1 399.12 215.52 Tm Tj 1 0 0 1 414.24 216.24 Tm Tj 1 0 0 1 463.92 218.40 Tm <54686520> Tj 1 0 0 1 485.76 219.60 Tm <707265637572736F725E736F6C7574696F6E73> Tj 0.48 Tc 1 0 0 1 70.80 189.84 Tm <6C6F7220> Tj 1 0 0 1 89.52 190.32 Tm <6120> Tj 1 0 0 1 99.60 190.80 Tm <72722D52752F416C7A6F7220> Tj 1 0 0 1 157.92 193.20 Tm <636174616C7973722C20> Tj 1 0 0 1 200.64 194.88 Tm <73757373657374726E6720> Tj 1 0 0 1 252.72 197.28 Tm <7468617420> Tj 1 0 0 1 275.04 198.24 Tm <6972696469756D20> Tj 1 0 0 1 335.76 191.76 Tm <2227E0EF3BEF20> Tj 1 0 0 1 385.44 202.32 Tm <6E277274F372742D395E2E752C747220> Tj 1 0 0 1 447.36 204.96 Tm <48636C20> Tj 1 0 0 1 470.16 205.92 Tm <616E6420> Tj 1 0 0 1 489.60 206.88 Tm <5275636C3320> Tj 1 0 0 1 520.08 208.32 Tm <302732324E20> Tj 1 0 0 1 551.04 209.52 Tm <48636C27> Tj 0.48 Tc 1 0 0 1 71.52 176.88 Tm <636F6E74656E747320> Tj 1 0 0 1 114.24 178.80 Tm <6D75737420> Tj 1 0 0 1 140.88 179.76 Tm <626520> Tj 1 0 0 1 157.20 180.48 Tm <6B65707420> Tj 1 0 0 1 182.40 181.44 Tm <617420> Tj 1 0 0 1 196.08 182.16 Tm <616E20> Tj 1 0 0 1 212.16 182.88 Tm <61746F6D726320> Tj 1 0 0 1 247.68 176.40 Tm <22E36E22226E74727574696F6E20> Tj 1 0 0 1 336.24 189.84 Tm <7072696F7220> Tj 1 0 0 1 361.44 188.16 Tm <746F20> Tj 1 0 0 1 372.96 188.64 Tm <74686520> Tj 1 0 0 1 389.52 189.60 Tm <696D707265676E6174696F6E2C20> Tj 1 0 0 1 453.84 192.24 Tm <74686520> Tj 1 0 0 1 470.64 192.96 Tm <737570706F727420> Tj 1 0 0 1 506.40 194.64 Tm <7761732C6F2E76656E20> Tj 1 0 0 1 550.08 196.56 Tm <6472696564> Tj 0.72 Tc 1 0 0 1 72.00 164.16 Tm <6265747765656E20> Tj 1 0 0 1 116.16 166.08 Tm <3330373020> Tj 1 0 0 1 148.56 167.28 Tm <616E64673037302E20> Tj 1 0 0 1 196.56 169.44 Tm <416E6F7474222E20> Tj 1 0 0 1 240.00 163.44 Tm <226F2A2A756E69636174696F6E20> Tj 1 0 0 1 336.96 174.48 Tm <742272EF69722272722E20> Tj 1 0 0 1 392.64 176.88 Tm <75725C67ED72632C75747465727768696369722D746865726573756C74696E67736F6C696473> Tj 0.48 Tc 1 0 0 1 72.72 150.96 Tm <72656C6174657320> Tj 1 0 0 1 108.72 152.64 Tm <74686520> Tj 1 0 0 1 129.36 153.36 Tm <646576656C6F706D656E7220> Tj 1 0 0 1 193.68 156.24 Tm <6F6620> Tj 1 0 0 1 206.64 150.96 Tm <2D3120> Tj 1 0 0 1 220.80 150.96 Tm <3A7574754A79727420> Tj 1 0 0 1 262.56 159.12 Tm <636F6E7461696E696E6720> Tj 1 0 0 1 337.20 161.52 Tm <747464223B3B3B20> Tj 1 0 0 1 388.80 163.68 Tm <487A20> Tj 1 0 0 1 404.88 164.64 Tm <666C6F772D647279696E6720> Tj 1 0 0 1 462.96 167.04 Tm <666F7220> Tj 1 0 0 1 480.48 168.00 Tm <3220> Tj 1 0 0 1 490.56 168.24 Tm <686F75727320> Tj 1 0 0 1 519.36 169.68 Tm <666F6C6C6F77656420> Tj 1 0 0 1 562.80 171.36 Tm <6279> Tj 0.48 Tc 1 0 0 1 73.20 138.24 Tm <72757468656E69756D20> Tj 1 0 0 1 122.88 140.16 Tm <6F6E72792C20> Tj 1 0 0 1 149.28 141.36 Tm <6361696C656420> Tj 1 0 0 1 180.00 142.56 Tm <5368652720> Tj 1 0 0 1 206.64 143.76 Tm <582D342C20> Tj 1 0 0 1 230.64 144.72 Tm <777469227420> Tj 1 0 0 1 261.60 145.92 Tm <697320> Tj 1 0 0 1 272.64 146.40 Tm <7265706F727465E120> Tj 1 0 0 1 338.16 148.32 Tm <2C224A222E6969222220> Tj 1 0 0 1 383.28 140.16 Tm <2220> Tj 1 0 0 1 396.48 150.96 Tm <3669334B726F276627E37574722720> Tj 1 0 0 1 478.56 154.80 Tm <54686520> Tj 1 0 0 1 499.20 155.52 Tm <6164646974696F6E20> Tj 1 0 0 1 538.32 157.44 Tm <6F6620> Tj 1 0 0 1 550.08 157.92 Tm <6D6574616C> Tj 0.48 Tc 1 0 0 1 73.68 125.04 Tm <746F20> Tj 1 0 0 1 88.56 125.76 Tm <6861766520> Tj 1 0 0 1 115.92 126.96 Tm <6265656E20> Tj 1 0 0 1 143.04 128.16 Tm <7573656420> Tj 1 0 0 1 170.40 129.36 Tm <7769746820> Tj 1 0 0 1 196.80 130.56 Tm <677265617420> Tj 1 0 0 1 225.36 131.52 Tm <2C752E2222722C20> Tj 1 0 0 1 264.72 133.20 Tm <2A20> Tj 1 0 0 1 279.60 133.68 Tm Tj 1 0 0 1 302.16 134.64 Tm <4E20> Tj 1 0 0 1 338.88 135.60 Tm <696E20> Tj 1 0 0 1 352.08 136.32 Tm <6561636820> Tj 1 0 0 1 377.28 137.28 Tm <6F6620> Tj 1 0 0 1 390.72 137.76 Tm <74686520> Tj 1 0 0 1 408.96 138.72 Tm <696D707265676E6174696F6E20> Tj 1 0 0 1 473.04 141.36 Tm <737465707320> Tj 1 0 0 1 499.68 142.80 Tm <77617320> Tj 1 0 0 1 521.28 143.52 Tm <616C7761797320> Tj 1 0 0 1 555.84 144.96 Tm <6B657074> Tj 0.24 Tc /F3 15.0 Tf 1 0 0 1 73.68 112.32 Tm Tj 1 0 0 1 115.92 112.32 Tm <72EFEF3BEF3BEC2A692C22312A2220> Tj 1 0 0 1 226.80 98.88 Tm <3A3A5470752E2220> Tj 1 0 0 1 270.72 107.76 Tm <72686520> Tj 1 0 0 1 289.44 108.72 Tm <6D61696E20> Tj 1 0 0 1 339.12 109.92 Tm <69EF3FEF27312D2721EF3BEF31EF3A20> Tj 1 0 0 1 427.68 114.00 Tm <6D6574686F643A20> Tj 1 0 0 1 466.80 115.68 Tm <72686520> Tj 1 0 0 1 488.16 116.40 Tm <73616D6520> Tj 1 0 0 1 513.36 117.84 Tm <70726F647563747320> Tj 1 0 0 1 554.88 119.52 Tm <77657265> Tj 0.48 Tc /F3 10.0 Tf 1 0 0 1 75.60 86.88 Tm <7265737572747320> Tj 1 0 0 1 108.24 88.08 Tm <6F6620> Tj 1 0 0 1 120.96 88.56 Tm <616E20> Tj 1 0 0 1 134.64 89.28 Tm <6576616C756174696F6E20> Tj 1 0 0 1 184.56 91.20 Tm <6F6620> Tj 1 0 0 1 197.04 91.92 Tm <6C722D52752F41727A6F7220> Tj 1 0 0 1 253.44 94.08 Tm <636174616C7973747320> Tj 1 0 0 1 295.20 96.00 Tm <696E20> Tj 1 0 0 1 307.44 96.48 Tm <6120> Tj 1 0 0 1 340.56 96.96 Tm <6F66E32A222E2C20> Tj 1 0 0 1 384.24 98.88 Tm <757327696E6720> Tj 1 0 0 1 411.84 100.08 Tm <74686520> Tj 1 0 0 1 429.60 100.80 Tm <73616D6520> Tj 1 0 0 1 455.76 102.00 Tm <6D6574686F646F6C6F677920> Tj 1 0 0 1 517.92 104.88 Tm <616E6420> Tj 1 0 0 1 537.12 105.84 Tm <74686520> Tj 1 0 0 1 554.64 106.32 Tm <73616D65> Tj 0.48 Tc /F3 7.0 Tf 1 0 0 1 256.56 70.08 Tm <4272617A2E696CED61747420> Tj 1 0 0 1 288.72 71.52 Tm <4A6F75726E756C20> Tj 1 0 0 1 316.56 72.72 Tm <6F2E6620> Tj 1 0 0 1 325.20 73.20 Tm <4368656D6963616C20> Tj 1 0 0 1 358.08 74.64 Tm <456E67EC6E65656E727467> Tj ET endstream endobj 15 0 obj 28429 endobj 16 0 obj << /Length 17 0 R >> stream 214 TG Soares Neto' J Gobbo-Ferreira' AJ GCobo and G M Cruzthe She' 405 (3OVorrlAlzor) catalysr by the she' 2 Nthruster with the results obtained with 307olrlAlzo:company represenre; a iundumeniut t".no-t;r*i 91t"t;;;i' *.11" S#:y'.tJL:'ftKlbtiiffir,";lii'""i'"",,,;i,l;H "',ril:. tql i:JJl^'i::"'b:u";;;'i;;o ,hose ob'faineddecompose low-temper?tu1:, (U:^^-? liquid "'ing " Shell405 commercial catayst'hydrazine in a very reprodlciblt Tunl-"tiArmstrong;i;., ida, t9zb, qsol' Thanks to this process' E*PERTMENTALhvdrazine monopropellant systems be came veryi-i'"o'r.,i' 'Jt"ule' Presentlv' the Shell 405ABSG catalyst ",r.Jr^ rrondreds of. .iJ-'rr"nt CatalystsPreparation??i*tl* r.rru':':li::i3:*fii: in."ii":"i,J*.:"i'-ii' *t'hot pulses r:l: rl ".J continuous shots of several p*p"J"t INPE to -11u" micro and macropores lnhours, when rhe caralysr bed reaches ,"Trffi; i: ^11"^r*"r product' a process of controlled generationhigh as 1373 K, on *tn a rime deravs of ress than 10 ;"L"J;,J.t#11". ri:iJ,"t#i"$ms"Sheu 405 has an elevated metal conrenr of about 1p1ryi:1,:::i"1lt the following characte307o, which prevents hydrazine rr"*"p""",;;*q l)Totalspecific atea:z2rrlg; deep in tt " "ututy*i' gruin, thereby prouiJin- goo zl p"t" ulo*" (humid point): 0'71 cm'/g:heat dissipu,,on u0"il"* "*t '" " i ctuin diameter: 0'6 to 0'8 mm;minimum rridium i.- o"poit"q d:*:i ^t il;"riHi,:"lii"J;*:r*.:iL": H;'il: ";;;;: *'ch hs interrinked micro and ",;:::":i','"".i;J.:'t,,i;;;'';r:loso1 ro obruin u,n"ropor", [Schmidt' 1984]' ' of incipient rvetness fCruzother countries contributed to the research on -.,"jonttnt of 30L' three irnpregnatiot] steps \\erehydrazinedecomposit"-uJyrtt""nnology rh]r_,_: n"..,;r'.-H,r.g!."f]d sorntion urrh a free acidthe case, for instance,-in r.un.., wh9r3 cfrsno'r .on..,i,ion-of 0 6 \ *as used as the precursor ofwas developed rnr"*r.'1;, valentine. 1g1i.. ,t. ".liir. rnetal phase. This producr as eitherSchmidt, 1gg4] and Germanl. *here.a cararr sr caired prepared in the laboraror) a'. r\pE or purchased fromKC 12 G was produced b-r raiicfrllil iHonung. ir-'" -Ens.ir"ra corporarion, France Prior io1974; Harrung et al.. , ;rr*rdt, 19g;rl. impregntion' the support was oven dried at 393KThe use or .ottr"nium, which is far cheaper than f:l ;th;;tt" t"t "un itnp'"gnation solids wereiridium, is a very promising alrernativq'*ii"v r", ari" ir *"uum for t hour nd reduced in Hz flow'#.;l'"rbJ*i:r'**J,""',, -,Xllii"; "';i"iJ'^1,".;"'r,,, containing 30%,5tar wasand apogee satettite m-oirr-is"rr*idt, 19841, where p'";;;; uy itre.abovl 'methodoogy' usin-g-as thetoral burning rime reaches a maximum of 5 minutes' n'J;;;' 'u'ion -ol -Rucl: with a free HCl acidIn this case a ,utettit" launching usesabout 800 g of t"""""ti"n of 0'2?.N' purchased from thecatalyst. According ro rhe.Engelt "g g^"rn";:* ett"fit^tJ "rporation,fSou'"i N"to et a'' 1999]'cost of the iridium metal precursor rs round US$ *"^rt"*nt methods were employed in the27.OOlgram, whie ruthenium cosrs about us$ o*n*i19" "lt'-n"lerzor catalysts fsoares Neto et,.gi the rast ,;;rs ther,lhas been liure 'ii3ijtl", wetness method: A series or 30vo metalresearch on new materials io be emproyed in satellite .J;;i;;;"rir' *itrt.rr/Ru mass ratios of 2lr' lllpropursion. o"" "r1t" latest devropments was u uno';;;; fr"po'"d, always with iridium as thepatent regisrered by Shell [Armstrong-;;i., 197gb] tirrt *"tur to e epo-sited. The precursor^solutionslor a rr-Ru/Alzor catalysr, sussestrng that iridium "'; n'rtrt-9^.u,tr Hcl and Rucl3 0'22N Hcl'contents must be kept at an atomrc "n""ntrution prior to the impregnation, the support was,o.ven driedbetween 3070 andg070. Anott". "o**unication t"rir"rr. ur\grc,utterwhicir-theresultingsolidsrelates the developmenr of -1 :utuJyrt containing ttd";;; Hz flow-drying for 2 hours followed byruthenium onry, cailed She' X-4, wti"t is reporte ,"J".ii"" " 6i3Kro'f'utr' The addition of metalto have been used with great ,u.""r, * :o N in each of the impregnation steps was always keptJ,:' r;;*i,"1*" ::Tpu." rhe main i?'1-'!;1: method: rhe same products wereresurts of an evaluation of lr-Ru/Arzor catalysts in a of*"., us'ing the same methodology and the same Braz.ilatt Journul o.f Chemical Engneenrtg endstream endobj 17 0 obj 4402 endobj 18 0 obj << /Length 27 >> stream % CANON_PFINF_TYPE0_TEXTON endstream endobj 19 0 obj << /Length 45 >> stream q 595.20 0 0 841.68 0.00 0.00 cm /Obj13 Do Q endstream endobj 20 0 obj << /Type /Page /MediaBox [ 0 0 595.20 841.68 ] /Parent 11 0 R /Resources << /Font << /F3 5 0 R >> /XObject << /Obj13 13 0 R >> /Subtype 16 0 R /ProcSet [ /PDF /Text /ImageB /ImageC /ImageI ] >> /Contents [ 18 0 R 19 0 R 14 0 R ] >> endobj 21 0 obj << /Type /XObject /Subtype /Image /Width 2480 /Height 3507 /BitsPerComponent 1 /ColorSpace /DeviceGray /Filter /CCITTFaxDecode /DecodeParms << /K -1 /Columns 2480 >> /Length 63426 >> stream &GDp<q;7A-`aaGbU Qo娜XhDM]S*/D&Etk6}AzWd p(GդDYoÇ8>mRz_h6~ںZDza/3c /}w6 zK$h}a/A"ϑYQ ꛤz`G(Pͳ&GGߙ:% ֕k_Ӥ' <8;0@b8Ffa";f=ʟzm\;.ݫH&X${TaT3gSB30}wGw?:_J< 8;p>0B熵>Tu>_B mvyG*n_|{G?=ZUWV𗄾Շ+ͧT[KL7`Pm?ooۥ6 @ݯV!Aޯ4UpG5[m ._Oy_((Ria Q vխ:V}7H1!2q ^Z _߮_q !*I4ӶҴBe}~7+tE" aɸI;av%JoR*HDDDDl&0M8L$m-bӴnDDDDDD1Q 6)6)U%xa]h֒da1Èbw;X#gy~2emdbGFXu(F΄|#R7z', Fvc܏g C33]}"PAappS HyzU#A; 0d$NN Al#[g 2qOƌ7~Z] bSpo [y#MV8w"UީA#m͛5ֺN2Tdu''&;&7 D&B EY՚/YAV[}+ҘP@#""N]oX?<%[]ѱa!ۄ DBd٧Jվ}8tA\26 °E[]7#v ] L" 0Eh"o0Utt䱆%[F'@!H#_]2~v^4BdA=9 a,6v2:/]Ste'J` `C~4kG$y!~6|: q_Q*AenvAAAB`(3Af4_[u]_G,9_tA6%MM(0T-A383H43i6uhuOu~v i:h &64l A]]-0׿޾b$߆M֬Vt&wx?4m<4)l'uu_K>KۮqIJ**iw8KoJXo%z_{~pl aPAH0MV6"""'Fzv"ɲ2cO;B(?ge"> J aL"c̄YJ~; NLJޱ:NWKr(͌3) ˜`lԐ5i0PT'LGu#$FmRcA6BlpC4"IYuŜdZw;I80E1+,lh&7CG\ #80#8=GDtGDJ@K[n:od$>6h ࠡ0 2ΤtE]W Vp3Gi>Oi~NtkCp|2t8PFp  9$~';}ZbU6PPD&LDa;gtKKߦWa:ZM(T:SL $!3IQtw;vUГ0Ÿ~m&ÆT5PF13$#;#B>G2GEZpG@/^_Iz m& A4p&6<)3ƿT68IOZt !+4 vNvF3(6|ieU(~=['݊tIv[ 4hu aaO+n-300P@@3DoOLTy y oO:m[h U C q)0GB n9ү| ] {#֐1*Ĭ 6AUL"!FA4!rd1JC5iOZ^C^_of?݇&di8czؕ 2b RF2q 2)Q&]ڶ~]vm7_ðZIMDtF|@BA(G sOZӶa_H7i0ڽm/鄓'I:ovA'Z,p„!vf3D OO XkoV~! 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Tj 1 0 0 1 157.68 411.84 Tm <76616375756D20> Tj 1 0 0 1 197.04 411.36 Tm <6368616D62657220> Tj 1 0 0 1 240.72 410.88 Tm <73696D756C6174696E67> Tj 0.96 Tc 1 0 0 1 54.48 399.84 Tm <737061636520> Tj 1 0 0 1 82.80 400.08 Tm <707265737375726520> Tj 1 0 0 1 125.52 399.36 Tm <636F6E646974696F6E7320> Tj 1 0 0 1 178.56 399.36 Tm <2846696775726520> Tj 1 0 0 1 217.44 398.40 Tm <31292E20> Tj 1 0 0 1 232.08 398.40 Tm <6163636F7264696E6720> Tj 1 0 0 1 281.28 397.68 Tm <746F> Tj 0.48 Tc /F3 7.0 Tf 1 0 0 1 235.44 813.84 Tm <6C722D52752F416C3A4F7220> Tj 1 0 0 1 275.28 813.36 Tm <436174616C7973747320> Tj 1 0 0 1 306.96 812.88 Tm <5573656420> Tj 1 0 0 1 325.20 812.88 Tm <696E20> Tj 1 0 0 1 333.84 812.64 Tm <536174656C6C69746520> Tj 1 0 0 1 362.16 814.56 Tm <70726F70756C73696F6E> Tj 0.72 Tc /F3 8.0 Tf 1 0 0 1 546.72 810.96 Tm <323735> Tj 0.48 Tc /F3 10.0 Tf 1 0 0 1 322.32 791.76 Tm <746F20> Tj 1 0 0 1 333.84 791.52 Tm <74686520> Tj 1 0 0 1 350.16 791.52 Tm <666F6C6C6F77696E6720> Tj 1 0 0 1 396.00 791.28 Tm <70726F636564757265733A> Tj 0.48 Tc 1 0 0 1 322.32 778.80 Tm <612920> Tj 1 0 0 1 333.84 778.80 Tm <53616D706C6520> Tj 1 0 0 1 369.60 778.32 Tm <647279696E6720> Tj 1 0 0 1 401.28 778.08 Tm <6F6620> Tj 1 0 0 1 413.28 778.08 Tm <74686520> Tj 1 0 0 1 429.84 777.84 Tm <636174616C79737420> Tj 1 0 0 1 466.80 777.60 Tm <666F7220> Tj 1 0 0 1 482.64 777.36 Tm <61626F757420> Tj 1 0 0 1 511.20 777.36 Tm <6C3220> Tj 1 0 0 1 523.44 777.12 Tm <686F75727320> Tj 1 0 0 1 550.80 776.88 Tm <6174> Tj 0.96 Tc 1 0 0 1 322.32 766.32 Tm <33393320> Tj 1 0 0 1 341.76 766.08 Tm <4B3B> Tj 0.48 Tc 1 0 0 1 322.08 753.60 Tm <622920> Tj 1 0 0 1 335.28 753.60 Tm <42656420> Tj 1 0 0 1 357.12 753.60 Tm <7061636B696E6720> Tj 1 0 0 1 396.48 752.88 Tm <6F6620> Tj 1 0 0 1 409.92 752.88 Tm <74686520> Tj 1 0 0 1 427.44 752.88 Tm <636174616C79737420> Tj 1 0 0 1 465.84 752.40 Tm <7468726F75676820> Tj 1 0 0 1 504.00 751.92 Tm <74686520> Tj 1 0 0 1 521.52 751.92 Tm <75736520> Tj 1 0 0 1 540.48 751.68 Tm <6F6620> Tj 1 0 0 1 553.68 751.44 Tm <61> Tj 0.48 Tc 1 0 0 1 322.08 740.88 Tm <7368616B696E6720> Tj 1 0 0 1 360.72 740.64 Tm <64657669636520> Tj 1 0 0 1 394.32 740.40 Tm <746F20> Tj 1 0 0 1 407.76 740.40 Tm <72656475636520> Tj 1 0 0 1 442.32 739.92 Tm <766F69647320> Tj 1 0 0 1 470.88 739.68 Tm <696E20> Tj 1 0 0 1 484.08 739.44 Tm <74686520> Tj 1 0 0 1 502.08 739.20 Tm <6265642C20> Tj 1 0 0 1 525.36 739.20 Tm <74686572656279> Tj 0.48 Tc 1 0 0 1 321.60 728.40 Tm <70726576656E74696E6720> Tj 1 0 0 1 372.00 727.92 Tm <677261696E20> Tj 1 0 0 1 397.68 727.44 Tm <766962726174696F6E20> Tj 1 0 0 1 440.64 726.96 Tm <647572696E6720> Tj 1 0 0 1 472.56 726.72 Tm <74686520> Tj 1 0 0 1 488.88 726.72 Tm <666972696E67733B> Tj 0.48 Tc 1 0 0 1 321.60 715.20 Tm <632920> Tj 1 0 0 1 334.08 715.20 Tm <417373656D626C696E6720> Tj 1 0 0 1 390.72 714.72 Tm <6F6620> Tj 1 0 0 1 403.44 714.72 Tm <74686520> Tj 1 0 0 1 420.96 714.48 Tm <746872757374657220> Tj 1 0 0 1 458.88 714.00 Tm <636174616C79737420> Tj 1 0 0 1 496.56 713.76 Tm <6265642C20> Tj 1 0 0 1 517.68 713.52 Tm <7573696E6720> Tj 1 0 0 1 545.28 715.92 Tm <70742D> Tj 0.72 Tc 1 0 0 1 321.60 702.48 Tm <526820> Tj 1 0 0 1 337.68 702.24 Tm <73637265656E7320> Tj 1 0 0 1 373.44 702.00 Tm <746F20> Tj 1 0 0 1 385.20 702.00 Tm <61737375726520> Tj 1 0 0 1 416.16 701.76 Tm <69747320> Tj 1 0 0 1 429.84 701.76 Tm <696E7465677269747920> Tj 1 0 0 1 470.64 701.28 Tm <616E6420> Tj 1 0 0 1 489.60 701.04 Tm <746F20> Tj 1 0 0 1 501.36 700.80 Tm <61766F696420> Tj 1 0 0 1 528.72 700.80 Tm <6C6F737320> Tj 1 0 0 1 548.88 700.56 Tm <6F66> Tj 0.72 Tc 1 0 0 1 321.36 689.76 Tm <636174616C7973743B> Tj 0.48 Tc 1 0 0 1 321.36 677.04 Tm <642920> Tj 1 0 0 1 333.36 676.80 Tm <417474616368696E6720> Tj 1 0 0 1 380.16 676.56 Tm <6F6620> Tj 1 0 0 1 391.92 676.32 Tm <74686520> Tj 1 0 0 1 408.48 676.32 Tm <6E6F7A7A6C6520> Tj 1 0 0 1 440.40 676.08 Tm <726F20> Tj 1 0 0 1 451.68 675.84 Tm <74686520> Tj 1 0 0 1 468.48 675.60 Tm <7365723A> Tj 0.48 Tc 1 0 0 1 321.36 664.32 Tm <642920> Tj 1 0 0 1 333.36 664.32 Tm <496E7374616C6C6174696F6E20> Tj 1 0 0 1 386.40 663.84 Tm <6F6620> Tj 1 0 0 1 398.16 663.60 Tm <74686520> Tj 1 0 0 1 414.72 663.60 Tm <746872757374657220> Tj 1 0 0 1 451.92 663.36 Tm <696E20> Tj 1 0 0 1 463.44 663.12 Tm <74686520> Tj 1 0 0 1 480.00 663.12 Tm <76616375756D20> Tj 1 0 0 1 516.96 662.64 Tm <6368616D6265722C> Tj 0.48 Tc 1 0 0 1 321.36 651.60 Tm <627920> Tj 1 0 0 1 344.64 651.60 Tm <6C696E6B696E6720> Tj 1 0 0 1 388.56 651.12 Tm <697420> Tj 1 0 0 1 406.56 651.12 Tm <746F20> Tj 1 0 0 1 427.44 650.88 Tm <74686520> Tj 1 0 0 1 453.60 650.64 Tm <6D6561737572656D656E7420> Tj 1 0 0 1 524.40 649.92 Tm <64657669636573> Tj 0.48 Tc 1 0 0 1 321.36 639.60 Tm <2874656D70657261747572652C20> Tj 1 0 0 1 383.28 638.88 Tm <70726573737572652C20> Tj 1 0 0 1 426.24 638.16 Tm <666C6F7720> Tj 1 0 0 1 449.52 637.92 Tm <726174652C20> Tj 1 0 0 1 472.08 637.68 Tm <616E6420> Tj 1 0 0 1 490.80 637.68 Tm <746872757374293B> Tj 0.72 Tc 1 0 0 1 320.88 626.64 Tm <652920> Tj 1 0 0 1 333.84 626.40 Tm <45737461626C6973686D656E7420> Tj 1 0 0 1 401.04 625.92 Tm <6F6620> Tj 1 0 0 1 414.24 625.92 Tm <74686520> Tj 1 0 0 1 432.48 625.68 Tm <76616375756D20> Tj 1 0 0 1 471.60 625.20 Tm <696E7369646520> Tj 1 0 0 1 502.08 624.96 Tm <74686520> Tj 1 0 0 1 519.36 624.96 Tm <6368616D626572> Tj 0.72 Tc 1 0 0 1 321.12 613.68 Tm <616E6420> Tj 1 0 0 1 340.32 613.44 Tm <68656174696E6720> Tj 1 0 0 1 376.32 613.20 Tm <6F6620> Tj 1 0 0 1 388.80 612.96 Tm <74686520> Tj 1 0 0 1 405.60 612.96 Tm <636174616C79737420> Tj 1 0 0 1 443.04 612.48 Tm <62656420> Tj 1 0 0 1 462.24 612.48 Tm <757020> Tj 1 0 0 1 476.64 612.24 Tm <746F20> Tj 1 0 0 1 488.64 612.24 Tm <33393320> Tj 1 0 0 1 508.08 612.00 Tm <4B2E20> Tj 1 0 0 1 521.52 612.00 Tm <57616974696E67> Tj 0.48 Tc 1 0 0 1 320.88 600.96 Tm <666F7220> Tj 1 0 0 1 336.72 600.96 Tm <3220> Tj 1 0 0 1 345.12 600.72 Tm <686F75727320> Tj 1 0 0 1 372.48 600.48 Tm <6265666F726520> Tj 1 0 0 1 403.68 600.24 Tm <666972737420> Tj 1 0 0 1 424.56 600.24 Tm <666972696E6720> Tj 1 0 0 1 452.40 599.76 Tm <746F20> Tj 1 0 0 1 463.68 599.76 Tm <72656D6F766520> Tj 1 0 0 1 499.68 599.52 Tm <68756D69646974793B> Tj 0.72 Tc 1 0 0 1 320.88 588.24 Tm <667420> Tj 1 0 0 1 332.88 588.00 Tm <5374617274696E5F6520> Tj 1 0 0 1 372.48 587.76 Tm <6F6620> Tj 1 0 0 1 386.16 587.52 Tm <74686520> Tj 1 0 0 1 404.16 587.52 Tm <666972696E6720> Tj 1 0 0 1 433.44 587.04 Tm <627920> Tj 1 0 0 1 449.04 586.80 Tm <6F70656E696E6720> Tj 1 0 0 1 489.12 586.56 Tm <74686520> Tj 1 0 0 1 507.12 586.56 Tm <6665656420> Tj 1 0 0 1 530.64 586.32 Tm <76616C76652C> Tj 0.72 Tc 1 0 0 1 320.88 575.76 Tm <7520> Tj 1 0 0 1 328.80 575.28 Tm <6872636820> Tj 1 0 0 1 350.88 575.04 Tm <696E74726F647563657320> Tj 1 0 0 1 399.84 574.56 Tm <68796472617A696E6520> Tj 1 0 0 1 446.64 574.08 Tm <696E746F20> Tj 1 0 0 1 466.56 573.84 Tm <74686520> Tj 1 0 0 1 482.88 573.84 Tm <6265643B20> Tj 1 0 0 1 504.96 573.60 Tm <616E643B> Tj 0.96 Tc 1 0 0 1 321.12 564.24 Tm <7120> Tj 1 0 0 1 327.84 563.52 Tm <7220> Tj 1 0 0 1 332.88 562.80 Tm <5CCD6F6E69746F72696E6720> Tj 1 0 0 1 393.84 562.08 Tm <69736E6974696F6E20> Tj 1 0 0 1 438.96 561.60 Tm <64656C61792E20> Tj 1 0 0 1 476.16 561.36 Tm <6368616E67657320> Tj 1 0 0 1 522.24 560.88 Tm <696E20> Tj 1 0 0 1 540.96 560.64 Tm <626564> Tj 0.96 Tc 1 0 0 1 320.64 550.08 Tm <697227CC6C5D70637261744CCC726520> Tj 1 0 0 1 376.56 550.08 Tm <7263727465726E616C6C7220> Tj 1 0 0 1 426.00 548.88 Tm <292E20> Tj 1 0 0 1 434.64 549.12 Tm <6665656420> Tj 1 0 0 1 456.96 548.88 Tm <6C696E6520> Tj 1 0 0 1 476.40 548.64 Tm <616E6420> Tj 1 0 0 1 495.12 548.40 Tm <646563636D706F736974696F6E> Tj 0.96 Tc 1 0 0 1 320.40 537.36 Tm <6368616E7262657220> Tj 1 0 0 1 361.44 537.36 Tm <70726520> Tj 1 0 0 1 375.84 536.88 Tm <5C5C4C6C72655C2E20> Tj 1 0 0 1 408.48 536.88 Tm <725DEC61737320> Tj 1 0 0 1 433.68 536.40 Tm <746C6F726920> Tj 1 0 0 1 456.72 536.16 Tm <726174652E20> Tj 1 0 0 1 479.04 535.92 Tm <616E6420> Tj 1 0 0 1 497.76 535.68 Tm <7468727573742E> Tj 0.96 Tc 1 0 0 1 334.56 524.40 Tm <54686520> Tj 1 0 0 1 358.32 524.16 Tm <69653A747320> Tj 1 0 0 1 384.72 524.40 Tm <7565726520> Tj 1 0 0 1 412.32 524.16 Tm <706572666F726E74656420> Tj 1 0 0 1 465.36 523.20 Tm <666F6C6C6F2A696E5F6520> Tj 1 0 0 1 514.32 522.72 Tm <74686520> Tj 1 0 0 1 534.48 522.72 Tm <73616D65> Tj 0.96 Tc 1 0 0 1 320.40 511.92 Tm <73657175656E636520> Tj 1 0 0 1 363.84 511.68 Tm <666F7220> Tj 1 0 0 1 379.68 511.44 Tm <616C6C20> Tj 1 0 0 1 393.36 511.44 Tm <636174616C7220> Tj 1 0 0 1 420.48 511.20 Tm <7374733A> Tj 0.96 Tc 1 0 0 1 320.16 499.20 Tm <612920> Tj 1 0 0 1 331.44 498.96 Tm <416E20> Tj 1 0 0 1 348.00 498.96 Tm <696E697469616C20> Tj 1 0 0 1 376.80 498.48 Tm <636F6E74696E756F757320> Tj 1 0 0 1 428.64 498.24 Tm <666972696E6720> Tj 1 0 0 1 456.24 497.76 Tm <6F6620> Tj 1 0 0 1 468.48 497.76 Tm <32303020> Tj 1 0 0 1 487.92 497.52 Tm <733A> Tj 0.72 Tc 1 0 0 1 319.92 486.24 Tm <622920> Tj 1 0 0 1 333.12 486.24 Tm <546872656520> Tj 1 0 0 1 363.36 486.00 Tm <666972696E677320> Tj 1 0 0 1 396.72 485.76 Tm <6F6620> Tj 1 0 0 1 410.64 485.52 Tm <39393920> Tj 1 0 0 1 430.80 485.76 Tm <70756C7365732C20> Tj 1 0 0 1 465.84 485.04 Tm <35303020> Tj 1 0 0 1 486.72 485.04 Tm <6D7320> Tj 1 0 0 1 503.28 484.80 Tm <6561636820> Tj 1 0 0 1 528.00 484.56 Tm <7769746820> Tj 1 0 0 1 551.52 484.32 Tm <61> Tj 0.48 Tc 1 0 0 1 319.68 473.76 Tm <3430566F20> Tj 1 0 0 1 346.32 473.52 Tm <6475747920> Tj 1 0 0 1 370.08 473.28 Tm <6379636C6520> Tj 1 0 0 1 398.88 473.52 Tm <286665656420> Tj 1 0 0 1 427.20 473.04 Tm <76616C766520> Tj 1 0 0 1 456.48 472.32 Tm <6F70656E20> Tj 1 0 0 1 483.12 472.32 Tm <666F7220> Tj 1 0 0 1 501.12 472.08 Tm <32303020> Tj 1 0 0 1 522.72 471.84 Tm <6D7320> Tj 1 0 0 1 540.48 471.84 Tm <616E64> Tj 0.72 Tc 1 0 0 1 319.68 460.80 Tm <636C6F73656420> Tj 1 0 0 1 350.88 460.80 Tm <666F7220> Tj 1 0 0 1 366.96 460.56 Tm <33303020> Tj 1 0 0 1 386.16 460.32 Tm <6D73293B20> Tj 1 0 0 1 408.72 460.08 Tm <616E64> Tj 0.72 Tc 1 0 0 1 319.44 448.08 Tm <632920> Tj 1 0 0 1 330.96 447.84 Tm <4120> Tj 1 0 0 1 341.52 447.84 Tm <636F6E74696E756F757320> Tj 1 0 0 1 393.36 447.36 Tm <666972696E6720> Tj 1 0 0 1 420.96 447.12 Tm <6F6620> Tj 1 0 0 1 433.20 447.12 Tm <32303020> Tj 1 0 0 1 452.88 446.88 Tm <732E> Tj 0.48 Tc 1 0 0 1 333.60 435.12 Tm <416674657220> Tj 1 0 0 1 361.44 434.88 Tm <74686520> Tj 1 0 0 1 379.20 434.64 Tm <74657374732C20> Tj 1 0 0 1 405.84 434.64 Tm <74686520> Tj 1 0 0 1 423.84 434.40 Tm <636174616C7973747320> Tj 1 0 0 1 466.56 434.16 Tm <7765726520> Tj 1 0 0 1 492.24 433.92 Tm <72656D6F76656420> Tj 1 0 0 1 534.48 433.44 Tm <66726F6D> Tj 0.48 Tc 1 0 0 1 319.44 422.64 Tm <74686520> Tj 1 0 0 1 336.96 422.40 Tm <74687275737465722C20> Tj 1 0 0 1 378.00 422.16 Tm <647269656420> Tj 1 0 0 1 405.12 421.92 Tm <617420> Tj 1 0 0 1 418.08 421.92 Tm <33393320> Tj 1 0 0 1 438.48 421.68 Tm <4B20> Tj 1 0 0 1 450.48 421.68 Tm <666F7220> Tj 1 0 0 1 467.76 421.44 Tm <61626F757420> Tj 1 0 0 1 497.52 421.20 Tm <313220> Tj 1 0 0 1 511.44 421.20 Tm <686F75727320> Tj 1 0 0 1 540.00 420.72 Tm <616E64> Tj 0.48 Tc 1 0 0 1 319.44 410.16 Tm <7765EC6768656420> Tj 1 0 0 1 360.00 409.68 Tm <746F20> Tj 1 0 0 1 371.76 409.68 Tm <64657465726D696E6520> Tj 1 0 0 1 419.28 409.20 Tm <74686520> Tj 1 0 0 1 436.56 409.20 Tm <6C6F737320> Tj 1 0 0 1 456.96 408.96 Tm <6F6620> Tj 1 0 0 1 469.20 408.72 Tm <636174616C7973747320> Tj 1 0 0 1 510.24 408.48 Tm <647572696E6720> Tj 1 0 0 1 542.16 408.24 Tm <746865> Tj 0.72 Tc 1 0 0 1 319.20 397.44 Tm <666972696E67732E> Tj 0.96 Tc 1 0 0 1 283.44 625.20 Tm <6F66> Tj 1.20 Tc 1 0 0 1 283.44 612.48 Tm <6F66> Tj 1.44 Tc /F3 19.0 Tf 1 0 0 1 256.80 357.36 Tm <566F6375756D20> Tj 1 0 0 1 324.00 356.64 Tm <43686F6D626572> Tj 0.72 Tc /F3 10.0 Tf 1 0 0 1 272.16 140.64 Tm <54656D706572617475726573656E736F7220> Tj 1 0 0 1 359.76 139.92 Tm <507265737375726573656E736F72> Tj 0.72 Tc 1 0 0 1 188.64 114.24 Tm <46696775726520> Tj 1 0 0 1 223.68 114.00 Tm <313A20> Tj 1 0 0 1 235.20 113.76 Tm <4469616772616D20> Tj 1 0 0 1 276.72 113.28 Tm <6F6620> Tj 1 0 0 1 288.48 113.04 Tm <74686520> Tj 1 0 0 1 305.04 112.80 Tm <746872757374657220> Tj 1 0 0 1 341.76 112.56 Tm <74657374696E6720> Tj 1 0 0 1 374.40 112.32 Tm <617070617261747573> Tj 0.48 Tc /F3 7.0 Tf 1 0 0 1 138.72 92.64 Tm <4272617A696C69616E20> Tj 1 0 0 1 170.88 92.40 Tm <4A6F75726E616C20> Tj 1 0 0 1 198.96 91.92 Tm <6F6620> Tj 1 0 0 1 207.60 91.92 Tm <636C7263726E6963616C20> Tj 1 0 0 1 240.48 91.68 Tm <456E67696E656572696E672C20> Tj 1 0 0 1 285.60 91.20 Tm <766F6C2E20> Tj 1 0 0 1 300.48 90.96 Tm <32302C20> Tj 1 0 0 1 316.08 90.72 Tm <4E6F2E20> Tj 1 0 0 1 328.32 90.72 Tm <30332C20> Tj 1 0 0 1 342.00 90.72 Tm <70702E20> Tj 1 0 0 1 354.96 90.72 Tm <32373320> Tj 1 0 0 1 369.60 92.16 Tm <2D20> Tj 1 0 0 1 375.12 90.48 Tm <3238322C20> Tj 1 0 0 1 392.16 90.24 Tm <4A756C7920> Tj 1 0 0 1 408.48 91.92 Tm <2D20> Tj 1 0 0 1 413.04 90.24 Tm <53657072656EFA657220> Tj 1 0 0 1 450.72 89.76 Tm <32303033> Tj 0.72 Tc /F3 9.0 Tf 1 0 0 1 123.60 347.52 Tm <56616375756D20> Tj 1 0 0 1 155.76 347.76 Tm <70756D70> Tj ET endstream endobj 23 0 obj 19345 endobj 24 0 obj << /Length 25 0 R >> stream precursors as above, but in this case both metals// were introduced simultaneously in three consecutiveimpregnations.Catalysts Characteri zationThe following were used to characterize thecatalysts:Gravimetry - for determination of metal weight;N2 Adsorption - for determination of specific surfacearea and specific pore volume (dpo,o, < 30 nm);Hg Porosimetry - for determination of specific pore volume (dp,,,,,, ) 30 nm):Irreversible H1 adsorption - for determin.rrronspecific nuntber of actir e sites and disper:iorrrr-retal phase. and: Transmissron eectrt nii r.nrcrr.scopr r TE\ r - fordetermination oi arerlse nteral pni.le :rze ISoare:\eto. 1 99E1.Hydrazine Decomposition in a 2\ ThrusterThe decomposition of N2Ha may occur by thefollowing reactions:N2H4 (l) -+ Nz (g) + 2H2(g)3 N2H4 (l) + N219; + 4NHr (B)Tests to evaluate the performance of the thrusterwere conducted in a vacuum chamber simulatingspace pressure conditions (Figure 1). according to lr-Ru/Al:Or Catalysts Used in Satellite propulsion 275 to the following procedures:a) Sample drying of the catalyst for about l2 hours at393 K;b) Bed packing of the catalyst through the use of ashaking device to reduce voids in the bed, therebypreventing grain vibration during the firings;c) Assembling of the thruster catalyst bed, using pt-Rh screens to assure its integrity and to avoid loss ofcatalyst;d) Attaching of the nozzle ro the ser:d) Installation of the thruster in the vacuum chamber,by linking it to the measurement devices(temperature, pressure, flow rate, and thrust);e) Establishment of the vacuum inside the chamberand heating of the catalyst bed up to 393 K. Waitingfor 2 hours before first firing to remove humidity;ft Startin_e of the firing by opening the feed valve,u hrch introduces hydrazine into the bed; and;q r \onitoring isnition delay. changes in bedir'l]pcratLre rcrternallr ). feed line and deccmpositionchanrber pre \\Llre\. r]ass tlori rate. and thrust.The ie:ts uere perfornted follo*in_e the samesequence for all catalr sts:a) An initial continuous firing of 200 s:b) Three firings of 999 pulses, 500 ms each with a40Vo duty cycle (feed valve open for 200 ms andclosed for 300 ms); andc) A continuous firing of 200 s.After the tests, the catalysts were removed fromthe thruster, dried at 393 K for about 12 hours andweghed to determine the loss of catalysts during thefirings. ofof Vocuum Chomber Temperaturesensor PressuresensorFigure 1: Diagram of the thruster testing apparatusBrazilian Journal of clrcrnical Engineering, vol. 20, No. 03, pp. 273 - 282, July - Seprener 2003 Vacuum pump endstream endobj 25 0 obj 2594 endobj 26 0 obj << /Length 27 >> stream % CANON_PFINF_TYPE0_TEXTON endstream endobj 27 0 obj << /Length 45 >> stream q 595.20 0 0 841.68 0.00 0.00 cm /Obj21 Do Q endstream endobj 28 0 obj << /Type /Page /MediaBox [ 0 0 595.20 841.68 ] /Parent 11 0 R /Resources << /Font << /F3 5 0 R >> /XObject << /Obj21 21 0 R >> /Subtype 24 0 R /ProcSet [ /PDF /Text /ImageB /ImageC /ImageI ] >> /Contents [ 26 0 R 27 0 R 22 0 R ] >> endobj 29 0 obj << /Type /XObject /Subtype /Image /Width 2480 /Height 3507 /BitsPerComponent 1 /ColorSpace /DeviceGray /Filter /CCITTFaxDecode /DecodeParms << /K -1 /Columns 2480 >> /Length 81830 >> stream )aw;pÆ Վ 7npݻ÷nv7n0v7 8aۇp0ۆ7n÷ 08nÆ8a0pݻ8na7 ;p݇e;nჷ7 ۰q72X@@h `标c FDKH.; d ,a-=kA T` U#du0D;Bۤ@;nE2}FH"B, %iXA }I4޽:O=t_񾆟[ox^oqRjٱ憁=Jnb!ٚ4ΪSO]v= *o @틴A A3vlgvlkzr:AdU?t_t B C6G!ZAa߰a'8P7pTk " H>_a8b{0m'aװ_ vNK}:-ooo''(Eo m}=m{׆p+;}{~ aWoc=ݏ~oÿ/G_j_ 7I ?x_y_}ҷWWKޓU֯v_^:_Kol[{׿m[׫޶}zi.m%_ﵾ\ow`4 % %{-$l+a+I6״IՊm6m $pI4$ au~P\x 8p B p` Pb0H 4ӑa'M 2 0TÈDqU,EX=&U$b 7WGA.$H a0 DDDDDDEDDDqn8a >p[aۼ7` 8n݇-ebn[&`2@sJ2Xq6AB3z %dvà p8x&[ #Oi"_z_w}WZ:Wft#xBL2d9)76GB!fdd35#q=@Z=/!9ڕlHhfR\T 4߄h izapϚ &#T‚ b@ #L F ا*!ra4| *a aN:6 Glha cIѰ0MAS`Q lF4l .mG>4| @++)8bP+ޫI& JIŰ aVtaqۤcI;ߦպu}t.aBmy+LIm& _G^m?u>;u+CMخmuaۧJ^Gtڷ}*>6y>iHߢ0G u[^7t~_ܧ[iw_{{lV솼H]H]x~_vCZLW*6_tknZ_u׷{~iZMK~ {a{o_׵m-*~aZMLU%t^ڭuV(aZiBث%8v6WKtJd^ai{i1 r61 ksL&AMB: 1A0Pi a R!4 [bqaIBbxMh6N"!56!DR 2 ` bPAB!M FiDDDRDDDDDDe!Z:iv- aa,`G[DwujW RaJBÇ q|Ȉ(Sp qH#9̎eaGcYٌ_\ ô"X*i Am;H:Ac&D `o_\0;ȕgeFkq~d:-_߄GZ뮿%+ǯk~dR<$#kKgS!dAQJޓ}0&A  D`VwWO?NtJ'IMO{uĬ~& N]Ӡ 3Ul2&ڧKդ1(}k[}~IoKt&?Em =պo)?lA;_[c?u_c׿{MoM-׏ [/ǻW#cg,X~ WXp5k:x._o?a~놉п#__+zڷ/[ ۅi}Q,00__ޟ =/ -_+?a ߷K7a?pkmij^]z7}Oo6{iW%Iآ!kP i~ᴿF[/_]Dy6m?tq$'] _܆!uU2G[Ka&Km/߿]/_iv}?a2:دm-[Ja{m/[_m{IJ_ii}{iuq)i&wm]S".:]_bG{O?ۮa+?M}}_O_>m-~ax M(  i)چi¦Eh0a¾*pJ%:b UmJ) }ޓ]^f_v_+ iv*\DDDIn"![aL)ia6(&Ml&dpŠՆP4 &0j`i;NL0vm*EJq!""" 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<636C6561726C79> Tj 0.48 Tc 1 0 0 1 43.44 574.32 Tm <73686F7720> Tj 1 0 0 1 72.00 574.32 Tm <7468617420> Tj 1 0 0 1 94.80 574.32 Tm <72757468656E69756D20> Tj 1 0 0 1 146.64 574.32 Tm <697320> Tj 1 0 0 1 159.84 574.32 Tm <6D75636820> Tj 1 0 0 1 190.08 574.08 Tm <6C65737320> Tj 1 0 0 1 212.64 574.08 Tm <64697370657273656420> Tj 1 0 0 1 260.40 574.08 Tm <7468616E> Tj 0.72 Tc 1 0 0 1 43.44 561.84 Tm <6972696469756D2E20> Tj 1 0 0 1 84.96 561.60 Tm <4576656E20> Tj 1 0 0 1 114.72 561.60 Tm <696E20> Tj 1 0 0 1 130.08 561.60 Tm <74686520> Tj 1 0 0 1 150.72 561.60 Tm <62696D6574616C6C696320> Tj 1 0 0 1 202.08 561.60 Tm <636174616C797374732C20> Tj 1 0 0 1 250.08 561.36 Tm <617320> Tj 1 0 0 1 266.16 561.36 Tm <746865> Tj 0.72 Tc 1 0 0 1 42.96 548.88 Tm <72757468656E69756D20> Tj 1 0 0 1 102.00 548.88 Tm <636F6E74656E7420> Tj 1 0 0 1 149.04 548.88 Tm <696E637265617365732C20> Tj 1 0 0 1 206.40 548.88 Tm <74686520> Tj 1 0 0 1 233.76 548.88 Tm <64697370657273696F6E> Tj 0.72 Tc 1 0 0 1 42.96 536.40 Tm <6465637265617365732E> Tj 0.48 Tc 1 0 0 1 56.88 523.44 Tm <5461626C657320> Tj 1 0 0 1 92.16 523.44 Tm <3320> Tj 1 0 0 1 102.72 523.44 Tm <616E6420> Tj 1 0 0 1 123.60 523.44 Tm <3420> Tj 1 0 0 1 134.40 523.44 Tm <636F6E7461696E20> Tj 1 0 0 1 172.32 523.44 Tm <74686520> Tj 1 0 0 1 191.04 523.44 Tm <726573756C747320> Tj 1 0 0 1 225.60 523.20 Tm <6F627461696E656420> Tj 1 0 0 1 268.56 523.20 Tm <6279> Tj 0.48 Tc 1 0 0 1 42.96 510.96 Tm <54454D2E20> Tj 1 0 0 1 72.96 510.96 Tm <496E20> Tj 1 0 0 1 85.68 510.96 Tm <5461626C6520> Tj 1 0 0 1 115.44 510.72 Tm <3320> Tj 1 0 0 1 124.56 510.72 Tm <7468657920> Tj 1 0 0 1 148.08 510.72 Tm <73686F7720> Tj 1 0 0 1 174.96 510.72 Tm <7468617420> Tj 1 0 0 1 195.84 510.72 Tm <616C6D6F737420> Tj 1 0 0 1 228.96 510.72 Tm <3930376120> Tj 1 0 0 1 253.20 510.48 Tm <6F6620> Tj 1 0 0 1 266.40 510.48 Tm <746865> Tj 0.48 Tc 1 0 0 1 42.96 498.00 Tm <6D6F6E6F6D6574616C6C696320> Tj 1 0 0 1 107.04 498.00 Tm <6972696469756D20> Tj 1 0 0 1 143.04 497.76 Tm <636174616C79737420> Tj 1 0 0 1 180.24 498.00 Tm <7061727469636C6520> Tj 1 0 0 1 217.44 497.76 Tm <6469616D657465727320> Tj 1 0 0 1 263.76 497.52 Tm <616E64> Tj 0.72 Tc 1 0 0 1 43.20 485.04 Tm <356C566F20> Tj 1 0 0 1 66.96 485.04 Tm <6F6620> Tj 1 0 0 1 79.92 485.28 Tm <74686520> Tj 1 0 0 1 97.20 485.04 Tm <72757468656E69756D20> Tj 1 0 0 1 146.64 485.04 Tm <6F6E657320> Tj 1 0 0 1 170.88 485.04 Tm <61726520> Tj 1 0 0 1 188.16 485.04 Tm <73686F7274657220> Tj 1 0 0 1 222.48 485.04 Tm <7468616E20> Tj 1 0 0 1 245.28 485.04 Tm <342E3120> Tj 1 0 0 1 262.80 485.04 Tm <6E6D2E> Tj 0.72 Tc 1 0 0 1 42.96 472.56 Tm <54686520> Tj 1 0 0 1 67.20 472.56 Tm <726573756C747320> Tj 1 0 0 1 103.44 472.56 Tm <666F7220> Tj 1 0 0 1 123.60 472.32 Tm <62696D6574616C6C696320> Tj 1 0 0 1 175.20 472.32 Tm <636174616C7973747320> Tj 1 0 0 1 220.80 472.32 Tm <66616C6C20> Tj 1 0 0 1 242.64 472.32 Tm <6265747765656E> Tj 0.48 Tc 1 0 0 1 42.96 459.60 Tm <74686573652C20> Tj 1 0 0 1 71.52 459.84 Tm <7769746820> Tj 1 0 0 1 94.32 459.60 Tm <72757468656E69756D20> Tj 1 0 0 1 143.04 459.60 Tm <7265666C656374696E6720> Tj 1 0 0 1 188.64 459.60 Tm <74686520> Tj 1 0 0 1 205.20 459.60 Tm <7472656E6420> Tj 1 0 0 1 231.12 459.60 Tm <746F776172647320> Tj 1 0 0 1 269.28 459.36 Tm <616E> Tj 0.72 Tc 1 0 0 1 43.20 446.88 Tm <696E63726561736520> Tj 1 0 0 1 84.00 446.88 Tm <696E20> Tj 1 0 0 1 96.96 446.88 Tm <74686520> Tj 1 0 0 1 114.96 446.88 Tm <6D65616E20> Tj 1 0 0 1 143.52 446.64 Tm <73697A6520> Tj 1 0 0 1 165.12 446.64 Tm <6F6620> Tj 1 0 0 1 178.56 446.64 Tm <74686520> Tj 1 0 0 1 196.80 446.88 Tm <6D6574616C20> Tj 1 0 0 1 225.60 447.12 Tm <7061727469636C65732E20> Tj 1 0 0 1 270.72 446.64 Tm <496E> Tj 0.48 Tc 1 0 0 1 42.96 434.16 Tm <5461626C6520> Tj 1 0 0 1 72.72 434.16 Tm <3420> Tj 1 0 0 1 83.28 434.16 Tm <697420> Tj 1 0 0 1 94.08 434.16 Tm <63616E20> Tj 1 0 0 1 114.24 433.92 Tm <626520> Tj 1 0 0 1 129.84 433.92 Tm <7365656E20> Tj 1 0 0 1 154.32 433.92 Tm <7468617420> Tj 1 0 0 1 175.68 433.92 Tm <74686520> Tj 1 0 0 1 194.16 433.92 Tm <6D65616E20> Tj 1 0 0 1 222.48 433.92 Tm <6469616D657465727320> Tj 1 0 0 1 270.48 433.92 Tm <6F66> Tj 0.48 Tc 1 0 0 1 42.96 421.44 Tm <72757468656E69756D20> Tj 1 0 0 1 91.68 421.68 Tm <7061727469636C657320> Tj 1 0 0 1 133.20 421.20 Tm <61726520> Tj 1 0 0 1 150.24 421.20 Tm <61626F757420> Tj 1 0 0 1 178.56 421.20 Tm <3630566F20> Tj 1 0 0 1 202.08 421.44 Tm <68696768657220> Tj 1 0 0 1 233.52 421.44 Tm <7468616E20> Tj 1 0 0 1 256.08 421.20 Tm <74686F7365> Tj 0.48 Tc 1 0 0 1 42.96 408.72 Tm <6F6620> Tj 1 0 0 1 58.56 408.72 Tm <6972696469756D20> Tj 1 0 0 1 97.44 408.96 Tm <7061727469636C657320> Tj 1 0 0 1 141.84 408.72 Tm <6E6F20> Tj 1 0 0 1 159.36 408.72 Tm <6D617474657220> Tj 1 0 0 1 194.16 408.72 Tm <776869636820> Tj 1 0 0 1 227.52 408.72 Tm <6F6620> Tj 1 0 0 1 242.88 408.48 Tm <74686520> Tj 1 0 0 1 262.80 408.48 Tm <74776F> Tj 0.72 Tc 1 0 0 1 42.96 396.00 Tm <6571756174696F6E7320> Tj 1 0 0 1 88.56 396.00 Tm <73686F776E20> Tj 1 0 0 1 120.24 396.00 Tm <697320> Tj 1 0 0 1 130.56 396.00 Tm <73656C656374656420> Tj 1 0 0 1 169.20 396.00 Tm <666F7220> Tj 1 0 0 1 185.04 396.00 Tm <746865697220> Tj 1 0 0 1 208.32 396.00 Tm <63616C63756C6174696F6E2E> Tj 0.72 Tc 1 0 0 1 56.88 383.28 Tm <546865736520> Tj 1 0 0 1 90.48 383.28 Tm <726573756C747320> Tj 1 0 0 1 126.72 383.28 Tm <616C736F20> Tj 1 0 0 1 151.92 383.04 Tm <73686F7720> Tj 1 0 0 1 181.92 383.04 Tm <7468617420> Tj 1 0 0 1 205.44 383.04 Tm <74686520> Tj 1 0 0 1 225.84 383.04 Tm <646563726561736520> Tj 1 0 0 1 271.44 383.28 Tm <696E> Tj 0.72 Tc 1 0 0 1 43.20 370.56 Tm <737065636966696320> Tj 1 0 0 1 83.04 370.56 Tm <766F6C756D6520> Tj 1 0 0 1 121.44 370.32 Tm <6F6620> Tj 1 0 0 1 136.08 370.32 Tm <74686520> Tj 1 0 0 1 155.28 370.56 Tm <706F72657320> Tj 1 0 0 1 184.80 370.56 Tm <77617320> Tj 1 0 0 1 207.36 370.56 Tm <6E65676C696769626C652E20> Tj 1 0 0 1 259.68 370.32 Tm <54686973> Tj 0.48 Tc 1 0 0 1 43.20 357.60 Tm <6173737572657320> Tj 1 0 0 1 79.20 357.60 Tm <7468617420> Tj 1 0 0 1 100.08 357.60 Tm <74686520> Tj 1 0 0 1 118.08 357.60 Tm <696E74726F64756374696F6E20> Tj 1 0 0 1 177.12 357.36 Tm <6F6620> Tj 1 0 0 1 190.80 357.36 Tm <3330376120> Tj 1 0 0 1 215.28 357.60 Tm <6D6574616C20> Tj 1 0 0 1 244.08 357.60 Tm <77696C6C20> Tj 1 0 0 1 265.20 357.36 Tm <6E6F74> Tj 0.48 Tc 1 0 0 1 43.20 345.12 Tm <696D7061697220> Tj 1 0 0 1 76.56 345.12 Tm <74686520> Tj 1 0 0 1 95.28 345.12 Tm <646966667573696F6E20> Tj 1 0 0 1 140.88 345.12 Tm <6F6620> Tj 1 0 0 1 155.04 345.36 Tm <676173657320> Tj 1 0 0 1 183.60 344.88 Tm <647572696E6720> Tj 1 0 0 1 217.68 344.88 Tm <74686520> Tj 1 0 0 1 236.16 345.12 Tm <68796472617A696E65> Tj 0.72 Tc 1 0 0 1 42.96 332.16 Tm <6465636F6D706F736974696F6E20> Tj 1 0 0 1 115.92 332.16 Tm <7265616374696F6E2E20> Tj 1 0 0 1 162.48 332.16 Tm <4465737069746520> Tj 1 0 0 1 204.48 332.16 Tm <69747320> Tj 1 0 0 1 222.48 332.16 Tm <696E74726F64756374696F6E2C> Tj 0.72 Tc 1 0 0 1 43.20 319.68 Tm <776869636820> Tj 1 0 0 1 74.40 319.68 Tm <7265647563657320> Tj 1 0 0 1 113.04 319.44 Tm <74686520> Tj 1 0 0 1 131.52 319.44 Tm <617661696C61626C6520> Tj 1 0 0 1 176.64 319.44 Tm <737065636966696320> Tj 1 0 0 1 216.00 319.44 Tm <7375726661636520> Tj 1 0 0 1 252.48 319.44 Tm <6F6620> Tj 1 0 0 1 265.92 319.44 Tm <746865> Tj 0.72 Tc 1 0 0 1 43.20 306.96 Tm <616C756D696E612C20> Tj 1 0 0 1 84.00 306.96 Tm <74686520> Tj 1 0 0 1 100.56 306.96 Tm <6D6574616C20> Tj 1 0 0 1 128.16 306.96 Tm <697320> Tj 1 0 0 1 138.48 306.96 Tm <7374696C6C20> Tj 1 0 0 1 158.16 306.96 Tm <7665727920> Tj 1 0 0 1 180.24 306.96 Tm <77656C6C20> Tj 1 0 0 1 202.32 306.72 Tm <646973747269627574656420> Tj 1 0 0 1 254.40 306.72 Tm <696E20> Tj 1 0 0 1 265.68 306.72 Tm <746865> Tj 0.48 Tc /F3 7.0 Tf 1 0 0 1 200.40 811.92 Tm <542E472E536F6172657320> Tj 1 0 0 1 238.32 811.92 Tm <4E65746F2E20> Tj 1 0 0 1 257.76 811.68 Tm <4A2E476F62626F2D46657272656972612E20> Tj 1 0 0 1 316.80 811.68 Tm <412E4A2E472E436F626F20> Tj 1 0 0 1 356.88 811.68 Tm <616E6420> Tj 1 0 0 1 370.80 811.68 Tm <472E4D2E4372757A> Tj 0.48 Tc /F3 10.0 Tf 1 0 0 1 214.80 281.28 Tm <5461626C6520> Tj 1 0 0 1 245.04 281.28 Tm <313A20> Tj 1 0 0 1 257.04 281.04 Tm <436F6D706F736974696F6E20> Tj 1 0 0 1 319.92 281.04 Tm <6F6620> Tj 1 0 0 1 331.92 281.04 Tm <636174616C79737473> Tj 0.48 Tc 1 0 0 1 308.16 790.32 Tm <66696E616C20> Tj 1 0 0 1 331.20 790.56 Tm <70726F647563742E> Tj 0.48 Tc 1 0 0 1 322.32 777.60 Tm <54686520> Tj 1 0 0 1 342.48 777.60 Tm <726573756C747320> Tj 1 0 0 1 374.64 777.36 Tm <6F6620> Tj 1 0 0 1 386.64 777.60 Tm <483220> Tj 1 0 0 1 400.80 777.36 Tm <6368656D69736F727074696F6E20> Tj 1 0 0 1 467.52 777.36 Tm <646F20> Tj 1 0 0 1 481.20 777.60 Tm <6E6F7420> Tj 1 0 0 1 498.48 777.36 Tm <616772656520> Tj 1 0 0 1 524.88 777.36 Tm <77697468> Tj 0.48 Tc 1 0 0 1 308.16 764.88 Tm <74686F736520> Tj 1 0 0 1 335.04 764.88 Tm <6F6620> Tj 1 0 0 1 347.52 764.88 Tm <54454D2E20> Tj 1 0 0 1 377.52 764.88 Tm <496E20> Tj 1 0 0 1 389.76 764.88 Tm <483220> Tj 1 0 0 1 404.64 764.88 Tm <6368656D69736F727074696F6E2C20> Tj 1 0 0 1 474.48 764.88 Tm <746865726520> Tj 1 0 0 1 500.16 764.88 Tm <697320> Tj 1 0 0 1 510.72 764.88 Tm <6120> Tj 1 0 0 1 518.88 764.88 Tm <6C6172676572> Tj 0.72 Tc 1 0 0 1 308.16 752.16 Tm <646563726561736520> Tj 1 0 0 1 349.44 752.40 Tm <696E20> Tj 1 0 0 1 360.48 752.40 Tm <74686520> Tj 1 0 0 1 376.80 752.16 Tm <64697370657273696F6E20> Tj 1 0 0 1 425.52 752.40 Tm <76616C75657320> Tj 1 0 0 1 456.24 752.16 Tm <636F72726573706F6E64696E6720> Tj 1 0 0 1 522.24 752.16 Tm <746F20> Tj 1 0 0 1 533.52 752.16 Tm <616C6C> Tj 0.48 Tc 1 0 0 1 308.16 739.44 Tm <72757468656E69756D2D636F6E7461696E696E6720> Tj 1 0 0 1 425.76 739.68 Tm <6D6174657269616C7320> Tj 1 0 0 1 487.68 739.44 Tm <7468616E20> Tj 1 0 0 1 527.76 739.44 Tm <74686174> Tj 0.72 Tc 1 0 0 1 308.16 726.72 Tm <636F72726573706F6E64696E6720> Tj 1 0 0 1 375.60 726.72 Tm <746F20> Tj 1 0 0 1 388.56 726.72 Tm <74686520> Tj 1 0 0 1 406.56 726.72 Tm <6972696469756D20> Tj 1 0 0 1 443.28 726.72 Tm <6D6F6E6F6D6574616C6C696320> Tj 1 0 0 1 507.84 726.72 Tm <636174616C7973742C> Tj 0.72 Tc 1 0 0 1 308.16 713.76 Tm <62757420> Tj 1 0 0 1 324.96 714.00 Tm <7468697320> Tj 1 0 0 1 343.92 714.00 Tm <7472656E6420> Tj 1 0 0 1 369.84 714.00 Tm <77617320> Tj 1 0 0 1 389.52 714.00 Tm <6E6F7420> Tj 1 0 0 1 406.56 714.00 Tm <636F6E6669726D656420> Tj 1 0 0 1 455.04 713.76 Tm <627920> Tj 1 0 0 1 468.48 714.00 Tm <54454D2E20> Tj 1 0 0 1 497.52 714.00 Tm <5468697320> Tj 1 0 0 1 519.84 714.00 Tm <636F756C64> Tj 0.72 Tc 1 0 0 1 308.40 701.28 Tm <696E64696361746520> Tj 1 0 0 1 347.52 701.28 Tm <7468617420> Tj 1 0 0 1 368.64 701.28 Tm <527520> Tj 1 0 0 1 385.92 701.28 Tm <77617320> Tj 1 0 0 1 407.04 701.28 Tm <6E6F7420> Tj 1 0 0 1 425.76 701.28 Tm <74686F726F7567686C7920> Tj 1 0 0 1 478.80 701.28 Tm <7265647563656420> Tj 1 0 0 1 517.68 701.04 Tm <627920> Tj 1 0 0 1 533.04 701.28 Tm <482C> Tj 0.48 Tc 1 0 0 1 308.16 688.56 Tm <726564756374696F6E20> Tj 1 0 0 1 352.80 688.56 Tm <74726561746D656E74732E20> Tj 1 0 0 1 404.64 688.56 Tm <5468697320> Tj 1 0 0 1 427.20 688.56 Tm <636F6E636C7573696F6E20> Tj 1 0 0 1 478.08 688.56 Tm <61677265657320> Tj 1 0 0 1 508.80 688.56 Tm <7769746820> Tj 1 0 0 1 530.88 688.56 Tm <746865> Tj 0.96 Tc 1 0 0 1 308.40 675.84 Tm <776F726B20> Tj 1 0 0 1 333.60 675.84 Tm <6F6620> Tj 1 0 0 1 345.36 675.84 Tm <4E617269746120> Tj 1 0 0 1 376.08 675.84 Tm <657420> Tj 1 0 0 1 387.36 675.84 Tm <616C2E20> Tj 1 0 0 1 401.28 674.16 Tm <5B393837612C20> Tj 1 0 0 1 438.72 675.84 Tm <31393837625D2E> Tj 0.48 Tc 1 0 0 1 322.32 663.12 Tm <4C696E6520> Tj 1 0 0 1 345.84 663.36 Tm <70726573737572653A20> Tj 1 0 0 1 390.00 663.12 Tm <696E697469616C20> Tj 1 0 0 1 419.28 663.12 Tm <616E6420> Tj 1 0 0 1 438.48 663.12 Tm <66696E616C20> Tj 1 0 0 1 462.48 663.12 Tm <74656D706572617475726520> Tj 1 0 0 1 518.64 663.12 Tm <6F6620> Tj 1 0 0 1 530.88 663.12 Tm <746865> Tj 0.48 Tc 1 0 0 1 308.16 650.40 Tm <636174616C7974696320> Tj 1 0 0 1 350.16 650.40 Tm <6265642C20> Tj 1 0 0 1 373.68 650.40 Tm <617320> Tj 1 0 0 1 387.60 650.40 Tm <6D6561737572656420> Tj 1 0 0 1 434.64 650.40 Tm <6F6E20> Tj 1 0 0 1 450.00 650.40 Tm <74686520> Tj 1 0 0 1 468.24 650.40 Tm <6F7574657220> Tj 1 0 0 1 495.60 650.40 Tm <7369646520> Tj 1 0 0 1 517.44 650.40 Tm <6F6620> Tj 1 0 0 1 530.88 650.40 Tm <746865> Tj 0.48 Tc 1 0 0 1 307.92 637.68 Tm <656E76656C6F70652C20> Tj 1 0 0 1 354.24 637.68 Tm <616E6420> Tj 1 0 0 1 373.44 637.68 Tm <737461676E6174696F6E20> Tj 1 0 0 1 421.92 638.16 Tm <707265737375726520> Tj 1 0 0 1 462.48 637.92 Tm <696E20> Tj 1 0 0 1 473.76 637.68 Tm <74686520> Tj 1 0 0 1 490.08 637.92 Tm <6368616D62657220> Tj 1 0 0 1 531.12 637.92 Tm <617265> Tj 0.48 Tc 1 0 0 1 308.40 624.96 Tm <73686F776E20> Tj 1 0 0 1 342.96 625.20 Tm <696E20> Tj 1 0 0 1 357.36 625.20 Tm <5461626C6520> Tj 1 0 0 1 389.04 624.96 Tm <3520> Tj 1 0 0 1 400.32 625.20 Tm <666F7220> Tj 1 0 0 1 419.52 625.20 Tm <74686520> Tj 1 0 0 1 438.96 625.20 Tm <636F6E74696E756F757320> Tj 1 0 0 1 493.92 625.20 Tm <616E6420> Tj 1 0 0 1 515.52 625.44 Tm <70756C736564> Tj 0.72 Tc 1 0 0 1 308.16 612.24 Tm <6D6F6465732E20> Tj 1 0 0 1 343.68 612.24 Tm <54686520> Tj 1 0 0 1 365.52 612.24 Tm <74687275737465727320> Tj 1 0 0 1 408.48 612.48 Tm <757375616C6C7920> Tj 1 0 0 1 445.44 612.48 Tm <776F726B20> Tj 1 0 0 1 472.32 612.48 Tm <696E20> Tj 1 0 0 1 485.52 612.48 Tm <6120> Tj 1 0 0 1 494.40 612.48 Tm <626C6F772D646F776E> Tj 0.48 Tc 1 0 0 1 308.16 599.76 Tm <726567696D652C20> Tj 1 0 0 1 346.56 599.76 Tm <776869636820> Tj 1 0 0 1 378.48 599.76 Tm <6D65616E7320> Tj 1 0 0 1 411.60 599.76 Tm <7468617420> Tj 1 0 0 1 433.20 599.76 Tm <74686520> Tj 1 0 0 1 451.68 600.00 Tm <707265737375726520> Tj 1 0 0 1 493.92 599.76 Tm <696E20> Tj 1 0 0 1 507.12 599.76 Tm <74686520> Tj 1 0 0 1 525.60 599.76 Tm <74616E6B> Tj 0.72 Tc 1 0 0 1 308.16 587.28 Tm <28616E6420> Tj 1 0 0 1 332.88 586.80 Tm <696E20> Tj 1 0 0 1 345.84 586.80 Tm <74686520> Tj 1 0 0 1 364.32 587.04 Tm <6C696E652920> Tj 1 0 0 1 389.76 586.80 Tm <7374656164696C7920> Tj 1 0 0 1 429.12 586.80 Tm <64656372656173657320> Tj 1 0 0 1 476.64 587.04 Tm <617320> Tj 1 0 0 1 490.56 587.28 Tm <70726573737572697A696E67> Tj 0.48 Tc 1 0 0 1 307.92 574.08 Tm <6E6974726F67656E20> Tj 1 0 0 1 349.20 573.84 Tm <616E6468796472617A696E6520> Tj 1 0 0 1 414.72 574.08 Tm <61726520> Tj 1 0 0 1 431.52 574.08 Tm <636F6E73756D656420> Tj 1 0 0 1 480.00 574.56 Tm <284669672E20> Tj 1 0 0 1 505.20 574.08 Tm <31292E20> Tj 1 0 0 1 519.36 574.08 Tm <497420> Tj 1 0 0 1 528.96 574.08 Tm <63616E> Tj 0.48 Tc 1 0 0 1 308.16 561.36 Tm <616C736F20> Tj 1 0 0 1 330.72 561.36 Tm <626520> Tj 1 0 0 1 346.08 561.36 Tm <6F6273657276656420> Tj 1 0 0 1 390.96 561.36 Tm <746861742C20> Tj 1 0 0 1 415.68 561.36 Tm <617320> Tj 1 0 0 1 429.60 561.36 Tm <746865736520> Tj 1 0 0 1 457.44 561.84 Tm <70726573737572657320> Tj 1 0 0 1 503.52 561.36 Tm <64656372656173652C> Tj 0.48 Tc 1 0 0 1 307.92 548.64 Tm <74686520> Tj 1 0 0 1 331.20 548.64 Tm <696E697469616C20> Tj 1 0 0 1 366.72 548.64 Tm <616E6420> Tj 1 0 0 1 391.92 548.88 Tm <66696E616C20> Tj 1 0 0 1 421.92 548.64 Tm <62656420> Tj 1 0 0 1 447.36 548.64 Tm <74656D70657261747572657320> Tj 1 0 0 1 513.84 548.88 Tm <72656D61696E> Tj 0.48 Tc 1 0 0 1 307.92 536.16 Tm <70726163746963616C6C7920> Tj 1 0 0 1 364.56 536.16 Tm <756E6368616E67656420> Tj 1 0 0 1 422.64 536.16 Tm <666F7220> Tj 1 0 0 1 445.68 536.16 Tm <74686520> Tj 1 0 0 1 469.20 536.16 Tm <5368656C6C20> Tj 1 0 0 1 502.32 536.16 Tm <3430352C20> Tj 1 0 0 1 530.40 536.16 Tm <627574> Tj 0.48 Tc 1 0 0 1 308.40 523.20 Tm <7369676E69666963616E746C7920> Tj 1 0 0 1 370.80 523.20 Tm <646563726561736520> Tj 1 0 0 1 416.64 523.44 Tm <666F7220> Tj 1 0 0 1 437.04 523.20 Tm <74686520> Tj 1 0 0 1 457.92 523.20 Tm <6F7468657220> Tj 1 0 0 1 487.92 523.44 Tm <636174616C797374732C20> Tj 1 0 0 1 535.92 523.44 Tm <696E> Tj 0.48 Tc 1 0 0 1 307.92 510.72 Tm <706172746963756C617220> Tj 1 0 0 1 356.16 510.72 Tm <696E20> Tj 1 0 0 1 369.60 510.48 Tm <74686520> Tj 1 0 0 1 388.32 510.72 Tm <6361736520> Tj 1 0 0 1 412.80 510.72 Tm <6F6620> Tj 1 0 0 1 427.20 510.72 Tm <66696E616C20> Tj 1 0 0 1 452.64 510.72 Tm <62656420> Tj 1 0 0 1 473.76 510.72 Tm <74656D706572617475726520> Tj 1 0 0 1 531.36 510.72 Tm <666F72> Tj 0.72 Tc 1 0 0 1 308.16 497.52 Tm <72757468656E69756D2D636F6E7461696E696E6720> Tj 1 0 0 1 410.40 497.76 Tm <6D6174657269616C2E20> Tj 1 0 0 1 456.00 497.76 Tm <496E20> Tj 1 0 0 1 471.12 497.76 Tm <74686520> Tj 1 0 0 1 490.56 497.76 Tm <6361736520> Tj 1 0 0 1 515.76 497.76 Tm <6F6620> Tj 1 0 0 1 530.88 497.76 Tm <746865> Tj 0.72 Tc 1 0 0 1 308.16 485.04 Tm <494E504520> Tj 1 0 0 1 335.28 485.04 Tm <636174616C797374732C20> Tj 1 0 0 1 379.92 485.04 Tm <7468697320> Tj 1 0 0 1 399.12 485.04 Tm <636F756C6420> Tj 1 0 0 1 427.20 485.04 Tm <626520> Tj 1 0 0 1 441.12 485.04 Tm <617474726962757461626C6520> Tj 1 0 0 1 494.88 485.04 Tm <746F20> Tj 1 0 0 1 506.40 485.04 Tm <6120> Tj 1 0 0 1 514.08 485.04 Tm <6365727461696E> Tj 0.72 Tc 1 0 0 1 308.40 472.32 Tm <73656E736974697669747920> Tj 1 0 0 1 357.12 472.32 Tm <746F20> Tj 1 0 0 1 368.88 472.32 Tm <74686520> Tj 1 0 0 1 385.92 472.32 Tm <646563726561736520> Tj 1 0 0 1 427.68 472.56 Tm <696E20> Tj 1 0 0 1 439.44 472.32 Tm <68796472617A696E6520> Tj 1 0 0 1 486.24 472.56 Tm <666C6F7720> Tj 1 0 0 1 509.52 472.56 Tm <726174652E20> Tj 1 0 0 1 531.84 472.56 Tm <546F> Tj 0.72 Tc 1 0 0 1 307.92 459.36 Tm <6578616D696E6520> Tj 1 0 0 1 352.08 459.60 Tm <7468697320> Tj 1 0 0 1 374.88 459.60 Tm <6879706F7468657369732C20> Tj 1 0 0 1 431.76 459.60 Tm <74616E6B20> Tj 1 0 0 1 457.68 459.60 Tm <616E6420> Tj 1 0 0 1 480.48 459.84 Tm <6C696E6520> Tj 1 0 0 1 503.04 459.84 Tm <707265737375726573> Tj 0.48 Tc 1 0 0 1 308.16 446.64 Tm <7765726520> Tj 1 0 0 1 333.60 446.64 Tm <72657475726E656420> Tj 1 0 0 1 374.40 446.64 Tm <746F20> Tj 1 0 0 1 387.12 446.88 Tm <696E697469616C20> Tj 1 0 0 1 417.12 446.88 Tm <76616C75657320> Tj 1 0 0 1 449.28 446.64 Tm <6265666F726520> Tj 1 0 0 1 481.44 446.88 Tm <6561636820> Tj 1 0 0 1 505.44 446.88 Tm <7465737420> Tj 1 0 0 1 524.64 446.88 Tm <77697468> Tj 0.48 Tc 1 0 0 1 307.92 433.92 Tm <74686520> Tj 1 0 0 1 326.16 433.92 Tm <72757468656E69756D20> Tj 1 0 0 1 376.56 433.92 Tm <636174616C7973742C20> Tj 1 0 0 1 418.32 434.16 Tm <6D61696E7461696E696E6720> Tj 1 0 0 1 475.92 434.16 Tm <68796472617A696E6520> Tj 1 0 0 1 524.16 434.16 Tm <666C6F77> Tj 0.48 Tc 1 0 0 1 307.92 421.20 Tm <7261746520> Tj 1 0 0 1 329.28 421.20 Tm <616E6420> Tj 1 0 0 1 349.92 421.20 Tm <737461676E6174696F6E20> Tj 1 0 0 1 399.84 421.68 Tm <707265737375726520> Tj 1 0 0 1 441.84 421.44 Tm <696E20> Tj 1 0 0 1 454.80 421.44 Tm <74686520> Tj 1 0 0 1 472.80 421.44 Tm <6368616D62657220> Tj 1 0 0 1 515.04 421.44 Tm <616C6D6F7374> Tj 0.72 Tc 1 0 0 1 307.92 408.48 Tm <636F6E7374616E7420> Tj 1 0 0 1 349.68 408.48 Tm <647572696E6720> Tj 1 0 0 1 383.52 408.72 Tm <74686520> Tj 1 0 0 1 401.76 408.72 Tm <77686F6C6520> Tj 1 0 0 1 433.92 408.72 Tm <73657269657320> Tj 1 0 0 1 463.92 408.72 Tm <6F6620> Tj 1 0 0 1 477.60 408.72 Tm <74657374732E20> Tj 1 0 0 1 504.48 408.72 Tm <4576656E20> Tj 1 0 0 1 532.08 408.72 Tm <736F2C> Tj 0.48 Tc 1 0 0 1 307.92 395.76 Tm <74686520> Tj 1 0 0 1 324.24 395.76 Tm <636974656420> Tj 1 0 0 1 348.72 395.76 Tm <74656D70657261747572657320> Tj 1 0 0 1 408.96 396.00 Tm <636F6E74696E75656420> Tj 1 0 0 1 456.00 396.00 Tm <746F20> Tj 1 0 0 1 467.52 396.00 Tm <66616C6C2E> Tj 0.48 Tc 1 0 0 1 322.32 383.04 Tm <497420> Tj 1 0 0 1 332.40 383.04 Tm <63616E20> Tj 1 0 0 1 351.60 383.04 Tm <626520> Tj 1 0 0 1 366.00 383.28 Tm <636F6E636C7564656420> Tj 1 0 0 1 415.44 383.28 Tm <7468617420> Tj 1 0 0 1 436.32 383.28 Tm <74686520> Tj 1 0 0 1 453.60 383.28 Tm <6368616E676520> Tj 1 0 0 1 488.88 383.52 Tm <696E20> Tj 1 0 0 1 501.12 383.52 Tm <68796472617A696E65> Tj 0.48 Tc 1 0 0 1 307.92 370.32 Tm <666C6F7720> Tj 1 0 0 1 336.96 370.32 Tm <7261746520> Tj 1 0 0 1 362.64 370.32 Tm <697320> Tj 1 0 0 1 378.48 370.32 Tm <6E6F7420> Tj 1 0 0 1 401.28 370.56 Tm <726573706F6E7369626C6520> Tj 1 0 0 1 461.04 370.56 Tm <666F7220> Tj 1 0 0 1 482.64 370.56 Tm <74686520> Tj 1 0 0 1 504.72 370.56 Tm <6F62736572766564> Tj 0.48 Tc 1 0 0 1 307.92 357.36 Tm <74656D706572617475726520> Tj 1 0 0 1 364.08 357.36 Tm <64656372656173652E20> Tj 1 0 0 1 408.48 357.60 Tm <5468697320> Tj 1 0 0 1 431.76 357.60 Tm <697320> Tj 1 0 0 1 442.32 357.60 Tm <63617573656420> Tj 1 0 0 1 475.68 357.60 Tm <627920> Tj 1 0 0 1 489.84 357.60 Tm <74686520> Tj 1 0 0 1 506.40 357.60 Tm <646563617920> Tj 1 0 0 1 535.20 357.60 Tm <6F66> Tj 0.48 Tc 1 0 0 1 307.92 344.88 Tm <74686520> Tj 1 0 0 1 325.20 344.88 Tm <494E504520> Tj 1 0 0 1 353.04 344.88 Tm <636174616C7973747320> Tj 1 0 0 1 395.28 345.12 Tm <617320> Tj 1 0 0 1 408.24 345.12 Tm <7468657920> Tj 1 0 0 1 431.04 345.12 Tm <61726520> Tj 1 0 0 1 448.08 345.12 Tm <7573656420> Tj 1 0 0 1 472.08 345.12 Tm <6265636175736520> Tj 1 0 0 1 510.72 345.12 Tm <74686520> Tj 1 0 0 1 527.76 345.36 Tm <72617465> Tj 0.72 Tc 1 0 0 1 308.16 331.92 Tm <6F6620> Tj 1 0 0 1 324.24 332.16 Tm <6C6F737320> Tj 1 0 0 1 348.48 332.16 Tm <6F6620> Tj 1 0 0 1 364.56 332.16 Tm <6D61737320> Tj 1 0 0 1 393.60 332.16 Tm <697320> Tj 1 0 0 1 408.24 332.16 Tm <7374696C6C20> Tj 1 0 0 1 432.00 332.40 Tm <7665727920> Tj 1 0 0 1 458.40 332.16 Tm <656C65766174656420> Tj 1 0 0 1 502.08 332.40 Tm <666F7220> Tj 1 0 0 1 521.52 332.40 Tm <7468657365> Tj 0.48 Tc 1 0 0 1 307.92 319.68 Tm <70726F64756374732C20> Tj 1 0 0 1 352.32 319.44 Tm <696E20> Tj 1 0 0 1 363.84 319.68 Tm <706172746963756C617220> Tj 1 0 0 1 409.68 319.68 Tm <666F7220> Tj 1 0 0 1 426.00 319.68 Tm <74686520> Tj 1 0 0 1 442.80 319.44 Tm <72757468656E69756D20> Tj 1 0 0 1 491.28 319.44 Tm <6F6E65732C20> Tj 1 0 0 1 517.20 319.68 Tm <617320> Tj 1 0 0 1 528.96 319.68 Tm <63616E> Tj 0.72 Tc 1 0 0 1 307.92 306.72 Tm <626520> Tj 1 0 0 1 321.60 306.72 Tm <7365656E20> Tj 1 0 0 1 343.92 306.72 Tm <696E20> Tj 1 0 0 1 355.20 306.72 Tm <5461626C6520> Tj 1 0 0 1 383.76 306.72 Tm <362E> Tj 0.96 Tc /F3 7.0 Tf 1 0 0 1 128.88 126.00 Tm <2A2D2843292D436F696D707265676E6174696F6E> Tj 0.48 Tc 1 0 0 1 134.88 114.00 Tm <2D20> Tj 1 0 0 1 139.68 112.80 Tm <28532920> Tj 1 0 0 1 151.68 113.76 Tm <2D20> Tj 1 0 0 1 156.24 112.08 Tm <5375636363737369766520> Tj 1 0 0 1 193.92 112.08 Tm <496D707265676E6174696F6E73> Tj 0.72 Tc /F3 8.0 Tf 1 0 0 1 117.36 247.92 Tm <53616D706C652D> Tj 0.48 Tc 1 0 0 1 210.48 255.36 Tm <4D61737320> Tj 1 0 0 1 232.80 255.36 Tm <6672616374696F6E> Tj 0.24 Tc 1 0 0 1 307.68 255.12 Tm <41746F6D696320> Tj 1 0 0 1 337.92 255.12 Tm <6672616374696F6E> Tj 0.24 Tc 1 0 0 1 402.48 255.12 Tm <41746F6D696320> Tj 1 0 0 1 432.96 255.12 Tm <726174696F> Tj 0.72 Tc 1 0 0 1 217.68 240.72 Tm <28566F2920> Tj 1 0 0 1 234.48 240.00 Tm <4972> Tj 0.48 Tc 1 0 0 1 264.48 240.48 Tm <28376F2920> Tj 1 0 0 1 281.28 239.76 Tm <5275> Tj 0.72 Tc /F3 7.0 Tf 1 0 0 1 312.72 240.48 Tm <2856612920> Tj 1 0 0 1 329.76 239.76 Tm <68> Tj 1.20 Tc /F3 9.0 Tf 1 0 0 1 358.08 240.48 Tm <28252920> Tj 1 0 0 1 375.12 239.76 Tm <5275> Tj 0.24 Tc 1 0 0 1 425.76 239.76 Tm <52FA4972> Tj 0.72 Tc 1 0 0 1 117.60 225.36 Tm <532D4972> Tj 0.96 Tc 1 0 0 1 117.36 210.96 Tm <432D3249726C5275> Tj 1.44 Tc 1 0 0 1 117.36 196.08 Tm <432D6C6C726C5275> Tj 0.96 Tc 1 0 0 1 117.60 181.68 Tm <532D20> Tj 1 0 0 1 126.48 181.68 Tm <6C20> Tj 1 0 0 1 130.32 181.68 Tm <49726C20> Tj 1 0 0 1 140.88 181.68 Tm <5275> Tj 0.00 Tc 1 0 0 1 117.36 167.04 Tm <432D20> Tj 1 0 0 1 127.68 167.28 Tm <4920> Tj 1 0 0 1 131.28 167.28 Tm <4972325275> Tj 0.00 Tc 1 0 0 1 117.60 152.40 Tm <532D20> Tj 1 0 0 1 126.48 152.40 Tm <4920> Tj 1 0 0 1 130.32 152.40 Tm <4972325275> Tj 0.72 Tc 1 0 0 1 117.60 138.00 Tm <532D5275> Tj 0.96 Tc 1 0 0 1 225.36 225.12 Tm <3330> Tj 0.72 Tc 1 0 0 1 225.36 210.72 Tm <3230> Tj 1.50 Tc 1 0 0 1 226.08 196.08 Tm <7435> Tj 1.50 Tc 1 0 0 1 226.32 181.44 Tm <6C35> Tj 1.50 Tc 1 0 0 1 226.08 167.04 Tm <6C30> Tj 1.50 Tc 1 0 0 1 226.08 152.16 Tm <6C30> Tj 0.00 Tc 1 0 0 1 227.28 137.76 Tm <30> Tj 0.00 Tc 1 0 0 1 276.24 224.88 Tm <30> Tj 1.50 Tc 1 0 0 1 275.04 210.48 Tm <6C30> Tj 1.50 Tc 1 0 0 1 275.04 195.84 Tm <3135> Tj 1.50 Tc 1 0 0 1 275.04 181.20 Tm <7435> Tj 0.24 Tc 1 0 0 1 274.32 166.80 Tm <3230> Tj 0.48 Tc 1 0 0 1 274.32 152.16 Tm <3230> Tj 0.72 Tc 1 0 0 1 274.32 137.52 Tm <3330> Tj 1.20 Tc 1 0 0 1 318.96 224.88 Tm <313030> Tj 1.50 Tc 1 0 0 1 317.04 210.48 Tm <35312E33> Tj 0.48 Tc 1 0 0 1 317.04 195.60 Tm <33342E35> Tj 0.48 Tc /F3 6.0 Tf 1 0 0 1 317.04 181.44 Tm <2D4A342E2D29> Tj 0.72 Tc /F3 9.0 Tf 1 0 0 1 317.04 166.80 Tm <32312E38> Tj 1.50 Tc 1 0 0 1 317.04 152.16 Tm <32312E38> Tj 0.00 Tc 1 0 0 1 322.56 137.52 Tm <30> Tj 0.00 Tc 1 0 0 1 369.84 224.88 Tm <30> Tj 0.24 Tc 1 0 0 1 364.80 210.48 Tm <34382E2737> Tj 0.96 Tc 1 0 0 1 364.32 195.60 Tm <36352E35> Tj 0.96 Tc 1 0 0 1 364.32 181.20 Tm <36352E35> Tj 0.72 Tc 1 0 0 1 364.08 171.60 Tm <2737392E32> Tj 0.72 Tc 1 0 0 1 364.08 156.72 Tm <2737392E32> Tj 0.96 Tc 1 0 0 1 366.24 137.52 Tm <313030> Tj 0.72 Tc 1 0 0 1 428.40 224.88 Tm <302E3030> Tj 0.96 Tc 1 0 0 1 428.40 210.48 Tm <302E3935> Tj 1.44 Tc 1 0 0 1 431.76 195.84 Tm <312E39> Tj 1.44 Tc 1 0 0 1 431.76 181.20 Tm <312E39> Tj 1.44 Tc 1 0 0 1 431.04 166.80 Tm <332E38> Tj 1.44 Tc 1 0 0 1 431.04 151.92 Tm <332E38> Tj 0.24 Tc /F3 7.0 Tf 1 0 0 1 222.96 89.04 Tm <4272757A2E696C69616E20> Tj 1 0 0 1 254.88 89.04 Tm <4A6F75726E616C20> Tj 1 0 0 1 282.48 88.80 Tm <6F6620> Tj 1 0 0 1 291.36 88.80 Tm <4368656E746963616C20> Tj 1 0 0 1 324.48 89.04 Tm <456E67696E656572696E67> Tj ET endstream endobj 31 0 obj 30897 endobj 32 0 obj << /Length 33 0 R >> stream 216 RESULTS AND DISCUSSIONTable I shows metal contents (on mass andatomic bases) and the IrlRu atomic ratio for allcatalysts prepared. As the differences between realand nominal metal contents, measured by gravimetricchemical analysis, were below 2Va, nominal valuesshown in Table 1 will be accepted as the rcal ones.Table 2 shows the values for specific area, porevolume, number of sites, and dispersion for allcatalysts, including Shell405 which was taken as thereference. It is interesting to note its small porevolume. It can be observed that the addition of 307oiridium barely affects the surface area and specificvolume of the alumina, showing that pore occlusiondue to introduction of the metal can be neglected.The results obtained by H, chemisorption clearlyshow that ruthenium is much less dispersed thaniridium. Even in the bimetallic catalysts, as theruthenium content increases, the dispersiondecreases.Tables 3 and 4 contain the results obtained byTEM. In Table 3 they show that almost 907a of themonometallic iridium catalyst particle diameters and5lVo of the ruthenium ones are shorter than 4.1 nm.The results for bimetallic catalysts fall betweenthese, with ruthenium reflecting the trend towards anincrease in the mean size of the metal particles. InTable 4 it can be seen that the mean diameters ofruthenium particles are about 60Vo higher than thoseof iridium particles no matter which of the twoequations shown is selected for their calculation.These results also show that the decrease inspecific volume of the pores was negligible. Thisassures that the introduction of 307a metal will notimpair the diffusion of gases during the hydrazinedecomposition reaction. Despite its introduction,which reduces the available specific surface of thealumina, the metal is still very well distributed in the T.G.Soares Neto. J.Gobbo-Ferreira. A.J.G.Cobo and G.M.Cruz Table 1: Composition of catalysts final product.The results of H2 chemisorption do not agree withthose of TEM. In H2 chemisorption, there is a largerdecrease in the dispersion values corresponding to allruthenium-containing materials than thatcorresponding to the iridium monometallic catalyst,but this trend was not confirmed by TEM. This couldindicate that Ru was not thoroughly reduced by H,reduction treatments. This conclusion agrees with thework of Narita et al. [987a, 1987b].Line pressure: initial and final temperature of thecatalytic bed, as measured on the outer side of theenvelope, and stagnation pressure in the chamber areshown in Table 5 for the continuous and pulsedmodes. The thrusters usually work in a blow-downregime, which means that the pressure in the tank(and in the line) steadily decreases as pressurizingnitrogen andhydrazine are consumed (Fig. 1). It canalso be observed that, as these pressures decrease,the initial and final bed temperatures remainpractically unchanged for the Shell 405, butsignificantly decrease for the other catalysts, inparticular in the case of final bed temperature forruthenium-containing material. In the case of theINPE catalysts, this could be attributable to a certainsensitivity to the decrease in hydrazine flow rate. Toexamine this hypothesis, tank and line pressureswere returned to initial values before each test withthe ruthenium catalyst, maintaining hydrazine flowrate and stagnation pressure in the chamber almostconstant during the whole series of tests. Even so,the cited temperatures continued to fall.It can be concluded that the change in hydrazineflow rate is not responsible for the observedtemperature decrease. This is caused by the decay ofthe INPE catalysts as they are used because the rateof loss of mass is still very elevated for theseproducts, in particular for the ruthenium ones, as canbe seen in Table 6. *-(C)-Coimpregnation- (S) - Succcssive Impregnations Sample- Mass fraction Atomic fraction Atomic ratio (Vo) Ir (7o) Ru (Va) h (%) Ru RIr S-IrC-2IrlRuC-llrlRuS- l Irl RuC- I Ir2RuS- I Ir2RuS-Ru 3020t5l5l0l00 0l015t5202030 10051.334.5-J4.-)21.821.80 048.'765.565.5'79.2'79.2100 0.000.951.91.93.83.8 Bruz.ilian Journal of Chentical Engineering endstream endobj 33 0 obj 4114 endobj 34 0 obj << /Length 27 >> stream % CANON_PFINF_TYPE0_TEXTON endstream endobj 35 0 obj << /Length 45 >> stream q 595.20 0 0 841.68 0.00 0.00 cm /Obj29 Do Q endstream endobj 36 0 obj << /Type /Page /MediaBox [ 0 0 595.20 841.68 ] /Parent 11 0 R /Resources << /Font << /F3 5 0 R >> /XObject << /Obj29 29 0 R >> /Subtype 32 0 R /ProcSet [ /PDF /Text /ImageB /ImageC /ImageI ] >> /Contents [ 34 0 R 35 0 R 30 0 R ] >> endobj 37 0 obj << /Type /XObject /Subtype /Image /Width 2480 /Height 3507 /BitsPerComponent 1 /ColorSpace /DeviceGray /Filter /CCITTFaxDecode /DecodeParms << /K -1 /Columns 2480 >> /Length 26112 >> stream &bj(S*(PVI08 0t#4/C  jE#uAv跻'zMȲ#( u:57BYvf(wޅzʕu]~Ѡ"?&:vx3p3A1ҏOuu#gzaCz.y3Y<~qϲtn2|޺CI!G=={BhxG0 63sRB+m컷[I>H7u/|?7Nl5oJfn^_wexAc޸tKպmU~|]P=t(}ûa߭;}G~zW8]Mz0B?=6=7[چ J~_Sk_oom#uozmmڄ쐿'||l_oIzV_iPA#R %uV^WBj&Bda4X;IT5UNմW]Z}ҿ%X K&L&BiQA&C.l6M86Mm&/m%TU!DDDhDDDDD B !a0 z*)'i_(Q[3QJMi'bBJ B(J A R NPJ G XZֵ-k XZ Z ¬CP z vY!à<3vHd!aP DvA!6䎭Q'jDmv_[-ޫ$`F;A﮺l:  Gij!0͝_k{i+V0h0oI鷯$aïֿU_յ}w_׉3/_[pytH!M *Z^AbK; C0"rG2/,AJg?bxuk_Ez~ D={&;A4,&2_8fJW]_oxkG:MF vl"v݄h 8Mpvaaf31 pyMpSfff]߼'JҽW'Iaa&| 0A0!؆0G.39qLr ¶M/!/ȃm~6Ɠm4{'pL' !ŨA26!vB<8 53Q6}zj=+נL;[ҷi/ݑN;Ioطŧ"vPl//pa0a ؁4Dp|C⽽C#vc{ޞEaJJHU6I>- pbvQ"p-z^῵jKo;m+^_ȑADw[jN0ྲ1%ᯰ_]/k_VӺ:W"_Ko'껑 PoR1}{-o5_IO%?z?6_ }zKp$?}j_KK'j׎_TmCOz/K*?DuE[fzmwm/kM?_Vmohu~K ?}l0m׿߻}vf'G%݇!;Jؠ[WN}ڶ{ϭ=p_h΁åZAkt|CW+V*_VXal/u]f}?ïӞ?Aj) F SLUݱRp튈}קSVfNt0㈈1ʰA= S CpA0i G4=qNvtV]׫inM4 3Sه({ L(Wl j]6)N׿aӽoK׈m%jFAMNnXV]ouj^`XD״RC zo &MYM4Ab(-Wd#bm$6DDDDGH4" )JAp )BTL2+DA m%DDDDDDDD :!jtM6ʀp q 6)4#:]-DDDDG.*I*%KA-7Fm@H qA)%Gm,S A1Mԛ@R#t#VNޡWIpOv=~?F!ݸL"C. 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Tj 1 0 0 1 361.20 751.92 Tm <6E756D62657220> Tj 1 0 0 1 401.52 751.68 Tm <6F6620> Tj 1 0 0 1 413.76 751.68 Tm <73697465732C20> Tj 1 0 0 1 440.16 751.44 Tm <616E6420> Tj 1 0 0 1 460.80 751.44 Tm <64697370657273696F6E2E> Tj 0.48 Tc /F3 9.0 Tf 1 0 0 1 129.36 726.72 Tm <436174616C797374> Tj 0.48 Tc /F3 8.0 Tf 1 0 0 1 201.84 726.24 Tm <536720> Tj 1 0 0 1 214.08 726.96 Tm <286D322E6727746C6F72> Tj 0.48 Tc 1 0 0 1 278.64 726.00 Tm <567020> Tj 1 0 0 1 292.56 726.72 Tm <28636D332E672D743B747A6C> Tj 0.48 Tc 1 0 0 1 354.48 725.52 Tm <53697465732E672D7220> Tj 1 0 0 1 387.12 726.24 Tm <287820> Tj 1 0 0 1 397.20 725.52 Tm <3130323029> Tj 0.48 Tc /F3 9.0 Tf 1 0 0 1 436.08 725.52 Tm <44697370657273696F6E20> Tj 1 0 0 1 479.52 726.00 Tm <282529> Tj 0.72 Tc /F3 8.0 Tf 1 0 0 1 128.16 711.84 Tm <5368656C6C20> Tj 1 0 0 1 148.80 711.84 Tm <343035> Tj 0.72 Tc 1 0 0 1 138.48 697.44 Tm <532D4972> Tj 0.72 Tc 1 0 0 1 127.68 683.28 Tm <432D3249726C20> Tj 1 0 0 1 152.16 683.28 Tm <5275> Tj 1.20 Tc 1 0 0 1 127.68 668.88 Tm <432D6C49726C5275> Tj 0.96 Tc 1 0 0 1 128.40 654.48 Tm <532D20> Tj 1 0 0 1 137.28 654.48 Tm <3120> Tj 1 0 0 1 141.12 654.48 Tm <49726C20> Tj 1 0 0 1 151.44 654.48 Tm <5275> Tj 1.20 Tc 1 0 0 1 127.68 639.84 Tm <432D20> Tj 1 0 0 1 138.00 640.08 Tm <6C6C72325275> Tj 1.20 Tc 1 0 0 1 128.40 625.44 Tm <532D20> Tj 1 0 0 1 137.52 625.44 Tm <6C6C726C5275> Tj 0.96 Tc 1 0 0 1 136.32 611.04 Tm <532D522E72> Tj 1.44 Tc /F3 9.0 Tf 1 0 0 1 219.60 711.60 Tm <743134> Tj 0.72 Tc 1 0 0 1 219.36 697.20 Tm <313435> Tj 0.72 Tc 1 0 0 1 219.60 682.80 Tm <743334> Tj 1.50 Tc 1 0 0 1 219.36 668.40 Tm <313331> Tj 0.72 Tc 1 0 0 1 219.60 639.60 Tm <743334> Tj 0.48 Tc 1 0 0 1 219.36 625.20 Tm <313437> Tj 1.50 Tc 1 0 0 1 219.60 610.80 Tm <313238> Tj 1.20 Tc 1 0 0 1 297.12 711.12 Tm <302E20> Tj 1 0 0 1 305.04 711.12 Tm <3136> Tj 0.96 Tc 1 0 0 1 297.12 696.72 Tm <302E3431> Tj 0.72 Tc 1 0 0 1 297.12 682.32 Tm <302E33276C> Tj 0.96 Tc 1 0 0 1 296.88 667.92 Tm <302E3338> Tj 0.96 Tc 1 0 0 1 296.88 653.52 Tm <302E3339> Tj 0.96 Tc 1 0 0 1 296.88 639.12 Tm <302E3335> Tj 0.72 Tc 1 0 0 1 296.88 624.72 Tm <302E3430> Tj 1.20 Tc 1 0 0 1 296.88 610.32 Tm <302E3339> Tj 0.96 Tc 1 0 0 1 378.96 710.88 Tm <342E33> Tj 0.96 Tc 1 0 0 1 378.96 696.48 Tm <342E36> Tj 1.50 Tc 1 0 0 1 379.92 682.32 Tm <312E35> Tj 1.50 Tc /F3 4.0 Tf 1 0 0 1 380.16 667.92 Tm <6C2E4A> Tj 1.44 Tc /F3 9.0 Tf 1 0 0 1 379.92 653.52 Tm <312E34> Tj 1.50 Tc 1 0 0 1 379.92 638.88 Tm <312E32> Tj 1.50 Tc 1 0 0 1 379.68 624.48 Tm <312E33> Tj 1.50 Tc 1 0 0 1 379.68 610.08 Tm <312E30> Tj 0.96 Tc 1 0 0 1 456.72 710.64 Tm <34352E38> Tj 0.48 Tc 1 0 0 1 457.44 696.24 Tm <34392E30> Tj 1.44 Tc 1 0 0 1 457.68 682.08 Tm <31332E30> Tj 1.20 Tc 1 0 0 1 461.28 667.44 Tm <392E32> Tj 0.96 Tc 1 0 0 1 457.68 653.28 Tm <7220> Tj 1 0 0 1 461.28 653.04 Tm <302E30> Tj 1.20 Tc 1 0 0 1 461.52 638.64 Tm <382E30> Tj 1.20 Tc 1 0 0 1 461.52 624.24 Tm <382E39> Tj 1.20 Tc 1 0 0 1 461.28 609.60 Tm <352E36> Tj 0.96 Tc /F3 5.0 Tf 1 0 0 1 136.56 598.56 Tm <542D20> Tj 1 0 0 1 150.00 599.76 Tm <2D> Tj 0.96 Tc /F3 10.0 Tf 1 0 0 1 136.56 587.28 Tm <2C2E20> Tj 1 0 0 1 149.76 588.48 Tm <2D> Tj 1.20 Tc /F3 4.0 Tf 1 0 0 1 167.52 596.88 Tm <3A6C3A2D692E> Tj 0.72 Tc /F3 7.0 Tf 1 0 0 1 198.96 601.20 Tm <2D20> Tj 1 0 0 1 204.96 596.64 Tm <3A20> Tj 1 0 0 1 210.96 596.64 Tm <2E6C6C756E723A6E7220> Tj 1 0 0 1 239.28 596.64 Tm <683A2E7220> Tj 1 0 0 1 252.24 596.40 Tm <2C7220> Tj 1 0 0 1 257.76 596.40 Tm <2E706363EC66EC6320> Tj 1 0 0 1 284.88 596.40 Tm <73757274EC636520> Tj 1 0 0 1 310.32 596.16 Tm <6172656120> Tj 1 0 0 1 325.44 596.16 Tm <6F6620> Tj 1 0 0 1 335.28 596.16 Tm <4920> Tj 1 0 0 1 338.16 596.16 Tm <343820> Tj 1 0 0 1 348.48 595.92 Tm <6E743A2E> Tj 0.96 Tc 1 0 0 1 198.96 589.92 Tm <2D3A3A6C756E726E6C20> Tj 1 0 0 1 239.28 585.36 Tm <66693B7220> Tj 1 0 0 1 252.00 585.36 Tm <2D272C20> Tj 1 0 0 1 258.00 586.08 Tm <727072273A6966EC6320> Tj 1 0 0 1 284.88 585.12 Tm <702E72726520> Tj 1 0 0 1 301.20 585.36 Tm <726FEC756E746320> Tj 1 0 0 1 327.12 584.88 Tm <6F6620> Tj 1 0 0 1 335.76 585.12 Tm <302E2D313520> Tj 1 0 0 1 352.08 584.64 Tm <636E7472> Tj 0.72 Tc /F3 10.0 Tf 1 0 0 1 97.20 522.96 Tm <5461626C6520> Tj 1 0 0 1 127.20 522.72 Tm <333A20> Tj 1 0 0 1 142.08 522.72 Tm <446973747269627574696F6E20> Tj 1 0 0 1 203.28 522.24 Tm <6F6620> Tj 1 0 0 1 215.52 522.24 Tm <74686520> Tj 1 0 0 1 233.04 522.24 Tm <6D6574616C20> Tj 1 0 0 1 262.56 522.48 Tm <7061727469636C6520> Tj 1 0 0 1 301.68 521.76 Tm <6469616D657465727320> Tj 1 0 0 1 351.36 521.76 Tm <6F6620> Tj 1 0 0 1 363.60 521.76 Tm <74686520> Tj 1 0 0 1 381.36 521.76 Tm <6361746168277374732E20> Tj 1 0 0 1 427.92 521.52 Tm <6F627461696E656420> Tj 1 0 0 1 472.08 521.28 Tm <627620> Tj 1 0 0 1 486.72 521.28 Tm <54454ECD> Tj 0.48 Tc 1 0 0 1 109.92 314.64 Tm <5461626C6520> Tj 1 0 0 1 139.92 314.64 Tm <343A20> Tj 1 0 0 1 155.04 314.40 Tm <4D65616E20> Tj 1 0 0 1 185.04 314.16 Tm <6F6620> Tj 1 0 0 1 197.04 314.16 Tm <74686520> Tj 1 0 0 1 214.80 314.16 Tm <6469616D657465727320> Tj 1 0 0 1 264.24 313.92 Tm <6D6574616C20> Tj 1 0 0 1 293.76 314.16 Tm <7061727469636C657320> Tj 1 0 0 1 337.44 313.68 Tm <6F6620> Tj 1 0 0 1 349.44 313.68 Tm <74686520> Tj 1 0 0 1 367.20 313.44 Tm <636174616C797374732C20> Tj 1 0 0 1 413.52 313.44 Tm <6F627461696E656420> Tj 1 0 0 1 457.92 313.20 Tm <627920> Tj 1 0 0 1 472.56 313.44 Tm <54424D> Tj 1.50 Tc /F3 16.0 Tf 1 0 0 1 182.16 151.20 Tm <722D6C6E722E723D23> Tj 1.50 Tc /F3 9.0 Tf 1 0 0 1 252.48 150.96 Tm <322D6A315E273D296E2C2E6166> Tj 1.20 Tc 1 0 0 1 288.24 138.24 Tm <5322EC2C> Tj 0.96 Tc /F3 4.0 Tf 1 0 0 1 288.00 133.20 Tm <4C2F223120> Tj 1 0 0 1 306.72 137.04 Tm <276C> Tj 0.48 Tc /F3 8.0 Tf 1 0 0 1 111.84 488.88 Tm <436174616C797374> Tj 0.72 Tc /F3 7.0 Tf 1 0 0 1 175.20 488.88 Tm <6E286C29> Tj 0.48 Tc /F3 8.0 Tf 1 0 0 1 269.04 495.84 Tm <50657263656E7461676520> Tj 1 0 0 1 313.68 495.60 Tm <6F6620> Tj 1 0 0 1 323.52 496.08 Tm <7061727469636C6520> Tj 1 0 0 1 355.20 495.60 Tm <6469616D657465727320> Tj 1 0 0 1 394.80 495.60 Tm <696E20> Tj 1 0 0 1 404.88 495.36 Tm <6561636820> Tj 1 0 0 1 424.56 495.36 Tm <72616E6765> Tj 1.50 Tc /F3 9.0 Tf 1 0 0 1 223.20 480.72 Tm <302D32> Tj 1.50 Tc 1 0 0 1 278.16 480.48 Tm <322E312D20> Tj 1 0 0 1 297.12 480.48 Tm <34> Tj 1.50 Tc 1 0 0 1 341.28 480.24 Tm <342E312D38> Tj 0.96 Tc /F3 10.0 Tf 1 0 0 1 397.68 480.00 Tm <382E7220> Tj 1 0 0 1 411.60 481.68 Tm <2D20> Tj 1 0 0 1 417.12 480.00 Tm <7432> Tj 1.50 Tc /F3 8.0 Tf 1 0 0 1 467.76 479.52 Tm <3E3132> Tj 0.72 Tc /F3 9.0 Tf 1 0 0 1 120.72 466.08 Tm <532D4972> Tj 0.72 Tc 1 0 0 1 109.92 451.44 Tm <432D324972315275> Tj 1.20 Tc 1 0 0 1 109.92 437.04 Tm <432D6C49726C5275> Tj 1.20 Tc 1 0 0 1 110.64 422.64 Tm <532D6C49726C5275> Tj 0.72 Tc 1 0 0 1 109.92 408.24 Tm <432D6C4972325275> Tj 0.72 Tc 1 0 0 1 110.40 393.84 Tm <532D6C4972325275> Tj 0.72 Tc 1 0 0 1 118.08 379.20 Tm <532D5275> Tj 0.72 Tc 1 0 0 1 176.88 465.60 Tm <363230> Tj 0.96 Tc 1 0 0 1 176.64 451.20 Tm <373431> Tj 0.24 Tc 1 0 0 1 177.12 436.80 Tm <363336> Tj 0.96 Tc 1 0 0 1 176.64 422.40 Tm <353638> Tj 1.20 Tc 1 0 0 1 176.64 408.00 Tm <333330> Tj 0.72 Tc 1 0 0 1 176.64 393.60 Tm <363232> Tj 0.48 Tc 1 0 0 1 177.12 378.96 Tm <363431> Tj 0.72 Tc 1 0 0 1 221.52 465.60 Tm <34312E3333> Tj 0.48 Tc 1 0 0 1 221.04 450.96 Tm <33342E3234> Tj 1.44 Tc 1 0 0 1 221.04 436.56 Tm <33312E3636> Tj 0.48 Tc 1 0 0 1 220.56 422.16 Tm <34322E277430> Tj 0.48 Tc 1 0 0 1 221.04 407.76 Tm <32352E3932> Tj 0.96 Tc 1 0 0 1 220.80 393.36 Tm <33322E3735> Tj 0.96 Tc 1 0 0 1 221.52 378.96 Tm <31352E3233> Tj 0.72 Tc 1 0 0 1 279.12 465.36 Tm <34362E3636> Tj 0.48 Tc 1 0 0 1 279.84 450.72 Tm <34352E3433> Tj 0.48 Tc 1 0 0 1 279.84 436.32 Tm <34352E3438> Tj 0.72 Tc 1 0 0 1 279.12 421.92 Tm <34302E3038> Tj 0.72 Tc 1 0 0 1 279.12 407.52 Tm <34342E3230> Tj 0.72 Tc 1 0 0 1 278.88 393.12 Tm <34342E3730> Tj 1.44 Tc 1 0 0 1 278.88 378.48 Tm <34312E3638> Tj 1.44 Tc 1 0 0 1 343.44 465.12 Tm <4920> Tj 1 0 0 1 348.00 465.12 Tm <722E3335> Tj 0.96 Tc 1 0 0 1 343.44 450.48 Tm <31392E3539> Tj 0.48 Tc 1 0 0 1 342.72 436.08 Tm <32302E3937> Tj 1.20 Tc 1 0 0 1 343.44 421.68 Tm <31362E3031> Tj 0.96 Tc 1 0 0 1 342.48 407.28 Tm <32372E3838> Tj 0.72 Tc 1 0 0 1 342.48 392.88 Tm <32302E3833> Tj 0.48 Tc 1 0 0 1 342.48 378.24 Tm <33362E3236> Tj 0.72 Tc 1 0 0 1 403.68 464.88 Tm <302E3438> Tj 0.96 Tc /F3 11.0 Tf 1 0 0 1 403.68 450.24 Tm <302E3520> Tj 1 0 0 1 416.16 450.48 Tm <72> Tj 1.20 Tc /F3 9.0 Tf 1 0 0 1 404.64 436.08 Tm <312E3635> Tj 1.50 Tc 1 0 0 1 404.64 421.68 Tm <742E326C> Tj 1.50 Tc 1 0 0 1 404.64 407.04 Tm <312E3531> Tj 1.44 Tc 1 0 0 1 404.40 392.64 Tm <312E3732> Tj 1.20 Tc 1 0 0 1 403.44 378.24 Tm <352E3836> Tj 1.44 Tc 1 0 0 1 467.28 464.64 Tm <302E3138> Tj 0.48 Tc 1 0 0 1 467.28 450.00 Tm <302E273233> Tj 0.72 Tc 1 0 0 1 467.28 435.84 Tm <302E3234> Tj 0.72 Tc 1 0 0 1 467.28 421.20 Tm <302E3030> Tj 0.72 Tc 1 0 0 1 467.28 406.80 Tm <302E3439> Tj 0.72 Tc 1 0 0 1 467.04 392.40 Tm <302E3030> Tj 0.96 Tc 1 0 0 1 467.04 378.00 Tm <302E3937> Tj 0.48 Tc /F3 7.0 Tf 1 0 0 1 125.52 365.28 Tm <4920> Tj 1 0 0 1 130.32 366.72 Tm <2D20> Tj 1 0 0 1 136.80 365.04 Tm <4E75726E62657220> Tj 1 0 0 1 165.36 364.80 Tm <6F6620> Tj 1 0 0 1 174.00 365.04 Tm <7061727469636C657320> Tj 1 0 0 1 203.52 364.80 Tm <636F756E746364> Tj 0.72 Tc /F3 8.0 Tf 1 0 0 1 371.04 283.20 Tm <6A20> Tj 1 0 0 1 379.44 281.76 Tm <6C74656C20> Tj 1 0 0 1 393.12 285.12 Tm <286E6D29283229> Tj 0.96 Tc /F3 9.0 Tf 1 0 0 1 205.92 264.48 Tm <532D6C7220> Tj 1 0 0 1 298.08 264.00 Tm <322E3420> Tj 1 0 0 1 388.80 263.76 Tm <342E37> Tj 0.96 Tc 1 0 0 1 195.36 250.08 Tm <432D3249726C20> Tj 1 0 0 1 219.60 250.08 Tm <527520> Tj 1 0 0 1 298.08 249.36 Tm <322E3820> Tj 1 0 0 1 389.04 249.12 Tm <352E35> Tj 0.96 Tc 1 0 0 1 195.36 235.44 Tm <432D20> Tj 1 0 0 1 205.44 235.44 Tm <6C20> Tj 1 0 0 1 209.28 235.44 Tm <49726C20> Tj 1 0 0 1 219.60 235.20 Tm <527520> Tj 1 0 0 1 297.84 234.72 Tm <322E3920> Tj 1 0 0 1 389.04 234.48 Tm <352E34> Tj 0.96 Tc 1 0 0 1 196.08 220.80 Tm <532D20> Tj 1 0 0 1 204.96 221.04 Tm <6C6C726C20> Tj 1 0 0 1 219.12 220.80 Tm <527520> Tj 1 0 0 1 297.84 220.32 Tm <322E273720> Tj 1 0 0 1 388.80 220.08 Tm <342E38> Tj 0.96 Tc 1 0 0 1 195.12 206.40 Tm <432D20> Tj 1 0 0 1 205.44 206.40 Tm <6C6C7232527520> Tj 1 0 0 1 297.84 205.68 Tm <332E3220> Tj 1 0 0 1 389.04 205.20 Tm <362E30> Tj 1.20 Tc 1 0 0 1 195.84 191.76 Tm <532D6C6C7232527520> Tj 1 0 0 1 297.84 191.04 Tm <332E3120> Tj 1 0 0 1 388.80 190.80 Tm <352E32> Tj 0.96 Tc 1 0 0 1 203.52 177.12 Tm <532D527520> Tj 1 0 0 1 297.60 176.64 Tm <342E3220> Tj 1 0 0 1 388.80 176.16 Tm <362E38> Tj 0.48 Tc /F3 7.0 Tf 1 0 0 1 139.68 92.40 Tm <4272757A2E696C69616E20> Tj 1 0 0 1 171.84 92.16 Tm <4A6F75726E616C20> Tj 1 0 0 1 199.92 92.16 Tm <6F6C20> Tj 1 0 0 1 208.56 91.92 Tm <4368656EFA63616C20> Tj 1 0 0 1 241.44 91.92 Tm <456E67696E656572696E672C20> Tj 1 0 0 1 286.32 91.44 Tm <566F6C2E32302C20> Tj 1 0 0 1 316.80 91.44 Tm <4E6F2E30332C20> Tj 1 0 0 1 342.72 91.44 Tm <70702E32373320> Tj 1 0 0 1 370.32 92.88 Tm <2D20> Tj 1 0 0 1 374.64 91.20 Tm <3235322C20> Tj 1 0 0 1 392.88 91.20 Tm <2E317531312C2D20> Tj 1 0 0 1 413.76 90.96 Tm <53657074656D62657220> Tj 1 0 0 1 450.00 90.96 Tm <32303033> Tj ET endstream endobj 39 0 obj 11865 endobj 40 0 obj << /Length 41 0 R >> stream / Ir-Ru/AlzOr Catalysts Used in Satellite Propusion Table 2: Results of specific area (Ss), pore volume (Vp), number of sites, and dispersion. Catalyst Sg (m2.g'tlor Vp (cm3.g-t;tzl Sites.g-r (x 1020) Dispersion (%) Shell 405S-IrC-2Irl RuC-lIrlRuS- 1 Irl RuC- llr2RuS- llrlRuS-R.r t14145t34131t34147128 0. 160.410.3'l0.380.390.350.400.39 4.34.61.5l.J1.41.21.31.0 45.849.013.09.2r 0.08.08.95.6 T- -,. - :l:-i. - : .llunr:nr h:.r ,r .pccfc surtce area of I 48 nt:.-::lunrnl fi;r -', rpr':ifc p.rre rountc of 0.-15 cntr Table 3: Distribution of the metal particle diameters of the catah'sts. obtained bv TEN Table 4: Mean of the diameters metal particles of the catalysts, obtained by TBM r-lnr.r=# 2-j1^'=)n,.afS",L/"1 'l Catalyst n(l) Percentage of particle diameters in each range 0-2 2.1- 4 4.1-8 8.r - t2 >12 S-IrC-2Ir1RuC-lIrlRuS-lIrlRuC-lIr2RuS-lIr2RuS-Ru 620741636568330622641 41.3334.2431.6642.'t025.9232.7515.23 46.6645.4345.4840.0844.2044.7041.68 I r.3519.5920.9716.0127.8820.8336.26 0.480.5 r1.65t.2l1.511.725.86 0.180.'230.240.000.490.000.97 I - Nurnber of particles countcd j ltel (nm)(2) S-lr 2.4 4.7C-2Irl Ru 2.8 5.5C- l Irl Ru 2.9 5.4S- llrl Ru 2.'7 4.8C- llr2Ru 3.2 6.0S-llr2Ru 3.1 5.2S-Ru 4.2 6.8 Bruz.ilian Journal ol Chencal Engineering, Vol.20, No.03, pp.273 - 252, .1u11,- September 2003 endstream endobj 41 0 obj 1317 endobj 42 0 obj << /Length 27 >> stream % CANON_PFINF_TYPE0_TEXTON endstream endobj 43 0 obj << /Length 45 >> stream q 595.20 0 0 841.68 0.00 0.00 cm /Obj37 Do Q endstream endobj 44 0 obj << /Type /Page /MediaBox [ 0 0 595.20 841.68 ] /Parent 11 0 R /Resources << /Font << /F3 5 0 R >> /XObject << /Obj37 37 0 R >> /Subtype 40 0 R /ProcSet [ /PDF /Text /ImageB /ImageC /ImageI ] >> /Contents [ 42 0 R 43 0 R 38 0 R ] >> endobj 45 0 obj << /Type /XObject /Subtype /Image /Width 2480 /Height 3507 /BitsPerComponent 1 /ColorSpace /DeviceGray /Filter /CCITTFaxDecode /DecodeParms << /K -1 /Columns 2480 >> /Length 33430 >> stream (PVn00~;vn۰p݇ ۰vnw{n ;vn0p ۆ;vavn݇nnÆ7aېH-pݻ7n÷nÆðᇸar3hexG@0f 1Y婁&D}82(TtI:3Iqhpdl,aa[B[ :V- ;b=lt85VBzCn(!'a,J!n/]yZWI/Ȅtʴ %IZ a">f+7se9ٙtU2!lgaR'˲DKkw8?]0\&ձG_Pp4gU3 .-o׶{loŕ76ᛃU)G}~tl=ǣ5f߿mL,k9֐bkkV@Oipˇ;W:I${sW|u󰙩tMGUyF$7å 6/lo.^>>V3֡U۽ca$ ähcNmnRun$!kcﶽh-geѩ~V{idHIՑ #gLnյ[O &Ici0N!i6.i{1,S (Nwa?vY a(gjio=G|]@q'aD0AAfFFz^^ Cj @aѳXM70pݻ7 8n0vჷ v \p÷n݇n7aۆ8n0w8n0۰pݻܳhQ#+ۖra#NE, BB,W!P:[%dwwȖ am+mm--mxo_M>3Id&G ں('av]o8Î>j`䃃#-MA$<.H]eXdL#[LO>gI3MAAN &"`A( h y313 d|f "6G̜bhg h")Nf oEA"0"isbp.Em]xkEߋnm-F f^MbT5HMa%i6*CA;"7 l- &턓v;}zoE܊i:N_!~?t5ZWB} jEO_{7V xU~5{ޚ|/Eq^M_e>G_'=O>I?6E\o;a7?K*v?_^ݿMOo__h>_oa벬~]߾'>`ᤶv}7yKpmK />^l0V +"[ܡT;ޠxpkQNvI_lSұ : ]MŜҶB5d[SMP@AbilM662-0I5IvM ZMCIg,aaPaN9C$jA; jX b &M5'Lڰ0da;ADDDDDDDDDDDDDDDDDDFDDDDDDDDDDDDDDCqnpܶ 鷃 ;ޛqûwplB>GdY|3 h&]Prsjrpg&糁 r$܈98 P偞re‡0DDDDDDDDDA$[u2̴G;2ޒl+"ζ3 +zʒ[j;*I,PKE!c#Đ .SYAc\f!X~"~VDh"pE2vnH wt22-ȩ j?|*+}a%|%vE{)Xj௿9INޗU׬;MRI醛\WW_o}oO|-]'w#B}jo.1OxW_|\}ץ_z*בKPHf4\tdgz?zk?Fb,wifaN V+V@T9d?'l0JiqI(;E m}GІP@l@{ ):mqRhꏅL l?`eTW K.Vi-<):Aom B_+:0J?ޟy.Z+⫫UHW:#װ$?czc_~^~u/fa/K_oA}ma/b __!Oi*n;T?rm턘ػdUkm/5uo)R(7CNm _m.m(v3 uw2=0L& ֞J¿OO Bz Tb*q%V+""#v"")c,qeWD\DD~eT^ʕrz+h?uVtxI_B>:l6qD?J_r+L1 (/̹vyE;.莍 3#xttE;8]f@fdqHHᤥ""""""""""""""""""""""""""""Al q\el[H[t.qcCfd#@m@Q AA/36 Cb""gaH[?Kn גη0Gpt,a|*620DdåhޓԈ<#S V }'I|;8I/z[!^+WWմگUzx2k_SIqdK ~I3F;=~?x ?{]_?ba,AH?׿uA տ_ץt^A7~JKGx|O\-[ւRt~aJk/_֖d=xnjG%([K :XW^C<ۿo+_ VHMQwoVοblS"+NF'- 4TՍ #˂J{ӃЃ #_J_2q"SΣ$2:3UOM XPl"0#A\!aM7M&ѝxR2#@8K'մul0Fsu+JŴþWi6_Ktޖz}>qNeHCK%([xcU|~;w_5'~{V} uK5g'zL?H_֏nKCo׸~/_?+[MkO_DnWI׶u={-m^Ma&(|ֻOaV Bpa6) (E!A q6/  b&!{XB/H GDDDDDYtg8$AS+Q&P0#eb^d2:d}Az5M#c+#QRtӠOO3oTA=~sւIҽ.VAFS7Rnotq m^^7&KOJld;&`_ۉPZN__vHd8/i:N]!*C OU}O~?Ko/櫥 Gw~ B_F#H iU_IuaKUuޓ]m4^UZMol~NKVj_}1 G: Mu_C,^7bҰIմ^V[K_hP 1LBZb*0a҃ 6O3L6CM\ aT28m1CqDDDDGhZ_ˑ$ƸP@esGF\2A2Te¤a0Fa3\jκ 4e#%{zNoH7 AW:Ma/nool3ͻK'K}{fQ~/_ޤw_ v M t߿/뻻留z[߰[}X29j<>a/@w'auy{7-W]OeBp[$K&=WYZIi??ZF/~~F]ץ~7IksIAaim &Av246 M b H0 cL?pb`f0h2SuDDܷ2CRд幒[/?Bүnd-җ_ndt,ΦTeTB„h #@xA3. fkʈgiMߣaBa#*uIV@G:7z8Vn/j>޿~&K":Ti/Fݞ 3ιg?_%WءPeL6Kb|3Ϗ .N{mOl{׏_IOo_5iAgh}_}qaKK4__VoOWiuߥO#DzW?^?sI(-q0ia`v &od鿿m!h1 &!+"h!PL&쓫M6iŰ=Dq "#@Bt}I[]XcsP8NDFr)r+8NfymE:/Ȏdwx+v[.q"xq@DDDķT Y 4#e‘LFB3t7[Z*20_ &625@NM#_ѲXA\(PIL\L!¨@ $.N5Hy\=$ªXeoC\Ax? 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HE>;Т?q An_7^ɎH?]߿uo_:{VJ5i~ mġ߶i+i no1&M AL0DDDGbAa6+0A%_촌g*3L%(,I S qL?2IѲ҆N\#8`AAZ3zH6$X5 tl Wo%u,iUwZK9%ti> stream BT 3 Tr 0.72 Tc /F3 7.0 Tf 1 0 0 1 207.36 810.72 Tm <542E472E536F6172657320> Tj 1 0 0 1 245.52 810.72 Tm <5C65746F2E20> Tj 1 0 0 1 264.96 810.72 Tm <4A20> Tj 1 0 0 1 270.00 810.72 Tm <472E2E74622C722D46632DCD3A6327EC724A2E2E7B2CCC20> Tj 1 0 0 1 336.72 810.72 Tm <4320> Tj 1 0 0 1 344.40 810.72 Tm <4320> Tj 1 0 0 1 354.24 810.72 Tm <3A20> Tj 1 0 0 1 364.08 810.72 Tm <273A3A20> Tj 1 0 0 1 378.00 810.72 Tm <4320> Tj 1 0 0 1 385.92 810.72 Tm <5CCD20> Tj 1 0 0 1 394.80 810.72 Tm <43723A727A> Tj 0.72 Tc /F3 10.0 Tf 1 0 0 1 160.08 789.36 Tm <5461626C6520> Tj 1 0 0 1 190.08 789.36 Tm <353A20> Tj 1 0 0 1 202.08 789.36 Tm <506572666F726D616E636520> Tj 1 0 0 1 266.88 789.36 Tm <6F6620> Tj 1 0 0 1 278.88 789.36 Tm <63617461682773747320> Tj 1 0 0 1 322.80 789.36 Tm <696E20> Tj 1 0 0 1 334.80 789.36 Tm <325C20> Tj 1 0 0 1 351.12 789.36 Tm <6D6963726F746872757374657220> Tj 1 0 0 1 420.72 789.36 Tm <7465737473> Tj 0.48 Tc /F3 7.0 Tf 1 0 0 1 93.60 269.52 Tm <4920> Tj 1 0 0 1 98.88 271.20 Tm <2D20> Tj 1 0 0 1 103.44 269.52 Tm <48796472617A696E6520> Tj 1 0 0 1 139.20 269.28 Tm <6C696E6520> Tj 1 0 0 1 153.36 269.52 Tm <70726573737572653B20> Tj 1 0 0 1 184.56 269.28 Tm <3220> Tj 1 0 0 1 190.80 270.72 Tm <2D20> Tj 1 0 0 1 195.60 269.28 Tm <496E697469616C20> Tj 1 0 0 1 216.72 269.04 Tm <74656D706572617475726520> Tj 1 0 0 1 257.28 269.04 Tm <696E20> Tj 1 0 0 1 265.68 269.04 Tm <74686520> Tj 1 0 0 1 277.44 268.80 Tm <74687275737465723B20> Tj 1 0 0 1 308.64 268.80 Tm <3320> Tj 1 0 0 1 314.88 270.48 Tm <2D20> Tj 1 0 0 1 319.44 268.80 Tm <46696E616C20> Tj 1 0 0 1 337.92 268.80 Tm <74656D706572617475726520> Tj 1 0 0 1 378.48 268.80 Tm <696E20> Tj 1 0 0 1 386.88 268.80 Tm <74686520> Tj 1 0 0 1 398.88 268.80 Tm <74687275737465723B> Tj 0.48 Tc 1 0 0 1 92.40 258.24 Tm <3420> Tj 1 0 0 1 98.88 259.92 Tm <2D20> Tj 1 0 0 1 103.68 258.24 Tm <537461676E6174696F6E20> Tj 1 0 0 1 140.40 258.24 Tm <707265737375726520> Tj 1 0 0 1 169.44 258.00 Tm <696E20> Tj 1 0 0 1 177.84 258.00 Tm <74686520> Tj 1 0 0 1 189.84 258.00 Tm <6368616D6265723B20> Tj 1 0 0 1 222.24 257.76 Tm <3520> Tj 1 0 0 1 228.24 259.44 Tm <2D20> Tj 1 0 0 1 233.04 257.76 Tm <466972696E6720> Tj 1 0 0 1 254.64 257.76 Tm <726567696D63> Tj 0.48 Tc /F3 10.0 Tf 1 0 0 1 232.08 235.92 Tm <5461626C6520> Tj 1 0 0 1 262.08 235.68 Tm <363A20> Tj 1 0 0 1 273.84 235.92 Tm <4461746120> Tj 1 0 0 1 299.52 235.68 Tm <6F6E20> Tj 1 0 0 1 313.68 235.68 Tm <6C6F737320> Tj 1 0 0 1 334.08 235.68 Tm <6F6620> Tj 1 0 0 1 346.08 235.68 Tm <6D617373> Tj 0.48 Tc /F3 8.0 Tf 1 0 0 1 205.44 214.80 Tm <436174616C767374> Tj 0.48 Tc 1 0 0 1 272.16 214.80 Tm <496E697469616C20> Tj 1 0 0 1 298.08 214.56 Tm <6D61737320> Tj 1 0 0 1 319.20 215.28 Tm <286729> Tj 0.48 Tc 1 0 0 1 348.96 214.56 Tm <4C6F737320> Tj 1 0 0 1 368.88 214.56 Tm <6F6620> Tj 1 0 0 1 378.72 214.56 Tm <6D61737328376F29> Tj 0.72 Tc /F3 9.0 Tf 1 0 0 1 216.00 202.56 Tm <534972> Tj 0.48 Tc 1 0 0 1 205.20 190.08 Tm <43497232527520> Tj 1 0 0 1 233.52 190.32 Tm <49> Tj 0.96 Tc 1 0 0 1 205.20 178.08 Tm <4349726C52756C> Tj 1.20 Tc 1 0 0 1 205.92 165.84 Tm <5349726C527520> Tj 1 0 0 1 233.28 166.08 Tm <49> Tj 0.72 Tc 1 0 0 1 205.20 153.60 Tm <4349726C527532> Tj 0.96 Tc 1 0 0 1 206.16 141.36 Tm <5349726C20> Tj 1 0 0 1 221.52 141.36 Tm <527532> Tj 0.48 Tc 1 0 0 1 213.60 129.36 Tm <535275> Tj 0.72 Tc 1 0 0 1 204.00 117.12 Tm <5368656C6C20> Tj 1 0 0 1 224.64 117.12 Tm <343035> Tj 0.72 Tc 1 0 0 1 286.08 202.08 Tm <302E3631343636> Tj 0.96 Tc 1 0 0 1 286.08 190.08 Tm <302E3620> Tj 1 0 0 1 298.56 190.08 Tm <7220> Tj 1 0 0 1 302.16 189.84 Tm <333839> Tj 0.96 Tc 1 0 0 1 286.08 177.84 Tm <302E3631303536> Tj 0.72 Tc 1 0 0 1 286.08 165.60 Tm <302C3633383036> Tj 0.96 Tc 1 0 0 1 286.08 153.36 Tm <302E3633323332> Tj 0.48 Tc 1 0 0 1 286.08 141.12 Tm <302E3632323431> Tj 0.72 Tc 1 0 0 1 286.08 129.12 Tm <302E3632373234> Tj 0.96 Tc 1 0 0 1 287.04 116.88 Tm <312E3031373132> Tj 0.00 Tc 1 0 0 1 381.60 202.32 Tm <49> Tj 0.00 Tc 1 0 0 1 380.64 189.84 Tm <37> Tj 0.00 Tc 1 0 0 1 380.64 177.84 Tm <6F> Tj 0.00 Tc 1 0 0 1 380.88 165.60 Tm <38> Tj 0.00 Tc 1 0 0 1 380.40 153.36 Tm <34> Tj 0.00 Tc 1 0 0 1 380.88 141.12 Tm <36> Tj 0.00 Tc 1 0 0 1 380.64 128.88 Tm <37> Tj 0.00 Tc 1 0 0 1 381.84 116.64 Tm <37> Tj 0.72 Tc /F3 8.0 Tf 1 0 0 1 94.32 766.80 Tm <436174616C767374> Tj 0.72 Tc /F3 7.0 Tf 1 0 0 1 158.64 766.80 Tm <50492C> Tj 1.20 Tc /F3 8.0 Tf 1 0 0 1 169.44 770.88 Tm <2772293162617229> Tj 0.48 Tc 1 0 0 1 234.24 766.80 Tm <54695020> Tj 1 0 0 1 249.84 771.12 Tm <28277A2920> Tj 1 0 0 1 259.44 765.60 Tm <434329> Tj 1.44 Tc 1 0 0 1 310.56 766.80 Tm <5472502772272827432920> Tj 1 0 0 1 387.60 766.80 Tm <502E20> Tj 1 0 0 1 399.36 770.88 Tm <722C31323120> Tj 1 0 0 1 424.56 768.00 Tm <2C20> Tj 1 0 0 1 464.16 766.56 Tm <526567696D6572> Tj 0.48 Tc 1 0 0 1 93.12 730.56 Tm <5368656C6C20> Tj 1 0 0 1 113.52 730.56 Tm <343035> Tj 0.48 Tc /F3 10.0 Tf 1 0 0 1 170.64 754.56 Tm <32312E2737> Tj 0.24 Tc 1 0 0 1 170.64 742.56 Tm <32302E36> Tj 0.24 Tc 1 0 0 1 170.64 730.56 Tm <32302E30> Tj 1.20 Tc 1 0 0 1 171.36 718.80 Tm <72392E39> Tj 1.20 Tc 1 0 0 1 171.36 706.80 Tm <31392E30> Tj 0.00 Tc 1 0 0 1 248.88 754.32 Tm <313032> Tj 0.96 Tc 1 0 0 1 248.88 742.56 Tm <723030> Tj 1.20 Tc /F3 8.0 Tf 1 0 0 1 249.84 732.48 Tm <6F65> Tj 0.96 Tc 1 0 0 1 249.84 718.56 Tm <3936> Tj 0.96 Tc 1 0 0 1 249.84 706.56 Tm <3935> Tj 1.20 Tc /F3 9.0 Tf 1 0 0 1 324.00 754.08 Tm <383330> Tj 0.96 Tc 1 0 0 1 323.76 742.32 Tm <383330> Tj 0.96 Tc 1 0 0 1 323.76 730.32 Tm <383330> Tj 0.96 Tc 1 0 0 1 323.76 718.32 Tm <383330> Tj 0.96 Tc 1 0 0 1 323.76 706.32 Tm <383330> Tj 0.96 Tc /F3 8.0 Tf 1 0 0 1 399.84 754.32 Tm <2E20> Tj 1 0 0 1 403.44 754.32 Tm <2D3A20> Tj 1 0 0 1 410.16 755.28 Tm <4920> Tj 1 0 0 1 462.00 754.32 Tm <43692C6E74696E756F7573> Tj 0.96 Tc 1 0 0 1 399.84 742.56 Tm <3120> Tj 1 0 0 1 403.44 742.56 Tm <2D3A2ECC20> Tj 1 0 0 1 413.04 743.28 Tm <6920> Tj 1 0 0 1 471.12 744.72 Tm <7075EC2E2E5F4A> Tj 1.20 Tc 1 0 0 1 399.60 730.32 Tm <49312E3020> Tj 1 0 0 1 471.12 730.32 Tm <5075EC3A2E2D4A> Tj 1.20 Tc 1 0 0 1 399.60 718.56 Tm <6920> Tj 1 0 0 1 404.16 718.56 Tm <312E3920> Tj 1 0 0 1 470.88 718.32 Tm <5075CC73654A> Tj 0.96 Tc 1 0 0 1 399.60 706.56 Tm <4920> Tj 1 0 0 1 404.16 706.56 Tm <312E3820> Tj 1 0 0 1 462.00 706.32 Tm <437472CCEC6CEC6C6C557272FC3A> Tj 0.72 Tc 1 0 0 1 104.88 670.32 Tm <534972> Tj 0.72 Tc /F3 9.0 Tf 1 0 0 1 170.64 694.08 Tm <32312E38> Tj 1.20 Tc 1 0 0 1 170.40 682.32 Tm <32322E31> Tj 0.72 Tc 1 0 0 1 170.64 670.08 Tm <32312E35> Tj 0.72 Tc 1 0 0 1 170.64 658.32 Tm <32312E30> Tj 0.24 Tc 1 0 0 1 170.64 646.32 Tm <32302E35> Tj 0.72 Tc 1 0 0 1 252.24 694.08 Tm <3032> Tj 0.48 Tc 1 0 0 1 252.00 682.08 Tm <3035> Tj 1.50 Tc 1 0 0 1 253.20 670.08 Tm <6C36> Tj 0.72 Tc 1 0 0 1 252.00 658.08 Tm <3030> Tj 0.96 Tc 1 0 0 1 251.76 646.08 Tm Tj 0.48 Tc 1 0 0 1 323.76 693.84 Tm <37277430> Tj 0.48 Tc 1 0 0 1 323.76 681.84 Tm <37273730> Tj 0.72 Tc 1 0 0 1 323.76 669.84 Tm <373630> Tj 0.96 Tc 1 0 0 1 323.76 658.08 Tm <373530> Tj 0.72 Tc 1 0 0 1 323.76 645.84 Tm <373330> Tj 0.96 Tc 1 0 0 1 402.96 694.08 Tm <342E30> Tj 0.48 Tc 1 0 0 1 402.96 682.08 Tm <342E2D6C> Tj 0.96 Tc 1 0 0 1 402.96 670.08 Tm <342E35> Tj 0.96 Tc 1 0 0 1 402.96 658.08 Tm <342E30> Tj 1.20 Tc 1 0 0 1 403.20 646.08 Tm <332E38> Tj 0.96 Tc /F3 8.0 Tf 1 0 0 1 462.00 693.84 Tm <436F6E74696E757472753A> Tj 0.96 Tc 1 0 0 1 470.88 682.08 Tm <5075CC736564> Tj 0.72 Tc 1 0 0 1 470.88 669.84 Tm <50756C736564> Tj 0.72 Tc 1 0 0 1 470.64 658.08 Tm <50756C736564> Tj 0.72 Tc 1 0 0 1 461.76 646.08 Tm <436F6E74696E756F7573> Tj 0.96 Tc /F3 9.0 Tf 1 0 0 1 94.08 609.60 Tm <433249726C5275> Tj 0.24 Tc 1 0 0 1 170.64 633.60 Tm <32302E39> Tj 0.48 Tc 1 0 0 1 170.64 621.84 Tm <32302E35> Tj 0.72 Tc 1 0 0 1 170.40 609.60 Tm <32302E30> Tj 0.72 Tc 1 0 0 1 171.36 597.60 Tm <31392E36> Tj 1.20 Tc 1 0 0 1 171.12 585.60 Tm <7220> Tj 1 0 0 1 174.72 585.36 Tm <392E33> Tj 0.48 Tc 1 0 0 1 252.24 633.60 Tm <3230> Tj 1.50 Tc 1 0 0 1 253.20 621.60 Tm <7437> Tj 1.50 Tc 1 0 0 1 252.24 609.36 Tm <326C> Tj 1.50 Tc 1 0 0 1 252.96 597.36 Tm <3137> Tj 0.72 Tc 1 0 0 1 251.76 585.36 Tm Tj 0.96 Tc 1 0 0 1 323.52 633.36 Tm <373530> Tj 1.44 Tc 1 0 0 1 323.52 621.36 Tm <373135> Tj 1.44 Tc 1 0 0 1 323.52 609.12 Tm <373135> Tj 1.50 Tc 1 0 0 1 323.52 597.12 Tm <377230> Tj 0.24 Tc 1 0 0 1 324.24 585.12 Tm <363935> Tj 1.20 Tc 1 0 0 1 403.20 633.36 Tm <332E39> Tj 0.96 Tc 1 0 0 1 402.96 621.60 Tm <342E30> Tj 1.20 Tc 1 0 0 1 403.20 609.12 Tm <332E39> Tj 0.96 Tc 1 0 0 1 403.20 597.12 Tm <332E34> Tj 0.96 Tc 1 0 0 1 403.20 585.36 Tm <322E39> Tj 0.72 Tc /F3 8.0 Tf 1 0 0 1 461.76 633.36 Tm <436F6E74696E756F7573> Tj 0.48 Tc 1 0 0 1 470.64 621.60 Tm <50756C736564> Tj 0.48 Tc 1 0 0 1 470.64 609.36 Tm <50756C736564> Tj 0.48 Tc 1 0 0 1 470.64 597.36 Tm <50756C736564> Tj 0.72 Tc 1 0 0 1 461.76 585.36 Tm <436F6E74696E756F7573> Tj 1.20 Tc 1 0 0 1 94.08 549.12 Tm <436C49726C5275> Tj 1.50 Tc /F3 9.0 Tf 1 0 0 1 170.40 572.88 Tm <32312E36> Tj 0.24 Tc 1 0 0 1 170.64 560.88 Tm <32302E35> Tj 1.44 Tc 1 0 0 1 171.36 548.88 Tm <31392E35> Tj 1.44 Tc 1 0 0 1 171.36 536.88 Tm <31382E37> Tj 1.20 Tc 1 0 0 1 171.36 524.64 Tm <31392E39> Tj 1.50 Tc 1 0 0 1 253.20 572.64 Tm <6C33> Tj 0.72 Tc 1 0 0 1 252.00 560.88 Tm <3035> Tj 0.00 Tc 1 0 0 1 253.20 548.88 Tm <696C> Tj 1.50 Tc /F3 5.0 Tf 1 0 0 1 253.20 539.04 Tm <31C1> Tj 0.72 Tc /F3 10.0 Tf 1 0 0 1 252.00 524.40 Tm <3030> Tj 0.72 Tc /F3 9.0 Tf 1 0 0 1 323.52 572.40 Tm <373334> Tj 0.24 Tc 1 0 0 1 324.24 560.64 Tm <363935> Tj 0.96 Tc 1 0 0 1 323.76 548.64 Tm <363835> Tj 0.48 Tc 1 0 0 1 323.76 536.40 Tm <36277435> Tj 0.48 Tc 1 0 0 1 324.24 524.40 Tm <36273135> Tj 0.96 Tc 1 0 0 1 402.96 572.64 Tm <342E30> Tj 1.20 Tc 1 0 0 1 403.20 560.64 Tm <332E35> Tj 1.20 Tc 1 0 0 1 403.20 548.64 Tm <332E34> Tj 0.96 Tc 1 0 0 1 403.20 536.64 Tm <322E38> Tj 1.20 Tc 1 0 0 1 403.20 524.40 Tm <332E35> Tj 0.72 Tc /F3 8.0 Tf 1 0 0 1 461.76 572.64 Tm <436F6E74696E756F7573> Tj 0.48 Tc 1 0 0 1 470.88 560.88 Tm <50756C736564> Tj 0.48 Tc 1 0 0 1 470.88 548.88 Tm <50756C736564> Tj 0.48 Tc 1 0 0 1 470.88 536.64 Tm <50756C736564> Tj 0.72 Tc 1 0 0 1 461.76 524.40 Tm <436F6E74696E756F7573> Tj 0.96 Tc 1 0 0 1 95.04 488.16 Tm <5320> Tj 1 0 0 1 100.80 488.16 Tm <6C49726C20> Tj 1 0 0 1 114.96 488.16 Tm <5275> Tj 0.72 Tc /F3 9.0 Tf 1 0 0 1 170.40 512.16 Tm <32312E33> Tj 0.24 Tc 1 0 0 1 170.64 500.16 Tm <32302E36> Tj 0.72 Tc 1 0 0 1 170.40 488.16 Tm <32302E38> Tj 0.72 Tc 1 0 0 1 170.40 475.92 Tm <32302E30> Tj 0.72 Tc 1 0 0 1 171.36 464.16 Tm <31392E34> Tj 0.00 Tc 1 0 0 1 256.80 511.92 Tm <35> Tj 0.00 Tc 1 0 0 1 256.80 499.92 Tm <37> Tj 0.00 Tc 1 0 0 1 256.80 487.92 Tm <35> Tj 0.00 Tc 1 0 0 1 256.80 475.92 Tm Tj 0.00 Tc 1 0 0 1 256.80 463.92 Tm <5F35> Tj 0.72 Tc 1 0 0 1 323.52 516.48 Tm <272F3335> Tj 0.72 Tc 1 0 0 1 323.76 499.68 Tm <363830> Tj 0.48 Tc 1 0 0 1 324.24 487.68 Tm <36273735> Tj 0.48 Tc 1 0 0 1 324.24 475.68 Tm <36273130> Tj 0.96 Tc 1 0 0 1 323.76 463.92 Tm <363730> Tj 1.20 Tc 1 0 0 1 403.20 511.92 Tm <332E38> Tj 0.96 Tc 1 0 0 1 402.96 499.92 Tm <342E30> Tj 1.44 Tc 1 0 0 1 403.20 487.92 Tm <332E39> Tj 1.44 Tc 1 0 0 1 403.20 475.68 Tm <332E36> Tj 1.50 Tc 1 0 0 1 403.20 463.92 Tm <332E31> Tj 0.72 Tc /F3 8.0 Tf 1 0 0 1 461.76 511.92 Tm <436F6E74696E756F7573> Tj 0.72 Tc 1 0 0 1 470.88 499.92 Tm <50756C736564> Tj 0.48 Tc 1 0 0 1 470.88 487.92 Tm <50756C736564> Tj 0.48 Tc 1 0 0 1 470.64 475.92 Tm <50756C736564> Tj 0.72 Tc 1 0 0 1 461.76 463.92 Tm <436F6E74696E756F7573> Tj 0.72 Tc 1 0 0 1 94.32 427.92 Tm <436C20> Tj 1 0 0 1 105.12 427.92 Tm <4972325275> Tj 1.50 Tc /F3 9.0 Tf 1 0 0 1 170.64 451.44 Tm <325C2E36> Tj 0.96 Tc 1 0 0 1 170.40 439.44 Tm <32302E38> Tj 0.72 Tc 1 0 0 1 170.40 427.68 Tm <32302E30> Tj 0.96 Tc 1 0 0 1 170.64 415.68 Tm <32312E33> Tj 0.24 Tc 1 0 0 1 170.64 403.68 Tm <32302E35> Tj 1.50 Tc 1 0 0 1 253.20 451.44 Tm <6C39> Tj 1.50 Tc 1 0 0 1 253.20 439.44 Tm <7432> Tj 1.50 Tc 1 0 0 1 253.20 427.68 Tm <6C35> Tj 1.50 Tc /F3 5.0 Tf 1 0 0 1 253.44 417.84 Tm <6C5E> Tj 0.48 Tc /F3 9.0 Tf 1 0 0 1 252.00 403.44 Tm <3034> Tj 0.00 Tc 1 0 0 1 323.52 456.24 Tm <2D373130> Tj 0.72 Tc 1 0 0 1 323.76 439.20 Tm <363830> Tj 0.00 Tc 1 0 0 1 324.24 427.44 Tm <362D3735> Tj 0.72 Tc 1 0 0 1 323.76 415.44 Tm <363735> Tj 0.72 Tc 1 0 0 1 323.76 403.20 Tm <363735> Tj 1.20 Tc 1 0 0 1 403.20 451.20 Tm <332E39> Tj 0.96 Tc 1 0 0 1 402.96 439.44 Tm <342E39> Tj 1.20 Tc 1 0 0 1 403.20 427.44 Tm <332E34> Tj 1.20 Tc 1 0 0 1 403.20 415.44 Tm <332E39> Tj 1.20 Tc 1 0 0 1 403.20 403.44 Tm <332E39> Tj 0.72 Tc 1 0 0 1 461.76 451.20 Tm <436F6E74696E756F7573> Tj 0.72 Tc 1 0 0 1 470.64 439.44 Tm <50756C736564> Tj 0.48 Tc 1 0 0 1 470.88 427.68 Tm <50756C736564> Tj 0.72 Tc 1 0 0 1 470.88 415.44 Tm <50756C736564> Tj 0.72 Tc 1 0 0 1 461.76 403.44 Tm <436F6E74696E756F7573> Tj 0.72 Tc 1 0 0 1 95.04 366.96 Tm <5320> Tj 1 0 0 1 100.80 366.96 Tm <316C72325275> Tj 1.44 Tc 1 0 0 1 170.40 390.96 Tm <32742E39> Tj 0.96 Tc 1 0 0 1 170.64 378.72 Tm <32312E32> Tj 0.24 Tc 1 0 0 1 170.40 366.96 Tm <32302E36> Tj 1.20 Tc 1 0 0 1 170.40 354.72 Tm <32302E31> Tj 1.20 Tc 1 0 0 1 171.36 342.96 Tm <31392E35> Tj 0.72 Tc 1 0 0 1 252.24 390.96 Tm <3236> Tj 1.50 Tc 1 0 0 1 253.20 378.72 Tm <6C38> Tj 0.72 Tc 1 0 0 1 252.24 366.72 Tm <3232> Tj 1.50 Tc 1 0 0 1 252.24 354.72 Tm <326C> Tj 1.50 Tc 1 0 0 1 253.20 342.72 Tm <6C30> Tj 0.72 Tc 1 0 0 1 323.52 390.72 Tm <373330> Tj 0.72 Tc 1 0 0 1 323.52 378.48 Tm <363630> Tj 0.96 Tc 1 0 0 1 323.52 366.48 Tm <363530> Tj 0.24 Tc 1 0 0 1 324.24 354.48 Tm <363435> Tj 0.96 Tc 1 0 0 1 323.76 342.48 Tm <363335> Tj 1.50 Tc /F3 10.0 Tf 1 0 0 1 403.44 381.36 Tm Tj 0.96 Tc /F3 8.0 Tf 1 0 0 1 402.96 366.72 Tm <342E34> Tj 1.20 Tc 1 0 0 1 403.20 354.48 Tm <332E39> Tj 0.72 Tc 1 0 0 1 461.76 390.72 Tm <436F6E74696E756F7573> Tj 0.48 Tc 1 0 0 1 470.64 378.72 Tm <5075CC736564> Tj 0.48 Tc 1 0 0 1 470.64 366.72 Tm <5075CC736564> Tj 0.72 Tc 1 0 0 1 470.88 354.48 Tm <5075EC736564> Tj 0.48 Tc 1 0 0 1 461.76 342.72 Tm <436F6E74696E756F7573> Tj 0.48 Tc /F3 9.0 Tf 1 0 0 1 102.48 306.48 Tm <535275> Tj 0.00 Tc 1 0 0 1 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Tc 1 0 0 1 402.96 306.24 Tm <342E36> Tj 0.96 Tc 1 0 0 1 402.96 294.00 Tm <342E36> Tj 0.96 Tc 1 0 0 1 402.96 281.76 Tm <342E36> Tj 0.72 Tc 1 0 0 1 461.76 330.00 Tm <436F6E74696E756F7573> Tj 0.72 Tc 1 0 0 1 470.64 318.00 Tm <50756C736564> Tj 0.72 Tc 1 0 0 1 470.64 306.24 Tm <50756C736564> Tj 0.72 Tc 1 0 0 1 470.64 294.00 Tm <50756C736564> Tj 0.72 Tc 1 0 0 1 461.76 281.76 Tm <436F6E74696E756F7573> Tj 0.24 Tc /F3 7.0 Tf 1 0 0 1 229.68 89.76 Tm <4272757A694969616E20> Tj 1 0 0 1 262.08 89.52 Tm <4A6F75726E616C20> Tj 1 0 0 1 289.68 89.52 Tm <6F6C20> Tj 1 0 0 1 298.32 89.28 Tm <4368656D6963616C20> Tj 1 0 0 1 331.20 89.52 Tm <456E67696E656572696E67> Tj ET endstream endobj 47 0 obj 15554 endobj 48 0 obj << /Length 49 0 R >> stream T.G.Soares \eto. J G..tb,r-Fc-:c'rJ..{, C C : ':: C \ Cr:rzTable 5: Performance of catah'sts in 2\ microthruster tests I - Hydrazine line pressure; 2 - Initial temperature in the thruster; 3 - Final temperature in the thruster;4 - Stagnation pressure in the chamber; 5 - Firing regimcTable 6: Data on loss of mass Catalvst Initial mass (g) Loss of mass(7o) SIrCIr2Ru ICIrlRulSIrlRu ICIrlRu2SIrl Ru2SRuShell 405 0.614660.6 r 3890.610560,638060.632320.622410.627241.01712 I7o84677 Catalvst PI, 'r)1bar) TiP ('z) CC) TrP'r'('C) P. r,121 , Regimer Shell 405 21.'720.620.0r9.919.0 102r00oe9695 830830830830830 . -: I Ci,ntinuous1 -:. i pu.._JI1.0 Pu:.-Ji 1.9 PuseJI 1.8 CtrlllUrr: SIr 21.822.121.521.020.5 0205l6009 7't07'70760750730 4.04.-l4.54.03.8 Continutru:PusedPulsedPulsedContinuous C2IrlRu 20.920.520.019.6r 9.3 20t72l179 7507157157r0695 3.94.03.93.42.9 ContinuousPulsedPulsedPulsedContinuous ClIrlRu 21.620.519.518.719.9 l305il100 7346956856't56'15 4.03.53.42.83.5 ContinuousPulsedPulsedPulsedContinuous S lIrl Ru 21.320.620.820.019.4 575_5 '/356806'756'10670 3.84.03.93.63.1 ContinuousPulsedPulsedPulsedContinuous Cl Ir2Ru 2\.620.820.021.320.5 l9t2l5l^04 -7106806-75675675 3.94.93.43.93.9 ContinuousPulsedPulsedPulsedContinuous S 1lr2Ru 2t.921.220.620.119.5 26l8222ll0 730660650645635 4.43.9 ContinuousPusedPusedPusedContinuous SRu 22222 55555 202422z308 '7357t0't10-7 t0645 4.4.64.64.64.6 ContinuousPulsedPulsedPulsedContinuous BruziIian Journal ol Chemical Engineering endstream endobj 49 0 obj 1499 endobj 50 0 obj << /Length 27 >> stream % CANON_PFINF_TYPE0_TEXTON endstream endobj 51 0 obj << /Length 45 >> stream q 595.20 0 0 841.68 0.00 0.00 cm /Obj45 Do Q endstream endobj 52 0 obj << /Type /Page /MediaBox [ 0 0 595.20 841.68 ] /Parent 11 0 R /Resources << /Font << /F3 5 0 R >> /XObject << /Obj45 45 0 R >> /Subtype 48 0 R /ProcSet [ /PDF /Text /ImageB /ImageC /ImageI ] >> /Contents [ 50 0 R 51 0 R 46 0 R ] >> endobj 53 0 obj << /Type /XObject /Subtype /Image /Width 2480 /Height 3507 /BitsPerComponent 1 /ColorSpace /DeviceGray /Filter /CCITTFaxDecode /DecodeParms << /K -1 /Columns 2480 >> /Length 95310 >> stream &CaeWXr@ R)*dEGkYޏUn|E;fd,ȸpUߺ vqMhv#Lgw]+.ۈޏWi9r ym'iG]wyGF/?^N}?}YJ$ fpgߙ f'^f'^NwA  4 T".83r8͞|g#A~ O}>SL('kIqvv ߅a#!kh[^ymoWuL^;I]/οQU B SZ>߮1v`jﷰlWC/%huoVG};}m?* =8 oapoQժ_~z*Kz׷y>y=v}նfommm/ja.vuX Q['jf8_ɏ+yjY*y#'GHp_]W_vGCAs# )D!D5-WUUWDtHBD F>| 29 CA!͑Г#E d%>ׯҴTuz  B ~m L&S3FG3dpS06mZy䖫21*?6A0x~aBg> vѱ਌xFႄ"d9 @aH4 7'FfGH9&tvHdkdueZ(G׏mCMZMI\4pġOO4aPNX* &8 L#@`e0Fa0L dC36H#A1ȇA>GN!i#D^:90L?o~ރ~w_~x:M4tJI6 ?%9Z .I|lSEsH8(P!0a 6{ *`0ࠩh!*0Apl hz_Z_w7ZOҴ%e%<7Jؔ%nA[TR FYӪMbT4@j:?2w[qZWI齡?OCMBAblz_oa:LNacK ~??ӯդwO^TxOokwPZ]!_Oix=ujiA #G/=y?_HGKmׄA~#G\=~E~":_wkK AA #qapD~Io/׶E U!AWI/nߥ_~!mC_d5_a^~{޿V/UZ[AI!n~ߥvKa-mSO_y zuY LJjمtB4/v/oۧ^׺?o[$/l~8f 6j(0J Iڰ{ f;/`_wkޗj_w[qtAA Z SȱM6*ðb1(p a2?eҵnJKKimiZ_VMQȈ`(BN0&M4 ӆ iĨa;bK/$مjYOaUk_il0K];`  0M=L BM0 5 4 '^INFA]ġJvT:dx+"ȶ*`aY+[K"""""""""!iS 1 0AaMBAL MMR 0A4ӥM vLOwIP ]]A'\DDD!ESB 0 0DbAp 4T $X DtGA"<0TP &l EV($GHҥ%JBI{  aV!X(n/+2Z3\C a_󲾮mpx`wKM+AW&2Z2;XNph2AALd;3x E<0j/~_h> ;KLMgn>A R_uZ2B G#S:#pLiYȿz?߮ B ¦i "; 0G ՝̝Q]W_-S& *  GnDqAB$  # 2dTO |ƈJ=h6nL&v&շ I6 %_A6]{@gGGZ`P ̾8GB dC&G0T0L#cG>|&*!  ##C´BD|`aP 0D!0A, hD#@YVI[ l1)t{huu~'xH6zAj6Am 47Q':~h#[M= v'B5 CWcVoҿhv!?_ m6r}&%m' ";8)ƓlJzI6 3߼JaKy84_k>?T|}ǾǮumVnm-L'hRohj~j%opDu~]oZMKK]]p_ ~vïDZoa{_ #GhwY| nComR5/_п~^_tB# a0?ދQamfOG$Dt[KP]w[u!g0Ib!/K 8Du;auAm6!!on?ۮ"?ڄ_Vv$%'Oaj׆~K ?/m/_l-׽o$.&_I-V $ 6{ip/'8b$-i diw!#+IZa؃^)m%akl0`yZokk!xh6)iȰ a!+( Ed /K$?3W]MV_k]?k. aWa  AUDæUb[l a]u .i:_k~X""! @aSAH>)0M4NU0Lz=l{ik{{ CO ^ڰ^مէZDDDDDR(E2 a 6&)zvJ [ 6a&AZL/bViLN=C]pd[{DDDDDHh0 61 B iUNA46A\Gm& Tҧ ĈP6B"""""""80T""B a0hR Fd 0֩""8@b@,i+m!yؘaWQi:1+2v,ȧ0RvA>;v 76PPPAGf\Z=;wF Eѐռv. ;Wlt֖u8]uZ_*<+־\"++hF fEEz~릾`AG<͊h"!<k&I fjNȢO__T4|n7F$: &hZA\ "EXE(I!)͙ԉ$kkgN}$V&p`ɫ,>6LƍL#8a-0a%s/F=02@CY%"/^V6 'IVRm]'`AwAt `n|aikk*giL!Q $ N"8Gf͌: s"KAg522H%8շK[zm&k+I=;ҺJƐo&zQI&A0AQðZhB` L#@aN (O h (Pl#c0?_M׾Э{:MZN6&oQ*! bxjīkh ĨmlJe*A7Inѻ>_V_֟Y+7Mpbt;A;ON^t' eV/_;ƵVڭ-&n _Ngn}CBa__{ttނ з0aB!f TZm^5w_7l?q޿F?0k̬ۙ?ڥ۶NH$&5Ka_\ ZH y ?K?KJ ׷^_{~q>HFo86;$+_Z턾Ikum~Ҷo܈O~[ 5JﶗL%LN6K.W+_6]rwB~a$i[P%Em%I\]ͦ / tUnm*v]j٥__դןOk$ &a4l*am&Zl0jԋԊ2_#wiua^iV/a݄pDDCІL)\RM0 iPa&jIPdWvᴚv)Ea?{iZم{ *V .Նa[S:"""""""""PxƂ #a&  ]pM8WmCzġ[Zm%Y-n\S}1L0X &MMPp B4 M;aRiih4J )4LW B0qL0M0m 4APֈ0 %h(HD$I}݂` >dA$ѝGcjUD&N UYnSdv"AApuaȰЩwVGGe9٥-cT^:A|BfB  vpᄡ=I$^}~uzO琏qK"% %Y]m&CDSiz:f( @ z!(Fa?&=I{5 J!莈ִ0VOzaF Ba&!G#9"A"L-"~LFζpīAgig>nT?0l2 >QIVfD'͟"2FY!A݄}&LJĬi6ħ{2& 0ep 6м{M#50l!lji>3431IEAIIH#T:d}2:͙ЊtIQlˣ!&_5 WOtWˢ|&hA?DpT<6pkg=x `4Bs0F<&aBdrDxB  b0AhakWOMxN/K[Ko%c'bTuT4 Yat J hgIYlaT88eG0&6'_xjN~MPVpl?Vn6 t_Ĭӆ%Gm[ J'+AbVw?]y,+o[Wz}龞IkN~FаH7&W_J?m]'[oW]q_ C#k__ g{~_8qq{87i*/l P}a?h_@mYc+oɎH[0l oo_Gê_z_/KH7. ۯ_Kܑ k 7UK/na o߫i?kӽ.HKoo}_/6ikkd4ֿ  —K 6 [Tdi}%B֞ !_5{ثbSa!. 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192.24 709.68 Tm <636174616C7973747320> Tj 1 0 0 1 239.04 709.68 Tm <6F6E6C7920> Tj 1 0 0 1 267.12 709.68 Tm <7768656E> Tj 0.48 Tc 1 0 0 1 54.24 698.16 Tm <6465636F6D706F736974696F6E20> Tj 1 0 0 1 122.88 698.16 Tm <697320> Tj 1 0 0 1 133.92 697.92 Tm <7374617274656420> Tj 1 0 0 1 166.80 697.92 Tm <617420> Tj 1 0 0 1 178.32 697.92 Tm <616D6269656E7420> Tj 1 0 0 1 217.20 697.68 Tm <74656D706572617475726520> Tj 1 0 0 1 273.60 698.16 Tm <28746865> Tj 0.48 Tc 1 0 0 1 54.48 686.16 Tm <736F2D63616C6C656420> Tj 1 0 0 1 97.68 687.36 Tm <22636F6C6420> Tj 1 0 0 1 125.04 686.16 Tm <73746172747322292E20> Tj 1 0 0 1 163.44 686.16 Tm <496E20> Tj 1 0 0 1 175.68 685.92 Tm <7468697320> Tj 1 0 0 1 195.12 685.92 Tm <636173652C20> Tj 1 0 0 1 220.56 685.92 Tm <49726C416C324F3320> Tj 1 0 0 1 259.20 685.92 Tm <68617320> Tj 1 0 0 1 277.20 685.92 Tm <746865> Tj 0.48 Tc 1 0 0 1 54.48 674.16 Tm <73686F727465737420> Tj 1 0 0 1 95.52 674.16 Tm <64656C61792E20> Tj 1 0 0 1 129.12 674.16 Tm <417320> Tj 1 0 0 1 148.32 674.16 Tm <74686520> Tj 1 0 0 1 168.72 674.40 Tm <706572666F726D616E63657320> Tj 1 0 0 1 236.16 674.16 Tm <6F6620> Tj 1 0 0 1 252.00 674.16 Tm <74686520> Tj 1 0 0 1 272.40 674.16 Tm <6E6577> Tj 0.48 Tc 1 0 0 1 54.24 662.40 Tm <636174616C7973747320> Tj 1 0 0 1 96.96 662.64 Tm <7765726520> Tj 1 0 0 1 122.88 662.40 Tm <6E6F7420> Tj 1 0 0 1 141.60 662.40 Tm <6B6E6F776E20> Tj 1 0 0 1 176.64 662.40 Tm <6120> Tj 1 0 0 1 185.76 662.64 Tm <7072696F72692C20> Tj 1 0 0 1 217.92 662.40 Tm <636F6C6420> Tj 1 0 0 1 241.68 662.40 Tm <73746172747320> Tj 1 0 0 1 269.52 662.40 Tm <77657265> Tj 0.72 Tc 1 0 0 1 54.24 650.88 Tm <6E6F7420> Tj 1 0 0 1 73.20 650.88 Tm <7374756469656420> Tj 1 0 0 1 109.68 650.88 Tm <696E20> Tj 1 0 0 1 122.64 650.64 Tm <7468697320> Tj 1 0 0 1 143.52 650.88 Tm <776F726B20> Tj 1 0 0 1 170.64 650.64 Tm <746F20> Tj 1 0 0 1 183.84 650.64 Tm <61766F696420> Tj 1 0 0 1 212.88 650.64 Tm <74686520> Tj 1 0 0 1 230.88 650.88 Tm <706F73736962696C69747920> Tj 1 0 0 1 281.76 650.64 Tm <6F66> Tj 0.72 Tc 1 0 0 1 54.48 638.88 Tm <496F6E6720> Tj 1 0 0 1 77.52 638.88 Tm <692D656E6974696F6E20> Tj 1 0 0 1 114.72 638.88 Tm <64656C6179732C20> Tj 1 0 0 1 149.52 639.12 Tm <776869636820> Tj 1 0 0 1 179.52 638.88 Tm <636F756C6420> Tj 1 0 0 1 207.60 638.88 Tm <726573756C7420> Tj 1 0 0 1 235.68 638.88 Tm <696E20> Tj 1 0 0 1 247.44 638.88 Tm <68796472617A696E65> Tj 0.72 Tc 1 0 0 1 54.48 626.88 Tm <616363756D756C6174696F6E20> Tj 1 0 0 1 119.52 626.88 Tm <696E20> Tj 1 0 0 1 132.96 626.88 Tm <74686520> Tj 1 0 0 1 151.68 626.88 Tm <6265642C20> Tj 1 0 0 1 175.68 626.88 Tm <666F6C6C6F77656420> Tj 1 0 0 1 220.32 626.88 Tm <627920> Tj 1 0 0 1 236.40 626.88 Tm <6120> Tj 1 0 0 1 246.24 627.12 Tm <68617A6172646F7573> Tj 0.96 Tc 1 0 0 1 54.48 614.88 Tm <726F755F656820> Tj 1 0 0 1 85.92 615.12 Tm <696E6974696174696F6E2E20> Tj 1 0 0 1 134.88 615.36 Tm <72696869636820> Tj 1 0 0 1 167.52 614.88 Tm <636F756C6420> Tj 1 0 0 1 198.00 614.88 Tm <64616D61676520> Tj 1 0 0 1 237.84 615.12 Tm <74686520> Tj 1 0 0 1 257.04 615.12 Tm <7468727573746572> Tj 1.20 Tc 1 0 0 1 54.48 602.88 Tm <616E6420> Tj 1 0 0 1 73.44 603.12 Tm <726E65613A757263726E636E7420> Tj 1 0 0 1 135.12 602.88 Tm <64655C20> Tj 1 0 0 1 151.44 603.12 Tm <6963632E2E> Tj 0.96 Tc 1 0 0 1 68.64 591.12 Tm <46696775726520> Tj 1 0 0 1 100.56 591.36 Tm <4920> Tj 1 0 0 1 108.72 591.12 Tm <73686F72697320> Tj 1 0 0 1 139.20 591.36 Tm <74686520> Tj 1 0 0 1 155.52 591.36 Tm <2E277263656C6C656E7420> Tj 1 0 0 1 198.96 591.36 Tm <73746162726C72746C20> Tj 1 0 0 1 237.36 591.36 Tm <6F6620> Tj 1 0 0 1 249.36 591.36 Tm <5368656C6C20> Tj 1 0 0 1 274.56 593.28 Tm <2D313035> Tj 0.96 Tc 1 0 0 1 54.48 579.12 Tm <666F7220> Tj 1 0 0 1 71.52 579.12 Tm <616C6C20> Tj 1 0 0 1 86.40 579.12 Tm <74686520> Tj 1 0 0 1 103.92 579.36 Tm <706172616D657465723A20> Tj 1 0 0 1 156.96 579.12 Tm <3A7475646965642E20> Tj 1 0 0 1 195.36 579.36 Tm <54686520> Tj 1 0 0 1 216.96 579.36 Tm <73CC6967687420> Tj 1 0 0 1 245.04 579.36 Tm <62757420> Tj 1 0 0 1 263.28 579.36 Tm <737465616476> Tj 0.96 Tc 1 0 0 1 54.72 567.12 Tm <66616C6C20> Tj 1 0 0 1 73.20 567.36 Tm <696E20> Tj 1 0 0 1 85.20 567.36 Tm <74686520> Tj 1 0 0 1 102.48 567.60 Tm <707265737375726520> Tj 1 0 0 1 143.04 567.36 Tm <637572766520> Tj 1 0 0 1 171.60 567.36 Tm <693A20> Tj 1 0 0 1 182.16 567.36 Tm <64756520> Tj 1 0 0 1 201.84 567.36 Tm <746F20> Tj 1 0 0 1 213.84 567.36 Tm <74686520> Tj 1 0 0 1 230.88 567.60 Tm <636C617373746320> Tj 1 0 0 1 264.00 567.84 Tm <7069657A6F2D> Tj 0.96 Tc 1 0 0 1 54.72 555.36 Tm <656C65637472696320> Tj 1 0 0 1 94.80 555.36 Tm <73656E736F7220> Tj 1 0 0 1 130.08 555.36 Tm <647269667420> Tj 1 0 0 1 156.72 555.60 Tm <696E20> Tj 1 0 0 1 172.32 555.60 Tm Tj 1 0 0 1 238.32 555.60 Tm <6F6920> Tj 1 0 0 1 254.40 555.60 Tm <636F72743A7461727474> Tj 0.96 Tc 1 0 0 1 54.96 543.60 Tm <76616C7565733A20> Tj 1 0 0 1 90.00 543.84 Tm <2A6869636820> Tj 1 0 0 1 120.72 543.84 Tm <5C5C27617320> Tj 1 0 0 1 141.60 543.60 Tm <6E6F7420> Tj 1 0 0 1 159.60 543.60 Tm <6F6273657272656420> Tj 1 0 0 1 203.52 543.84 Tm <696E20> Tj 1 0 0 1 215.76 543.60 Tm <74686520> Tj 1 0 0 1 233.28 543.84 Tm <73696E2D72756C74616E656F7573> Tj 0.96 Tc 1 0 0 1 54.96 531.36 Tm <6F7363696C6C6F73636F706520> Tj 1 0 0 1 112.56 531.60 Tm <6D6F6E69746F72696E6720> Tj 1 0 0 1 164.88 531.60 Tm <6F6620> Tj 1 0 0 1 176.88 531.60 Tm <7468697320> Tj 1 0 0 1 195.84 532.08 Tm <706172616D657465722E> Tj 0.72 Tc 1 0 0 1 68.88 519.84 Tm <46696775726520> Tj 1 0 0 1 104.16 519.84 Tm <3320> Tj 1 0 0 1 115.92 519.84 Tm <73686F777320> Tj 1 0 0 1 149.76 519.84 Tm <746861742C20> Tj 1 0 0 1 175.20 520.08 Tm <6465737069746520> Tj 1 0 0 1 213.36 520.08 Tm <686176696E6720> Tj 1 0 0 1 249.36 520.08 Tm <74686520> Tj 1 0 0 1 269.04 520.08 Tm <73616D65> Tj 0.72 Tc 1 0 0 1 54.72 507.84 Tm <636F6D706F736974696F6E2C20> Tj 1 0 0 1 117.36 508.08 Tm <74686520> Tj 1 0 0 1 135.36 508.08 Tm <3330632F6F20> Tj 1 0 0 1 160.32 508.32 Tm <49726C416C7A4F7220> Tj 1 0 0 1 201.36 508.32 Tm <636174616C79737420> Tj 1 0 0 1 240.00 508.56 Tm <707265706172656420> Tj 1 0 0 1 283.44 508.32 Tm <6174> Tj 0.72 Tc 1 0 0 1 54.96 496.08 Tm <494E504520> Tj 1 0 0 1 81.84 496.32 Tm <77617320> Tj 1 0 0 1 102.00 496.08 Tm <736C696768746C7920> Tj 1 0 0 1 138.00 496.32 Tm <6C65737320> Tj 1 0 0 1 157.44 496.08 Tm <737461626C6520> Tj 1 0 0 1 186.00 496.32 Tm <7468616E20> Tj 1 0 0 1 207.84 496.32 Tm <74686520> Tj 1 0 0 1 224.16 496.32 Tm <5368656C6C20> Tj 1 0 0 1 249.60 496.56 Tm <3430352E20> Tj 1 0 0 1 271.68 496.56 Tm <54686973> Tj 0.48 Tc 1 0 0 1 54.96 484.08 Tm <64656D6F6E7374726174657320> Tj 1 0 0 1 120.00 484.32 Tm <7468617420> Tj 1 0 0 1 143.52 484.32 Tm <74686520> Tj 1 0 0 1 163.92 484.32 Tm <6D616A6F7220> Tj 1 0 0 1 196.80 484.56 Tm <696D70726F76656D656E7420> Tj 1 0 0 1 262.32 484.56 Tm <6F6620> Tj 1 0 0 1 278.16 484.56 Tm <746865> Tj 0.48 Tc 1 0 0 1 54.96 472.08 Tm <636F6D6D65726369616C20> Tj 1 0 0 1 111.36 472.32 Tm <636174616C79737420> Tj 1 0 0 1 150.48 472.32 Tm <697320> Tj 1 0 0 1 162.00 472.32 Tm <6265636175736520> Tj 1 0 0 1 202.08 472.56 Tm <6F6620> Tj 1 0 0 1 215.52 472.56 Tm <74686520> Tj 1 0 0 1 233.52 472.80 Tm <70726F7065727469657320> Tj 1 0 0 1 282.48 472.56 Tm <6F66> Tj 0.48 Tc 1 0 0 1 55.20 460.32 Tm <74686520> Tj 1 0 0 1 71.52 460.56 Tm <616C756D696E6120> Tj 1 0 0 1 109.44 460.56 Tm <7573656420> Tj 1 0 0 1 133.20 460.56 Tm <617320> Tj 1 0 0 1 145.20 460.56 Tm <74686520> Tj 1 0 0 1 162.00 460.56 Tm <737570706F72742E> Tj 0.48 Tc 1 0 0 1 69.12 448.56 Tm <46696775726520> Tj 1 0 0 1 102.48 448.56 Tm <3420> Tj 1 0 0 1 113.04 448.56 Tm <73686F777320> Tj 1 0 0 1 145.20 448.56 Tm <74686520> Tj 1 0 0 1 163.44 448.80 Tm <706572666F726D616E636520> Tj 1 0 0 1 224.40 448.80 Tm <6F6620> Tj 1 0 0 1 238.08 448.80 Tm <6120> Tj 1 0 0 1 247.20 448.80 Tm <62696D6574616C6C6963> Tj 0.48 Tc 1 0 0 1 55.20 436.56 Tm <636174616C79737420> Tj 1 0 0 1 94.56 436.80 Tm <696E20> Tj 1 0 0 1 108.48 437.04 Tm <70756C73656420> Tj 1 0 0 1 143.04 436.80 Tm <726567696D652E20> Tj 1 0 0 1 181.68 437.04 Tm <54686520> Tj 1 0 0 1 204.72 436.80 Tm <6F766572707265737375726520> Tj 1 0 0 1 266.64 437.28 Tm <7065616B73> Tj 0.48 Tc 1 0 0 1 55.44 424.80 Tm <6F6273657276656420> Tj 1 0 0 1 98.88 424.80 Tm <61726520> Tj 1 0 0 1 115.68 425.28 Tm <70726F6261626C7920> Tj 1 0 0 1 158.88 425.04 Tm <64756520> Tj 1 0 0 1 178.56 425.04 Tm <746F20> Tj 1 0 0 1 190.80 425.04 Tm <74686520> Tj 1 0 0 1 208.08 425.28 Tm <6661637420> Tj 1 0 0 1 228.24 425.28 Tm <7468617420> Tj 1 0 0 1 248.40 425.28 Tm <68796472617A696E65> Tj 0.48 Tc 1 0 0 1 55.44 413.04 Tm <70656E6574726174657320> Tj 1 0 0 1 102.96 413.04 Tm <74686520> Tj 1 0 0 1 119.28 413.04 Tm <636174616C79737420> Tj 1 0 0 1 156.24 413.52 Tm <706F72657320> Tj 1 0 0 1 183.12 413.28 Tm <616E6420> Tj 1 0 0 1 201.60 413.28 Tm <6465636F6D706F73657320> Tj 1 0 0 1 258.24 413.52 Tm <7468657265696E2E> Tj 0.72 Tc 1 0 0 1 55.20 401.04 Tm <546865736520> Tj 1 0 0 1 85.20 401.52 Tm <7065616B7320> Tj 1 0 0 1 113.76 401.04 Tm <73686F756C6420> Tj 1 0 0 1 146.64 401.28 Tm <626520> Tj 1 0 0 1 160.56 401.28 Tm <61766F6964656420> Tj 1 0 0 1 198.96 401.28 Tm <6265636175736520> Tj 1 0 0 1 237.36 401.52 Tm <7468657920> Tj 1 0 0 1 259.68 401.52 Tm <68656176696C79> Tj 0.48 Tc 1 0 0 1 319.20 792.48 Tm <636F6E7472696275746520> Tj 1 0 0 1 367.20 792.24 Tm <746F20> Tj 1 0 0 1 378.72 792.48 Tm <66726163747572657320> Tj 1 0 0 1 420.72 792.48 Tm <696E20> Tj 1 0 0 1 432.00 792.24 Tm <74686520> Tj 1 0 0 1 448.32 792.24 Tm <6D6174657269616C2C20> Tj 1 0 0 1 490.32 792.24 Tm <63617573696E6720> Tj 1 0 0 1 526.56 792.24 Tm <6C6F737320> Tj 1 0 0 1 546.48 792.24 Tm <6F66> Tj 0.48 Tc 1 0 0 1 319.20 780.48 Tm <6D6173732E20> Tj 1 0 0 1 349.20 780.48 Tm <5468657920> Tj 1 0 0 1 377.52 780.48 Tm <7765726520> Tj 1 0 0 1 404.16 780.48 Tm <6F6273657276656420> Tj 1 0 0 1 449.52 780.48 Tm <6D6F726520> Tj 1 0 0 1 477.36 780.48 Tm <6672657175656E746C7920> Tj 1 0 0 1 528.00 780.24 Tm <617320> Tj 1 0 0 1 542.16 780.24 Tm <746865> Tj 0.48 Tc 1 0 0 1 319.20 768.48 Tm <72757468656E69756D20> Tj 1 0 0 1 367.44 768.48 Tm <636F6E74656E7420> Tj 1 0 0 1 403.44 768.48 Tm <696E637265617365642E> Tj 0.48 Tc 1 0 0 1 333.60 756.72 Tm <496E20> Tj 1 0 0 1 345.36 756.72 Tm <46696775726520> Tj 1 0 0 1 377.76 756.72 Tm <3520> Tj 1 0 0 1 386.64 756.72 Tm <697420> Tj 1 0 0 1 395.76 756.72 Tm <63616E20> Tj 1 0 0 1 414.48 756.72 Tm <626520> Tj 1 0 0 1 428.40 756.72 Tm <7365656E20> Tj 1 0 0 1 451.20 756.72 Tm <7468617420> Tj 1 0 0 1 471.12 756.72 Tm <74686520> Tj 1 0 0 1 487.92 756.72 Tm <72757468656E69756D20> Tj 1 0 0 1 536.40 756.48 Tm <6F6E6C79> Tj 0.48 Tc 1 0 0 1 319.20 744.96 Tm <636174616C79737420> Tj 1 0 0 1 356.64 744.96 Tm <68617320> Tj 1 0 0 1 375.12 744.96 Tm <74686520> Tj 1 0 0 1 392.16 744.96 Tm <6869676865737420> Tj 1 0 0 1 427.92 744.96 Tm <6368616D62657220> Tj 1 0 0 1 469.92 744.96 Tm <737461676E6174696F6E20> Tj 1 0 0 1 518.64 745.20 Tm <7072657373757265> Tj 0.72 Tc 1 0 0 1 319.44 733.20 Tm <696E73746162696C69747920> Tj 1 0 0 1 367.20 733.20 Tm <6F6620> Tj 1 0 0 1 379.68 733.20 Tm <616C6C20> Tj 1 0 0 1 394.08 732.96 Tm <74686520> Tj 1 0 0 1 410.88 733.20 Tm <636174616C797374732E20> Tj 1 0 0 1 455.28 733.20 Tm <5468697320> Tj 1 0 0 1 478.56 733.20 Tm <696E73746162696C6974792C20> Tj 1 0 0 1 528.72 733.20 Tm <7768696368> Tj 0.72 Tc 1 0 0 1 319.44 721.44 Tm <68617320> Tj 1 0 0 1 339.12 721.20 Tm <6265656E20> Tj 1 0 0 1 365.52 721.20 Tm <6F6273657276656420> Tj 1 0 0 1 410.88 721.20 Tm <73696E636520> Tj 1 0 0 1 438.96 721.20 Tm <74686520> Tj 1 0 0 1 457.68 721.44 Tm <666972737420> Tj 1 0 0 1 480.96 721.44 Tm <666972696E677320> Tj 1 0 0 1 515.04 721.44 Tm <7769746820> Tj 1 0 0 1 539.52 721.20 Tm <74686973> Tj 0.72 Tc 1 0 0 1 319.20 709.44 Tm <6D6174657269616C2C20> Tj 1 0 0 1 367.20 709.68 Tm <696E6372656173657320> Tj 1 0 0 1 416.40 709.68 Tm <7769746820> Tj 1 0 0 1 444.72 709.44 Tm <6D6574616C20> Tj 1 0 0 1 477.84 709.44 Tm <636F6E74656E742E20> Tj 1 0 0 1 521.52 709.68 Tm <417320> Tj 1 0 0 1 542.16 709.44 Tm <746865> Tj 0.48 Tc 1 0 0 1 319.44 697.44 Tm <737570706F727420> Tj 1 0 0 1 357.12 697.68 Tm <697320> Tj 1 0 0 1 368.88 697.68 Tm <616C7761797320> Tj 1 0 0 1 403.92 697.68 Tm <74686520> Tj 1 0 0 1 422.40 697.68 Tm <73616D652C20> Tj 1 0 0 1 451.92 697.68 Tm <697420> Tj 1 0 0 1 462.48 697.68 Tm <63616E20> Tj 1 0 0 1 482.40 697.68 Tm <626520> Tj 1 0 0 1 497.28 697.68 Tm <617373756D656420> Tj 1 0 0 1 539.04 697.68 Tm <74686174> Tj 0.24 Tc 1 0 0 1 319.20 685.68 Tm <7468697320> Tj 1 0 0 1 340.32 685.92 Tm <697320> Tj 1 0 0 1 352.80 685.92 Tm <63617573656420> Tj 1 0 0 1 387.60 685.92 Tm <627920> Tj 1 0 0 1 403.92 685.92 Tm <696E636F6D706C65746520> Tj 1 0 0 1 456.72 685.92 Tm <6D6574616C20> Tj 1 0 0 1 485.76 685.92 Tm <726564756374696F6E2E20> Tj 1 0 0 1 533.52 686.16 Tm <417320> Tj 1 0 0 1 551.04 685.92 Tm <61> Tj 0.24 Tc 1 0 0 1 319.20 673.92 Tm <636F6E73657175656E63652C20> Tj 1 0 0 1 378.96 673.92 Tm <746865726520> Tj 1 0 0 1 403.20 674.16 Tm <697320> Tj 1 0 0 1 413.28 674.16 Tm <6120> Tj 1 0 0 1 420.96 674.40 Tm <6772656174657220> Tj 1 0 0 1 453.36 674.16 Tm <6C6F737320> Tj 1 0 0 1 472.80 674.16 Tm <6F6620> Tj 1 0 0 1 484.56 674.16 Tm <6D61737320> Tj 1 0 0 1 508.32 674.16 Tm <7768656E20> Tj 1 0 0 1 534.00 674.16 Tm <7468657365> Tj 0.24 Tc 1 0 0 1 319.20 662.40 Tm <70726F647563747320> Tj 1 0 0 1 358.80 662.16 Tm <61726520> Tj 1 0 0 1 374.40 662.16 Tm <757365642C20> Tj 1 0 0 1 399.12 662.40 Tm <776869636820> Tj 1 0 0 1 428.16 662.40 Tm <6372656174657320> Tj 1 0 0 1 460.80 662.40 Tm <6D6F726520> Tj 1 0 0 1 485.52 662.40 Tm <766F69647320> Tj 1 0 0 1 511.20 662.64 Tm <696E20> Tj 1 0 0 1 522.24 662.40 Tm <74686520> Tj 1 0 0 1 537.84 662.40 Tm <6265642C> Tj 0.24 Tc 1 0 0 1 319.20 650.64 Tm <636F6E73657175656E746C7920> Tj 1 0 0 1 377.76 650.64 Tm <696E74726F647563696E6720> Tj 1 0 0 1 428.88 650.88 Tm <6D616E7920> Tj 1 0 0 1 454.80 650.88 Tm <707265666572656E7469616C20> Tj 1 0 0 1 505.92 651.12 Tm <70617468732E> Tj 0.48 Tc 1 0 0 1 333.60 638.88 Tm <5468697320> Tj 1 0 0 1 356.88 638.88 Tm <6879706F74686573697320> Tj 1 0 0 1 407.76 638.88 Tm <697320> Tj 1 0 0 1 418.80 638.88 Tm <737570706F7274656420> Tj 1 0 0 1 465.84 638.88 Tm <627920> Tj 1 0 0 1 480.24 639.12 Tm <74686520> Tj 1 0 0 1 497.04 639.12 Tm <6461746120> Tj 1 0 0 1 518.88 639.12 Tm <696E20> Tj 1 0 0 1 530.40 639.12 Tm <5461626C65> Tj 0.48 Tc 1 0 0 1 319.44 626.88 Tm <362C20> Tj 1 0 0 1 332.40 626.88 Tm <776869636820> Tj 1 0 0 1 364.08 626.88 Tm <73686F7720> Tj 1 0 0 1 391.68 626.88 Tm <74686520> Tj 1 0 0 1 409.92 627.12 Tm <696E697469616C20> Tj 1 0 0 1 440.64 627.12 Tm <6D61737320> Tj 1 0 0 1 467.28 627.12 Tm <696E20> Tj 1 0 0 1 480.24 627.12 Tm <74686520> Tj 1 0 0 1 498.24 627.36 Tm <636174616C7974696320> Tj 1 0 0 1 539.76 627.36 Tm <626564> Tj 0.72 Tc 1 0 0 1 319.68 614.88 Tm <616E6420> Tj 1 0 0 1 338.64 614.88 Tm <74686520> Tj 1 0 0 1 355.20 615.12 Tm <636F72726573706F6E64696E6720> Tj 1 0 0 1 422.40 615.36 Tm <6C6F737320> Tj 1 0 0 1 442.80 615.12 Tm <6D61737320> Tj 1 0 0 1 468.24 615.12 Tm <6F6620> Tj 1 0 0 1 480.48 615.36 Tm <647572696E6720> Tj 1 0 0 1 512.16 615.60 Tm <666972696E67732E20> Tj 1 0 0 1 546.96 615.60 Tm <496E> Tj 0.48 Tc 1 0 0 1 319.44 603.12 Tm <5461626C6520> Tj 1 0 0 1 348.72 603.12 Tm <3620> Tj 1 0 0 1 358.32 603.36 Tm <697420> Tj 1 0 0 1 368.40 603.12 Tm <63616E20> Tj 1 0 0 1 387.60 603.12 Tm <626520> Tj 1 0 0 1 402.00 603.36 Tm <6F6273657276656420> Tj 1 0 0 1 446.16 603.36 Tm <7468617420> Tj 1 0 0 1 466.80 603.36 Tm <74686520> Tj 1 0 0 1 484.32 603.60 Tm <6C6F7373657320> Tj 1 0 0 1 514.32 603.60 Tm <61726520> Tj 1 0 0 1 531.60 603.60 Tm <6D756368> Tj 0.48 Tc 1 0 0 1 319.68 591.36 Tm <68696768657220> Tj 1 0 0 1 350.64 591.60 Tm <666F7220> Tj 1 0 0 1 366.72 591.36 Tm <74686520> Tj 1 0 0 1 383.28 591.60 Tm <636174616C7973747320> Tj 1 0 0 1 424.56 591.84 Tm <707265706172656420> Tj 1 0 0 1 466.80 591.60 Tm <617420> Tj 1 0 0 1 477.60 591.84 Tm <494E504520> Tj 1 0 0 1 504.72 591.84 Tm <7468616E20> Tj 1 0 0 1 526.56 591.84 Tm <666F7220> Tj 1 0 0 1 542.40 591.84 Tm <746865> Tj 0.72 Tc 1 0 0 1 319.92 579.36 Tm <49726C416C7A4F3A20> Tj 1 0 0 1 359.76 579.36 Tm <5368656C6C20> Tj 1 0 0 1 386.16 579.60 Tm <34303520> Tj 1 0 0 1 406.32 579.60 Tm <636174616C79737420> Tj 1 0 0 1 444.48 579.60 Tm <616E6420> Tj 1 0 0 1 463.92 579.60 Tm <7468617420> Tj 1 0 0 1 484.56 579.84 Tm <7468657920> Tj 1 0 0 1 507.12 579.84 Tm <696E63726561736520> Tj 1 0 0 1 546.96 579.84 Tm <6173> Tj 0.96 Tc 1 0 0 1 319.92 567.60 Tm <74686520> Tj 1 0 0 1 341.04 567.60 Tm <72757468656E69756D20> Tj 1 0 0 1 394.08 567.84 Tm <636F6E74656E7420> Tj 1 0 0 1 434.88 567.84 Tm <696E637265617365732E20> Tj 1 0 0 1 486.24 568.08 Tm <5468697320> Tj 1 0 0 1 513.60 568.08 Tm <636F756C6420> Tj 1 0 0 1 545.52 568.08 Tm <6265> Tj 0.72 Tc 1 0 0 1 319.92 555.60 Tm <6173736F63696174656420> Tj 1 0 0 1 373.92 555.84 Tm <666972737420> Tj 1 0 0 1 400.08 556.32 Tm <752C69746820> Tj 1 0 0 1 427.92 556.08 Tm <74686520> Tj 1 0 0 1 449.76 556.08 Tm <6661637420> Tj 1 0 0 1 474.72 556.08 Tm <7468617420> Tj 1 0 0 1 499.44 556.08 Tm <74686520> Tj 1 0 0 1 520.80 556.32 Tm <616C756D696E61> Tj 0.96 Tc 1 0 0 1 319.92 544.32 Tm <707265706172656420> Tj 1 0 0 1 362.64 544.08 Tm <617420> Tj 1 0 0 1 374.64 544.08 Tm <495C504520> Tj 1 0 0 1 402.48 544.08 Tm <68617320> Tj 1 0 0 1 420.96 544.32 Tm <6120> Tj 1 0 0 1 429.60 544.32 Tm <6C6F7527657220> Tj 1 0 0 1 458.64 544.32 Tm <6D656368616E6963616C20> Tj 1 0 0 1 512.64 544.56 Tm <726573697374616E6365> Tj 0.72 Tc 1 0 0 1 320.16 532.08 Tm <616E6420> Tj 1 0 0 1 338.88 532.08 Tm <636F6E7461696E7320> Tj 1 0 0 1 379.20 532.08 Tm <6120> Tj 1 0 0 1 387.36 532.32 Tm <6C617267657220> Tj 1 0 0 1 416.40 532.32 Tm <61CC6E6F756E7420> Tj 1 0 0 1 452.40 532.32 Tm <6F6620> Tj 1 0 0 1 464.64 532.32 Tm <6D6163726F706F72657320> Tj 1 0 0 1 519.12 532.56 Tm <616E6420> Tj 1 0 0 1 537.84 532.56 Tm <74687573> Tj 0.96 Tc 1 0 0 1 319.92 518.16 Tm <6C20> Tj 1 0 0 1 325.68 520.32 Tm <69656C647320> Tj 1 0 0 1 357.60 520.32 Tm <6C65732D7320> Tj 1 0 0 1 384.96 520.56 Tm <64656E736520> Tj 1 0 0 1 421.20 520.56 Tm <636174616C2920> Tj 1 0 0 1 448.32 520.56 Tm <7374732E20> Tj 1 0 0 1 473.52 520.80 Tm <496E20> Tj 1 0 0 1 493.44 520.80 Tm <6164646974696F6E2C20> Tj 1 0 0 1 542.88 520.80 Tm <746865> Tj 0.72 Tc 1 0 0 1 320.16 508.56 Tm <696E636F6D706965746520> Tj 1 0 0 1 377.28 508.56 Tm <726564756374696F6E20> Tj 1 0 0 1 427.44 508.80 Tm <6F6620> Tj 1 0 0 1 444.72 508.80 Tm <72757468656E69756D20> Tj 1 0 0 1 498.00 509.28 Tm <70726576656E747320> Tj 1 0 0 1 542.88 509.04 Tm <746865> Tj 0.72 Tc 1 0 0 1 320.16 496.56 Tm <6D6574616C20> Tj 1 0 0 1 356.64 497.04 Tm <7061727469636C657320> Tj 1 0 0 1 406.80 496.80 Tm <66726F6D20> Tj 1 0 0 1 440.40 497.28 Tm <70726F766964696E6720> Tj 1 0 0 1 495.60 497.04 Tm <616E20> Tj 1 0 0 1 517.68 497.28 Tm <656666656374697665> Tj 0.72 Tc 1 0 0 1 320.16 484.80 Tm <70726F74656374696F6E20> Tj 1 0 0 1 368.40 484.80 Tm <666F7220> Tj 1 0 0 1 384.72 484.80 Tm <74686520> Tj 1 0 0 1 401.52 485.04 Tm <737570706F72742C20> Tj 1 0 0 1 441.12 485.28 Tm <776869636820> Tj 1 0 0 1 471.36 485.28 Tm <697320> Tj 1 0 0 1 481.92 485.28 Tm <7365766572656C7920> Tj 1 0 0 1 521.76 485.52 Tm <7374726573736564> Tj 0.48 Tc 1 0 0 1 319.92 472.56 Tm <627920> Tj 1 0 0 1 334.80 472.80 Tm <74686520> Tj 1 0 0 1 352.32 472.80 Tm <746865726D6F2D6D656368616E6963616C20> Tj 1 0 0 1 442.08 473.28 Tm <6C6F616420> Tj 1 0 0 1 465.12 473.28 Tm <6173736F63696174656420> Tj 1 0 0 1 514.80 473.52 Tm <7769746820> Tj 1 0 0 1 538.08 473.52 Tm <68656174> Tj 0.48 Tc 1 0 0 1 320.40 461.04 Tm <616E6420> Tj 1 0 0 1 346.32 461.04 Tm <6D61737320> Tj 1 0 0 1 378.48 461.28 Tm <7472616E7366657220> Tj 1 0 0 1 422.64 461.76 Tm <7068656E6F6D656E6120> Tj 1 0 0 1 484.08 461.76 Tm <647572696E6720> Tj 1 0 0 1 522.72 461.76 Tm <7468727573746572> Tj 0.48 Tc 1 0 0 1 320.40 449.04 Tm <6F7065726174696F6E2E20> Tj 1 0 0 1 367.92 449.28 Tm <4F6E20> Tj 1 0 0 1 384.00 449.28 Tm <74686520> Tj 1 0 0 1 400.32 449.28 Tm <6F7468657220> Tj 1 0 0 1 426.00 449.76 Tm <68616E642C20> Tj 1 0 0 1 453.12 449.76 Tm <6972696469756D20> Tj 1 0 0 1 488.16 449.76 Tm <64697370657273657320> Tj 1 0 0 1 531.36 450.00 Tm <626574746572> Tj 0.48 Tc 1 0 0 1 320.40 437.28 Tm <6F6E20> Tj 1 0 0 1 335.76 437.28 Tm <74686520> Tj 1 0 0 1 354.00 437.28 Tm <737570706F727420> Tj 1 0 0 1 391.44 437.52 Tm <616E6420> Tj 1 0 0 1 411.84 437.76 Tm <68617320> Tj 1 0 0 1 431.28 437.76 Tm <6120> Tj 1 0 0 1 440.16 437.76 Tm <68696768657220> Tj 1 0 0 1 473.28 438.00 Tm <6C6576656C20> Tj 1 0 0 1 498.96 438.00 Tm <6F6620> Tj 1 0 0 1 512.16 438.24 Tm <726564756374696F6E2C> Tj 0.48 Tc 1 0 0 1 320.40 425.52 Tm <7468657265627920> Tj 1 0 0 1 357.60 426.00 Tm <70726F766964696E6720> Tj 1 0 0 1 404.64 425.76 Tm <62657474657220> Tj 1 0 0 1 434.40 426.24 Tm <70726F74656374696F6E20> Tj 1 0 0 1 483.60 426.24 Tm <746F20> Tj 1 0 0 1 496.32 426.24 Tm <74686520> Tj 1 0 0 1 513.84 426.24 Tm <5368656C6C20> Tj 1 0 0 1 540.24 426.48 Tm <343035> Tj 0.72 Tc 1 0 0 1 320.64 413.52 Tm <616C756D696E6120> Tj 1 0 0 1 359.52 414.00 Tm <77686963682C20> Tj 1 0 0 1 392.88 414.00 Tm <696E20> Tj 1 0 0 1 405.12 414.00 Tm <6164646974696F6E2E20> Tj 1 0 0 1 448.08 414.24 Tm <7365656D7320> Tj 1 0 0 1 478.32 414.48 Tm <746F20> Tj 1 0 0 1 490.08 414.48 Tm <626520> Tj 1 0 0 1 504.00 414.48 Tm <696E7472696E736963616C6C79> Tj 0.48 Tc 1 0 0 1 320.64 401.76 Tm <6D6F726520> Tj 1 0 0 1 345.84 402.00 Tm <726573697374616E7420> Tj 1 0 0 1 386.16 402.00 Tm <7468616E20> Tj 1 0 0 1 408.00 402.24 Tm <74686520> Tj 1 0 0 1 424.56 402.48 Tm <494E504520> Tj 1 0 0 1 451.92 402.24 Tm <616C756D696E612E> Tj 0.00 Tc /F3 14.0 Tf 1 0 0 1 378.48 260.64 Tm <2B2C2C2369CB653B24C8242E46CB23642B> Tj 0.24 Tc /F3 3.0 Tf 1 0 0 1 468.00 180.24 Tm <3A4A> Tj 0.48 Tc 1 0 0 1 456.48 176.16 Tm <3A20> Tj 1 0 0 1 459.60 176.16 Tm Tj 1 0 0 1 463.20 176.16 Tm <3A2E3A3A69> Tj 0.48 Tc /F3 11.0 Tf 1 0 0 1 134.16 155.76 Tm <3020> Tj 1 0 0 1 412.32 156.48 Tm Tj 1 0 0 1 454.80 156.48 Tm <32303020> Tj 1 0 0 1 471.84 156.48 Tm <73> Tj 0.48 Tc 1 0 0 1 68.40 141.12 Tm <46696775726520> Tj 1 0 0 1 105.12 141.36 Tm <323A20> Tj 1 0 0 1 118.08 141.36 Tm <506572666F726D616E636520> Tj 1 0 0 1 182.88 141.36 Tm <6F6620> Tj 1 0 0 1 196.08 141.36 Tm <5368656C6C20> Tj 1 0 0 1 223.68 141.60 Tm <34303520> Tj 1 0 0 1 245.04 141.60 Tm <636F6D6D65726369616C20> Tj 1 0 0 1 304.80 141.60 Tm <636174616C79737420> Tj 1 0 0 1 344.40 141.60 Tm <696E20> Tj 1 0 0 1 356.64 141.60 Tm <74686520> Tj 1 0 0 1 374.40 141.84 Tm <6C61737420> Tj 1 0 0 1 393.84 141.84 Tm <636F6E74696E756F757320> Tj 1 0 0 1 450.24 142.08 Tm <666972696E672E20> Tj 1 0 0 1 483.36 142.08 Tm <4F7264696E61746520> Tj 1 0 0 1 528.24 142.32 Tm <61786973> Tj 1.20 Tc 1 0 0 1 78.48 127.20 Tm <72616E67653A20> Tj 1 0 0 1 112.56 127.20 Tm <312D54656D70657261747572653A20> Tj 1 0 0 1 197.52 127.20 Tm <302D20> Tj 1 0 0 1 217.44 127.44 Tm <3130303022433A322D20> Tj 1 0 0 1 278.88 127.44 Tm <4C696E6570726573737572653A20> Tj 1 0 0 1 350.16 127.68 Tm <302D34306261722C20> Tj 1 0 0 1 405.36 127.68 Tm <332D537461676E6174696F6E7072657373757265696E746865> Tj 0.72 Tc 1 0 0 1 158.40 113.76 Tm <6368616D6265723A20> Tj 1 0 0 1 203.52 116.16 Tm <2D313020> Tj 1 0 0 1 222.96 116.16 Tm <2D32306261723B20> Tj 1 0 0 1 264.24 114.00 Tm <3420> Tj 1 0 0 1 273.60 116.16 Tm <2D5468727573743A20> Tj 1 0 0 1 316.08 114.00 Tm <3020> Tj 1 0 0 1 324.00 116.16 Tm <2D20> Tj 1 0 0 1 332.40 114.00 Tm <3420> Tj 1 0 0 1 340.80 114.00 Tm <4E3B20> Tj 1 0 0 1 354.96 114.00 Tm <3520> Tj 1 0 0 1 362.88 116.40 Tm <2D20> Tj 1 0 0 1 371.28 114.24 Tm <466C6F7720> Tj 1 0 0 1 396.96 114.24 Tm <726174653A20> Tj 1 0 0 1 419.76 114.48 Tm <3020> Tj 1 0 0 1 427.92 116.64 Tm <2D20> Tj 1 0 0 1 436.32 114.48 Tm <3420> Tj 1 0 0 1 446.16 114.72 Tm <676C73> Tj 0.48 Tc /F3 7.0 Tf 1 0 0 1 143.52 90.72 Tm <4272617A2E696C6974757420> Tj 1 0 0 1 175.92 90.48 Tm <4A6F75726E616C20> Tj 1 0 0 1 204.00 90.48 Tm <6F664368656DEC63616C20> Tj 1 0 0 1 245.52 90.72 Tm <456E67696E656572696E672C20> Tj 1 0 0 1 290.64 90.48 Tm <566F6C2E32302C20> Tj 1 0 0 1 319.68 90.48 Tm <4E6F2E30332C20> Tj 1 0 0 1 347.04 90.72 Tm <70702E32373320> Tj 1 0 0 1 374.64 92.16 Tm <2D20> Tj 1 0 0 1 378.96 90.72 Tm <3238322C20> Tj 1 0 0 1 397.44 90.72 Tm <4A756C7920> Tj 1 0 0 1 413.52 92.40 Tm <2D20> Tj 1 0 0 1 418.08 90.72 Tm <53657074656D62657232303033> Tj 0.48 Tc /F3 10.0 Tf 1 0 0 1 467.28 240.96 Tm <2CCC> Tj 0.24 Tc /F3 6.0 Tf 1 0 0 1 467.76 229.92 Tm <2C6C> Tj 0.00 Tc /F3 9.0 Tf 1 0 0 1 304.08 214.80 Tm <692EEF7B6920> Tj 1 0 0 1 317.28 213.36 Tm <24714A3422733B64CA6569EC722E727222672E2AC16C69722C657523727427276E2A2E20> Tj 1 0 0 1 426.48 215.52 Tm <432E2E2F726C2E2C3B272A2B20> Tj 1 0 0 1 455.04 216.24 Tm <222C2C2A453B> Tj 1.50 Tc 1 0 0 1 336.72 211.44 Tm <272D662E2C> Tj 0.00 Tc 1 0 0 1 360.00 202.56 Tm <2F2D> Tj 1.50 Tc /F3 7.0 Tf 1 0 0 1 334.56 195.12 Tm <352D74> Tj ET endstream endobj 55 0 obj 27816 endobj 56 0 obj << /Length 57 0 R >> stream Ir-Ru/AlzOr Catalysts Used in Satellite Propulsion / Figures 2 to 5 allow a better visualization of theperformance of different catalysts in the thruster.One evaluation of these test results showed that, forinitial bed temperatures of 373 K, all catalysts had asimilar ignition delay of about 20 ms. According toArmstrong et al. [1978b], there are very significantdifferences in ignition delay between the lrlAlzOr,Ru/Al2O3, and Ir-Ru/AlzOr catalysts only whendecomposition is started at ambient temperature (theso-called "cold starts"). In this case, IrlAl2O3 has theshortest delay. As the performances of the newcatalysts were not known a priori, cold starts werenot studied in this work to avoid the possibility ofIong i-enition delays, which could result in hydrazineaccumulation in the bed, followed by a hazardousrou_eh initiation. rihich could damage the thrusterand rnea:urcrncnt de\ icc..Figure I shoris the .'rcellent stabrlrtl of Shell -105for all the parameter: :tudied. The sight but steadvfall in the pressure curve i: due to the classtc piezo-electric sensor drift in reasurement oi cort:tarttvalues: *hich \\'as not obserred in the sin-rultaneousoscilloscope monitoring of this parameter.Figure 3 shows that, despite having the samecomposition, the 30c/o IrlAlzOr catalyst prepared atINPE was slightly less stable than the Shell 405. Thisdemonstrates that the major improvement of thecommercial catalyst is because of the properties ofthe alumina used as the support.Figure 4 shows the performance of a bimetalliccatalyst in pulsed regime. The overpressure peaksobserved are probably due to the fact that hydrazinepenetrates the catalyst pores and decomposes therein.These peaks should be avoided because they heavily contribute to fractures in the material, causing loss ofmass. They were observed more frequently as theruthenium content increased.In Figure 5 it can be seen that the ruthenium onlycatalyst has the highest chamber stagnation pressureinstability of all the catalysts. This instability, whichhas been observed since the first firings with thismaterial, increases with metal content. As thesupport is always the same, it can be assumed thatthis is caused by incomplete metal reduction. As aconsequence, there is a greater loss of mass when theseproducts are used, which creates more voids in the bed,consequently introducing many preferential paths.This hypothesis is supported by the data in Table6, which show the initial mass in the catalytic bedand the corresponding loss mass of during firings. InTable 6 it can be observed that the losses are muchhigher for the catalysts prepared at INPE than for theIrlAlzO: Shell 405 catalyst and that they increase asthe ruthenium content increases. This could beassociated first u,ith the fact that the aluminaprepared at I\PE has a lou'er mechanical resistanceand contains a larger anount of macropores and thusl ields les-s dense catal) sts. In addition, theincompiete reduction of ruthenium prevents themetal particles from providing an effectiveprotection for the support, which is severely stressedby the thermo-mechanical load associated with heatand mass transfer phenomena during thrusteroperation. On the other hand, iridium disperses betteron the support and has a higher level of reduction,thereby providing better protection to the Shell 405alumina which, in addition. seems to be intrinsicallymore resistant than the INPE alumina. +,,#ie;$$.F#d+ :J: :.::i 0 lME 200 sFigure 2: Performance of Shell 405 commercial catalyst in the last continuous firing. Ordinate axisrange: 1-Temperature: 0- 1000"C:2- Linepressure: 0-40bar, 3-Stagnationpressureinthechamber: -10 -20bar; 4 -Thrust: 0 - 4 N; 5 - Flow rate: 0 - 4 glsBraz.ilitut Journal ofChemcal Engineering, Vol.20, No.03, pp.273 - 282, July - September2003 ,,li.{i $qJ4"s;deir.rr"g.*lir,eu#rt''n*. 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0.48 Tc 1 0 0 1 53.76 178.08 Tm <537572666163652C20> Tj 1 0 0 1 94.56 177.84 Tm <556E69766572736974E920> Tj 1 0 0 1 145.20 177.36 Tm <50696572726520> Tj 1 0 0 1 176.16 177.12 Tm <657420> Tj 1 0 0 1 188.40 177.12 Tm <4D6172696520> Tj 1 0 0 1 219.60 176.88 Tm <43757269652C20> Tj 1 0 0 1 251.04 176.64 Tm <506172697320> Tj 1 0 0 1 277.44 176.40 Tm <666F72> Tj 0.48 Tc 1 0 0 1 53.76 165.60 Tm <70726F766964696E6720> Tj 1 0 0 1 99.84 165.12 Tm <74686520> Tj 1 0 0 1 116.40 164.88 Tm <54454D20> Tj 1 0 0 1 143.52 164.64 Tm <616E616C7973697320> Tj 1 0 0 1 182.40 164.40 Tm <616E6420> Tj 1 0 0 1 201.36 164.16 Tm <746F20> Tj 1 0 0 1 213.12 164.16 Tm <44722E20> Tj 1 0 0 1 230.40 163.92 Tm <4A6F73E920> Tj 1 0 0 1 252.72 163.92 Tm <4175677573746F> Tj 0.48 Tc 1 0 0 1 53.52 152.40 Tm <4A6F72676520> Tj 1 0 0 1 88.56 152.16 Tm <526F6472696775657320> Tj 1 0 0 1 145.44 151.68 Tm <616E6420> Tj 1 0 0 1 172.32 151.44 Tm <4472612E20> Tj 1 0 0 1 202.80 151.20 Tm <4D617269736120> Tj 1 0 0 1 244.56 150.96 Tm <417061726563696461> Tj 0.48 Tc 1 0 0 1 53.76 139.44 Tm <5A616368617269617320> Tj 1 0 0 1 100.08 139.20 Tm <617420> Tj 1 0 0 1 111.60 138.96 Tm <4C61626F726174F372696F20> Tj 1 0 0 1 167.76 138.72 Tm <4173736F636961646F20> Tj 1 0 0 1 217.68 138.24 Tm <646520> Tj 1 0 0 1 231.60 138.00 Tm <436F6D62757374E36F20> Tj 1 0 0 1 285.12 137.76 Tm <65> Tj 0.72 Tc 1 0 0 1 53.52 126.48 Tm <50726F70756C73E36F2C20> Tj 1 0 0 1 103.44 126.00 Tm <496E7374697475746F20> Tj 1 0 0 1 143.04 125.76 Tm <4E6163696F6E616C20> Tj 1 0 0 1 186.24 125.28 Tm <646520> Tj 1 0 0 1 199.20 125.28 Tm <50657371756973617320> Tj 1 0 0 1 245.28 125.04 Tm <4573706163696169732C> Tj 0.48 Tc 1 0 0 1 53.52 113.52 Tm <4272617A696C20> Tj 1 0 0 1 83.28 113.28 Tm <666F7220> Tj 1 0 0 1 98.88 113.52 Tm <707265706172696E6720> Tj 1 0 0 1 144.48 112.80 Tm <74686520> Tj 1 0 0 1 161.04 112.56 Tm <616C756D696E6120> Tj 1 0 0 1 199.92 112.32 Tm <737570706F72742E> Tj 0.48 Tc 1 0 0 1 400.80 469.20 Tm <5245464552454E434553> Tj 0.72 Tc 1 0 0 1 319.68 444.48 Tm <416C746D616E2C20> Tj 1 0 0 1 359.28 444.24 Tm <442E20> Tj 1 0 0 1 373.68 444.24 Tm <616E6420> Tj 1 0 0 1 392.88 444.24 Tm <54686F6D61732C20> Tj 1 0 0 1 435.36 444.00 Tm <442E442E20> Tj 1 0 0 1 459.84 444.72 Tm <2831393439292C20> Tj 1 0 0 1 495.60 443.76 Tm <4576616C756174696F6E20> Tj 1 0 0 1 546.96 443.28 Tm <6F66> Tj 0.48 Tc 1 0 0 1 333.84 431.52 Tm <48796472617A696E6520> Tj 1 0 0 1 388.80 431.28 Tm <617320> Tj 1 0 0 1 406.80 431.28 Tm <6120> Tj 1 0 0 1 420.24 431.28 Tm <4D6F6E6F70726F70656C6C616E7420> Tj 1 0 0 1 501.12 430.80 Tm <616E6420> Tj 1 0 0 1 525.60 430.80 Tm <6120> Tj 1 0 0 1 539.04 430.56 Tm <476173> Tj 0.48 Tc 1 0 0 1 333.84 418.56 Tm <47656E65726174652E20> Tj 1 0 0 1 379.44 418.56 Tm <4349542D4A504C20> Tj 1 0 0 1 420.96 418.56 Tm <506570742E20> Tj 1 0 0 1 446.64 418.08 Tm <392D33362E> Tj 0.72 Tc 1 0 0 1 319.44 405.84 Tm <41726D7374726F6E672C20> Tj 1 0 0 1 382.32 405.60 Tm <572E452E2C20> Tj 1 0 0 1 420.00 405.36 Tm <52796C616E642C20> Tj 1 0 0 1 466.80 405.36 Tm <4C2E382E2C20> Tj 1 0 0 1 501.60 405.12 Tm <616E6420> Tj 1 0 0 1 529.20 404.88 Tm <566F67652C> Tj 0.72 Tc 1 0 0 1 333.84 393.12 Tm <482E482E20> Tj 1 0 0 1 358.08 393.60 Tm <283139373861292C20> Tj 1 0 0 1 417.12 392.88 Tm <436174616C79737420> Tj 1 0 0 1 475.44 392.64 Tm <666F7220> Tj 1 0 0 1 510.00 392.40 Tm <48796472617A696E65> Tj 0.48 Tc 1 0 0 1 333.60 380.64 Tm <4465636F6D706F736974696F6E20> Tj 1 0 0 1 407.04 380.40 Tm <616E6420> Tj 1 0 0 1 428.40 380.16 Tm <4D6574686F6420> Tj 1 0 0 1 468.72 380.16 Tm <666F7220> Tj 1 0 0 1 487.20 380.16 Tm <507265706172696E6720> Tj 1 0 0 1 535.92 379.68 Tm <73756368> Tj 0.72 Tc 1 0 0 1 333.60 367.68 Tm <436174616C7973742E20> Tj 1 0 0 1 375.60 367.68 Tm <554B20> Tj 1 0 0 1 394.32 367.68 Tm <506174656E7420> Tj 1 0 0 1 425.04 367.44 Tm <4170706C69636174696F6E20> Tj 1 0 0 1 480.72 367.20 Tm <474220> Tj 1 0 0 1 498.96 367.20 Tm <322E3032372E3335312E> Tj 0.72 Tc 1 0 0 1 319.20 355.20 Tm <41726D7374726F6E672C20> Tj 1 0 0 1 376.32 354.96 Tm <572E452E2C20> Tj 1 0 0 1 408.48 354.96 Tm <52796C616E642C20> Tj 1 0 0 1 450.00 354.72 Tm <4C2E382E2C20> Tj 1 0 0 1 479.28 354.48 Tm <616E6420> Tj 1 0 0 1 501.36 354.48 Tm <566F67652C20> Tj 1 0 0 1 534.48 354.24 Tm <482E482E> Tj 0.72 Tc 1 0 0 1 333.60 342.96 Tm <283139373862292C20> Tj 1 0 0 1 377.52 342.24 Tm <436174616C79737420> Tj 1 0 0 1 420.24 342.00 Tm <436F6D70726973696E6720> Tj 1 0 0 1 479.04 342.00 Tm <497220> Tj 1 0 0 1 492.48 341.76 Tm <6F7220> Tj 1 0 0 1 507.60 341.76 Tm <497220> Tj 1 0 0 1 521.04 341.76 Tm <616E6420> Tj 1 0 0 1 542.88 341.52 Tm <5275> Tj 0.48 Tc 1 0 0 1 333.36 329.76 Tm <48796472617A696E6520> Tj 1 0 0 1 384.96 329.52 Tm <4465636F6D706F736974696F6E2E20> Tj 1 0 0 1 460.80 329.28 Tm <556E6974656420> Tj 1 0 0 1 496.56 329.04 Tm <53746174657320> Tj 1 0 0 1 527.76 329.04 Tm <506174656E74> Tj 1.20 Tc 1 0 0 1 333.36 317.04 Tm <342E3132342E3533382E> Tj 0.72 Tc 1 0 0 1 319.20 304.32 Tm <41726D7374726F6E672C20> Tj 1 0 0 1 375.36 304.08 Tm <572E452E2C20> Tj 1 0 0 1 406.56 304.08 Tm <52796C616E642C20> Tj 1 0 0 1 446.88 303.84 Tm <4C2E422E2C20> Tj 1 0 0 1 475.20 303.60 Tm <616E6420> Tj 1 0 0 1 496.56 303.60 Tm <566F67652C20> Tj 1 0 0 1 528.72 303.60 Tm <482E20> Tj 1 0 0 1 544.80 303.36 Tm <482E> Tj 0.72 Tc 1 0 0 1 333.60 292.08 Tm <2831393830292C20> Tj 1 0 0 1 372.96 291.12 Tm <436174616C797365757220> Tj 1 0 0 1 427.68 291.36 Tm <706F757220> Tj 1 0 0 1 455.52 290.88 Tm <6C6120> Tj 1 0 0 1 470.64 290.88 Tm <4465636F6D706F736974696F6E20> Tj 1 0 0 1 545.04 290.40 Tm <6465> Tj 0.72 Tc 1 0 0 1 333.60 278.64 Tm <492748796472617A696E652E20> Tj 1 0 0 1 390.00 278.40 Tm <42726576657420> Tj 1 0 0 1 422.40 278.16 Tm <4427496E76656E74696F6E20> Tj 1 0 0 1 477.36 277.92 Tm <4E2720> Tj 1 0 0 1 491.76 277.92 Tm <372E3832342E20> Tj 1 0 0 1 520.32 277.92 Tm <4920> Tj 1 0 0 1 524.88 277.68 Tm <39352E> Tj 0.48 Tc 1 0 0 1 319.20 265.92 Tm <4372757A2C20> Tj 1 0 0 1 349.44 265.68 Tm <472E4D2E3B20> Tj 1 0 0 1 381.84 265.68 Tm <43756E68612C20> Tj 1 0 0 1 419.52 265.44 Tm <442E532E2C20> Tj 1 0 0 1 448.32 265.20 Tm <616E6420> Tj 1 0 0 1 470.88 265.20 Tm <536F6172657320> Tj 1 0 0 1 505.92 264.96 Tm <4E65746F2C20> Tj 1 0 0 1 536.16 264.96 Tm <542E472E> Tj 0.48 Tc 1 0 0 1 333.60 253.68 Tm <2831393839292C20> Tj 1 0 0 1 375.60 252.96 Tm <45766F6C75E7E36F20> Tj 1 0 0 1 427.20 252.72 Tm <64617320> Tj 1 0 0 1 453.12 252.48 Tm <4361726163746572ED73746963617320> Tj 1 0 0 1 526.56 252.24 Tm <46ED7369636F2D> Tj 0.24 Tc 1 0 0 1 333.36 238.08 Tm <5175ED6D6963617320> Tj 1 0 0 1 377.52 240.00 Tm <646520> Tj 1 0 0 1 391.20 240.00 Tm <436174616C697361646F72657320> Tj 1 0 0 1 452.16 239.76 Tm <49726C416C324F6A20> Tj 1 0 0 1 490.32 239.52 Tm <636FCCCCEC20> Tj 1 0 0 1 512.16 239.28 Tm <6F20> Tj 1 0 0 1 520.80 239.28 Tm <4EFA6D65726F> Tj 0.48 Tc 1 0 0 1 333.12 227.52 Tm <646520> Tj 1 0 0 1 352.80 227.52 Tm <496D707265676E61E7F565732E20> Tj 1 0 0 1 423.84 227.04 Tm <356F20> Tj 1 0 0 1 442.08 226.80 Tm <53656D696EE172696F20> Tj 1 0 0 1 494.88 226.80 Tm <42726173726C6569726F20> Tj 1 0 0 1 545.28 226.56 Tm <6465> Tj 0.72 Tc 1 0 0 1 333.12 214.56 Tm <436174E16C6973652C20> Tj 1 0 0 1 372.24 214.56 Tm <47756172756AE120> Tj 1 0 0 1 409.20 216.48 Tm <2D20> Tj 1 0 0 1 414.96 214.32 Tm <53502C20> Tj 1 0 0 1 431.76 214.32 Tm <4272617A696C2C20> Tj 1 0 0 1 462.72 214.08 Tm <766F6C2E20> Tj 1 0 0 1 482.40 214.08 Tm <312C20> Tj 1 0 0 1 491.76 214.08 Tm <3231362D3232342E> Tj 0.72 Tc 1 0 0 1 318.96 202.08 Tm <48617274756E672C20> Tj 1 0 0 1 367.20 201.60 Tm <572E20> Tj 1 0 0 1 383.52 202.32 Tm <2831393734292C20> Tj 1 0 0 1 425.28 201.36 Tm <4576616C756174696F6E20> Tj 1 0 0 1 482.88 201.12 Tm <546573747320> Tj 1 0 0 1 516.00 200.88 Tm <6F6620> Tj 1 0 0 1 534.24 200.64 Tm <4E6577> Tj 0.48 Tc 1 0 0 1 333.12 188.64 Tm <4765726D616E20> Tj 1 0 0 1 384.24 188.40 Tm <436174616C7973747320> Tj 1 0 0 1 440.88 188.40 Tm <666F7220> Tj 1 0 0 1 469.68 188.16 Tm <74686520> Tj 1 0 0 1 498.96 187.92 Tm <53706F6E74616E656F7573> Tj 0.48 Tc 1 0 0 1 333.12 176.16 Tm <4465636F6D706F736974696F6E20> Tj 1 0 0 1 404.64 175.68 Tm <6F6620> Tj 1 0 0 1 417.84 175.68 Tm <48796472617A696E652E20> Tj 1 0 0 1 470.64 175.44 Tm <50726F63656564696E677320> Tj 1 0 0 1 528.72 174.96 Tm <6F6620> Tj 1 0 0 1 541.68 174.96 Tm <746865> Tj 0.48 Tc 1 0 0 1 332.88 163.20 Tm <496E7465726E6174696F6E616C20> Tj 1 0 0 1 396.72 162.72 Tm <436F6E666572656E636520> Tj 1 0 0 1 455.28 162.48 Tm <6F6E20> Tj 1 0 0 1 473.28 162.48 Tm <74686520> Tj 1 0 0 1 493.92 162.48 Tm <50726F7065727469657320> Tj 1 0 0 1 546.00 162.00 Tm <6F66> Tj 0.48 Tc 1 0 0 1 332.88 150.24 Tm <48796472617A696E6520> Tj 1 0 0 1 384.72 150.00 Tm <616E6420> Tj 1 0 0 1 406.08 149.76 Tm <49747320> Tj 1 0 0 1 422.40 149.76 Tm <506F74656E7469616C20> Tj 1 0 0 1 467.76 149.52 Tm <4170706C69636174696F6E7320> Tj 1 0 0 1 530.16 149.04 Tm <617320> Tj 1 0 0 1 544.80 149.04 Tm <616E> Tj 0.48 Tc 1 0 0 1 332.64 137.28 Tm <456E6572677920> Tj 1 0 0 1 367.44 137.04 Tm <536F757263652C20> Tj 1 0 0 1 403.92 136.80 Tm <434E45532F556E69762E20> Tj 1 0 0 1 462.96 136.56 Tm <506F6974696572732C20> Tj 1 0 0 1 504.48 136.32 Tm <3130392D3132362E> Tj 0.72 Tc 1 0 0 1 318.48 124.32 Tm <48617274756E672C20> Tj 1 0 0 1 360.24 124.08 Tm <572E2C20> Tj 1 0 0 1 378.96 124.08 Tm <57656964656E626163682C20> Tj 1 0 0 1 440.64 123.60 Tm <472E2C20> Tj 1 0 0 1 456.96 123.60 Tm <616E6420> Tj 1 0 0 1 475.68 123.60 Tm <546965646B746B652C452E502E20> Tj 1 0 0 1 539.04 124.08 Tm <283139> Tj 0.48 Tc 1 0 0 1 332.88 111.36 Tm <3137292C20> Tj 1 0 0 1 353.04 111.36 Tm <4120> Tj 1 0 0 1 372.96 111.12 Tm <4E657720> Tj 1 0 0 1 405.84 110.88 Tm <436174616C7973747320> Tj 1 0 0 1 458.64 110.88 Tm <666F7220> Tj 1 0 0 1 483.36 110.64 Tm <4D6F6E6F70726F70656C6C616E74> Tj 0.48 Tc /F3 7.0 Tf 1 0 0 1 316.56 89.28 Tm <4E6F2E20> Tj 1 0 0 1 330.24 89.28 Tm <30332C20> Tj 1 0 0 1 343.92 89.28 Tm <70702E32373320> Tj 1 0 0 1 371.52 90.72 Tm <2D20> Tj 1 0 0 1 375.84 89.28 Tm <3238322C20> Tj 1 0 0 1 394.08 89.04 Tm <4A756C7920> Tj 1 0 0 1 410.40 90.72 Tm <2D20> Tj 1 0 0 1 414.72 89.04 Tm <53657074656E7462657220> Tj 1 0 0 1 451.20 89.04 Tm <32303033> Tj 0.48 Tc 1 0 0 1 140.64 90.24 Tm <496C72617A2E696C69616E20> Tj 1 0 0 1 172.80 90.00 Tm <4A6F756E6E6C20> Tj 1 0 0 1 200.88 89.76 Tm <6F6620> Tj 1 0 0 1 209.52 89.76 Tm <4368656D6963756C20> Tj 1 0 0 1 242.40 89.76 Tm <456E67696E656572696E672C20> Tj 1 0 0 1 287.28 89.52 Tm <566F6C2E32302C> Tj ET endstream endobj 71 0 obj 19447 endobj 72 0 obj << /Length 73 0 R >> stream / r-Ru/AlzO: Catalysts Used in Satellite Propulsion ., , , , | , , , , | , , , u1s , L r u Lr ru l ,r.ulg-r-rJ-r ,rr!'r: [, ,., rlurrJurrlt ruLru.d.rullrrulur,l-tar".rl.rlJ0 TIME 200 SFigure 5: Performance of S-Ru catalist in the last continuous firing. Ordinate axis range;1 - Temperature: 0 - 1000 oC: I - Line pressure: 0 - J0 bar:3 - Stagnation pressure in the chamber: - l-5 - l-i bar:4-Flowrate: 0-4e/s CONCLUSIONSThe results obtained in this work show that theruthenium-containing catalysts have problems suchas 50Vo faster mechanical degradation and a higherhydrazine decomposition instability. However, theyalso demonstrated that the performance of thesecatalysts was compatible with their use in short-period space applications that require a large amountof catalyst at a cost considerably lower than that ofconventiona IrlAlzOr catalysts. It seems that partialor total substitution of ruthenium for iridium incatalysts for the aforementioned reaction is a verypromising procedure. For these new products, itwould also be advisable to use alumina with a lowerspecific volume with the aim of increasing itsmechanical resistance.ACKNOWLEDGEMBNTSThe authors are indebted to Prof. Dr. GeraldDjga-Mariadassou at Laboratoire de Ractivit deSurface, Universit Pierre et Marie Curie, Paris forproviding the TEM analysis and to Dr. Jos AugustoJorge Rodrigues and Dra. Marisa AparecidaZacharias at Laboratrio Associado de Combusto ePropulso, Instituto Nacional de Pesquisas Espaciais,Brazil for preparing the alumina support. REFERENCESAltman, D. and Thomas, D.D. (1949), Evaluation ofHydrazine as a Monopropellant and a GasGenerate. CIT-JPL Pept. 9-36.Armstrong, W.E., Ryland, L.8., and Voge,H.H. (1978a), Catalyst for HydrazineDecomposition and Method for Preparing suchCatalyst. UK Patent Application GB 2.027.351.Armstrong, W.E., Ryland, L.8., and Voge, H.H.(1978b), Catalyst Comprising Ir or Ir and RuHydrazine Decomposition. United States Patent4.124.538.Armstrong, W.E., Ryland, L.B., and Voge, H. H.(1980), Catalyseur pour la Decomposition deI'Hydrazine. Brevet D'Invention N' 7.824. I 95.Cruz, G.M.; Cunha, D.S., and Soares Neto, T.G.(1989), Evoluo das Caractersticas Fsico-Qumicas de Catalisadores IrlAl2Oj co o Nmerode Impregnaes. 5o Seminrio Brasrleiro deCatlise, Guaruj - SP, Brazil, vol. 1, 216-224.Hartung, W. (1974), Evaluation Tests of NewGerman Catalysts for the SpontaneousDecomposition of Hydrazine. Proceedings of theInternational Conference on the Properties ofHydrazine and Its Potential Applications as anEnergy Source, CNES/Univ. Poitiers, 109-126.Hartung, W., Weidenbach, G., and Tiedktke,E.P. 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Proceedings of AOCSConference, Noordwij k.Narita,T., Miura, H., Ohira, M., Hondu, H..Sugiyama, K. Matsuda, T., and Gonzalez, R.D.(1987a), The Effect of Reduction Temperature onthe Chemisorptive Properties of Ru/Al:Or: Effectof Chlorine. Applied Catalysis, 32, 185- 190.Narita,T., Miura,H., Sugyama, K., Matsuda, T., andGonzalez, R.D (1987b), The Effect of ReductionTemperature on the Chemisorptive Properties ofRu/SiOz: Effect of Chlorine. Journal of Catalysis,103,492-495.Pfeffer, H.A. (1976), ESA Activities in the Field ofHydrazine Monopropellant Technology forSatellite Auxiliary Propulsion. ESA Scientific &Technical Review 2, 43.Schmidt, E.W. (1984), Hydrazine and Its Derivatives- Preparation, Properties, Applications. JohnWilev & Sons. Inc., New York. T.G.Soares Neto. J.Gobbo-Ferreira. A.J.G.Cobo and G.M.Cruz Soares Neto, T.G., Cruz, A .M.A ., Djega-Mariadassou,G., and Cruz. G.M. (1993), Comparao deCatalisadores Ir-Ru/Al1O. Preparados porImpregnaes Sucessivas e por Coimpregnao.7" Seminrio Brasiieiro de Catlise. Gramado,RS. Brazil. r'ol. 2. 329-310.Soares Neto, T.G. (1998), Catalisadores de IrlAl:Or eIr-RAl2Or para a Decomposio de Hidrazna. Ph.D.diss., Campinas State University, Campinas, Brazil.Soares Neto, T.G., Djega-Mariadassou, G., Cobo,A.J.C., and Cruz, G.M. (1999), Evoluo dePropriedades de Catalisadores Mono eBimetlicos de Ir e Ru Suportados em AluminaDurante o Emprego em Sistemas Micropropulsivosde Satlites. 10" Congresso Brasileiro de Catlise,Salvador, BA, Brazil, vol. 2, 154-161..Valentini, R. (1977), Hydrazine Thrusters for SpaceApplications. 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